Narrow-linewidth diamond single-photon sources prepared via femtosecond laser
Nitrogen-vacancy (NV) color centers in diamonds with narrow optical linewidths are commonly used as solid-state single-photon sources that emit indistinguishable photons. However, NV color centers prepared using ion implantation typically have large optical linewidths of over 100 MHz. Herein, we use...
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Veröffentlicht in: | Applied physics letters 2022-01, Vol.120 (2) |
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creator | Gao, Si Yin, Si-Yu Liu, Zhao-Xin Zhang, Zong-Da Tian, Zhen-Nan Chen, Qi-Dai Chen, Nian-Ke Sun, Hong-Bo |
description | Nitrogen-vacancy (NV) color centers in diamonds with narrow optical linewidths are commonly used as solid-state single-photon sources that emit indistinguishable photons. However, NV color centers prepared using ion implantation typically have large optical linewidths of over 100 MHz. Herein, we used the femtosecond laser direct writing (FsLDW) technique to prepare single NV color centers in diamond with a narrow optical linewidth of 13.05 ± 0.2 MHz and a long decoherence time of 445 ± 27.6 μs. In addition, the density functional theory was adopted to establish calculation models and illustrate why single NV color centers prepared by FsLDW have narrower linewidths compared to those of the ion implantation method. Thus, this study provides an effective reference for the preparation of narrow-linewidth single-color centers in diamonds and other wide-gap crystals. |
doi_str_mv | 10.1063/5.0079335 |
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However, NV color centers prepared using ion implantation typically have large optical linewidths of over 100 MHz. Herein, we used the femtosecond laser direct writing (FsLDW) technique to prepare single NV color centers in diamond with a narrow optical linewidth of 13.05 ± 0.2 MHz and a long decoherence time of 445 ± 27.6 μs. In addition, the density functional theory was adopted to establish calculation models and illustrate why single NV color centers prepared by FsLDW have narrower linewidths compared to those of the ion implantation method. Thus, this study provides an effective reference for the preparation of narrow-linewidth single-color centers in diamonds and other wide-gap crystals.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/5.0079335</identifier><identifier>CODEN: APPLAB</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Applied physics ; Color centers ; Density functional theory ; Diamonds ; Direct laser writing ; Ion implantation ; Photons</subject><ispartof>Applied physics letters, 2022-01, Vol.120 (2)</ispartof><rights>Author(s)</rights><rights>2022 Author(s). 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However, NV color centers prepared using ion implantation typically have large optical linewidths of over 100 MHz. Herein, we used the femtosecond laser direct writing (FsLDW) technique to prepare single NV color centers in diamond with a narrow optical linewidth of 13.05 ± 0.2 MHz and a long decoherence time of 445 ± 27.6 μs. In addition, the density functional theory was adopted to establish calculation models and illustrate why single NV color centers prepared by FsLDW have narrower linewidths compared to those of the ion implantation method. Thus, this study provides an effective reference for the preparation of narrow-linewidth single-color centers in diamonds and other wide-gap crystals.</description><subject>Applied physics</subject><subject>Color centers</subject><subject>Density functional theory</subject><subject>Diamonds</subject><subject>Direct laser writing</subject><subject>Ion implantation</subject><subject>Photons</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNqd0E1LAzEQBuAgCtbqwX-w4EkhNR-bTXKU4hdUveg5ZLOzNmW7WZO0xX_vlgrePQ0DD-8ML0KXlMwoqfitmBEiNefiCE0okRJzStUxmhBCOK60oKfoLKXVuArG-QS9vNoYww53voedb_KyaLxdh74pku8_O8DDMuTQFylsooNUDBEGG6Eptt4WLaxzSOD2vLMJ4jk6aW2X4OJ3TtHHw_37_Akv3h6f53cL7DiTGSvdyhZKIikjpauVspVgQMDVVuiqpo3gpXKsqZlSQlREKalrIkBoDbbkFZ-iq0PuEMPXBlI2q_G_fjxpWEWV5EJqMarrg3IxpBShNUP0axu_DSVm35YR5ret0d4cbHI-2-xD_z-8DfEPmqFp-Q8lP3gD</recordid><startdate>20220110</startdate><enddate>20220110</enddate><creator>Gao, Si</creator><creator>Yin, Si-Yu</creator><creator>Liu, Zhao-Xin</creator><creator>Zhang, Zong-Da</creator><creator>Tian, Zhen-Nan</creator><creator>Chen, Qi-Dai</creator><creator>Chen, Nian-Ke</creator><creator>Sun, Hong-Bo</creator><general>American Institute of Physics</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0003-2127-8610</orcidid><orcidid>https://orcid.org/0000-0002-6957-5721</orcidid></search><sort><creationdate>20220110</creationdate><title>Narrow-linewidth diamond single-photon sources prepared via femtosecond laser</title><author>Gao, Si ; Yin, Si-Yu ; Liu, Zhao-Xin ; Zhang, Zong-Da ; Tian, Zhen-Nan ; Chen, Qi-Dai ; Chen, Nian-Ke ; Sun, Hong-Bo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c327t-89f7fe4071204cb88a652e0ecba596b1d5348c2db28855608879b05e599ea4363</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Applied physics</topic><topic>Color centers</topic><topic>Density functional theory</topic><topic>Diamonds</topic><topic>Direct laser writing</topic><topic>Ion implantation</topic><topic>Photons</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gao, Si</creatorcontrib><creatorcontrib>Yin, Si-Yu</creatorcontrib><creatorcontrib>Liu, Zhao-Xin</creatorcontrib><creatorcontrib>Zhang, Zong-Da</creatorcontrib><creatorcontrib>Tian, Zhen-Nan</creatorcontrib><creatorcontrib>Chen, Qi-Dai</creatorcontrib><creatorcontrib>Chen, Nian-Ke</creatorcontrib><creatorcontrib>Sun, Hong-Bo</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gao, Si</au><au>Yin, Si-Yu</au><au>Liu, Zhao-Xin</au><au>Zhang, Zong-Da</au><au>Tian, Zhen-Nan</au><au>Chen, Qi-Dai</au><au>Chen, Nian-Ke</au><au>Sun, Hong-Bo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Narrow-linewidth diamond single-photon sources prepared via femtosecond laser</atitle><jtitle>Applied physics letters</jtitle><date>2022-01-10</date><risdate>2022</risdate><volume>120</volume><issue>2</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>Nitrogen-vacancy (NV) color centers in diamonds with narrow optical linewidths are commonly used as solid-state single-photon sources that emit indistinguishable photons. However, NV color centers prepared using ion implantation typically have large optical linewidths of over 100 MHz. Herein, we used the femtosecond laser direct writing (FsLDW) technique to prepare single NV color centers in diamond with a narrow optical linewidth of 13.05 ± 0.2 MHz and a long decoherence time of 445 ± 27.6 μs. In addition, the density functional theory was adopted to establish calculation models and illustrate why single NV color centers prepared by FsLDW have narrower linewidths compared to those of the ion implantation method. Thus, this study provides an effective reference for the preparation of narrow-linewidth single-color centers in diamonds and other wide-gap crystals.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/5.0079335</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0003-2127-8610</orcidid><orcidid>https://orcid.org/0000-0002-6957-5721</orcidid></addata></record> |
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subjects | Applied physics Color centers Density functional theory Diamonds Direct laser writing Ion implantation Photons |
title | Narrow-linewidth diamond single-photon sources prepared via femtosecond laser |
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