Four-mode multi-selection in the dual phase control of a molecular ionization induced by Fourier-synthesized laser fields
Coherent laser fields have been used to maximize the rate of a photochemical reaction or provide control over a single targeted property or function of matter by tuning of single-laser or multi-laser parameters. However, there is a need for multi-functionality control, albeit with as few parameters...
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| Veröffentlicht in: | Applied physics letters 2019-02, Vol.114 (5) |
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| container_title | Applied physics letters |
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| creator | Ohmura, Hideki Yoshida, Tsuyoshi Saito, Naoaki |
| description | Coherent laser fields have been used to maximize the rate of a photochemical reaction or provide control over a single targeted property or function of matter by tuning of single-laser or multi-laser parameters. However, there is a need for multi-functionality control, albeit with as few parameters as possible. Here, we report simultaneous control of molecular geometry (selection of molecular orientation) and electron dynamics (electron removal) with dual-phase control of Fourier-synthesized laser fields. Directionally asymmetric tunneling ionization induced by intense, nanosecond, three-color Fourier-synthesized laser fields led to four-mode selection with a combination of positive/negative orientation-selected and yield-enhanced/suppressed molecular ionization of carbonyl sulfide. |
| doi_str_mv | 10.1063/1.5082578 |
| format | Article |
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However, there is a need for multi-functionality control, albeit with as few parameters as possible. Here, we report simultaneous control of molecular geometry (selection of molecular orientation) and electron dynamics (electron removal) with dual-phase control of Fourier-synthesized laser fields. Directionally asymmetric tunneling ionization induced by intense, nanosecond, three-color Fourier-synthesized laser fields led to four-mode selection with a combination of positive/negative orientation-selected and yield-enhanced/suppressed molecular ionization of carbonyl sulfide.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/1.5082578</identifier><identifier>CODEN: APPLAB</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Applied physics ; Carbonyl sulfide ; Carbonyls ; Chemical synthesis ; Ionization ; Lasers ; Modal choice ; Parameters ; Phase control ; Photochemical reactions</subject><ispartof>Applied physics letters, 2019-02, Vol.114 (5)</ispartof><rights>Author(s)</rights><rights>2019 Author(s). 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Directionally asymmetric tunneling ionization induced by intense, nanosecond, three-color Fourier-synthesized laser fields led to four-mode selection with a combination of positive/negative orientation-selected and yield-enhanced/suppressed molecular ionization of carbonyl sulfide.</description><subject>Applied physics</subject><subject>Carbonyl sulfide</subject><subject>Carbonyls</subject><subject>Chemical synthesis</subject><subject>Ionization</subject><subject>Lasers</subject><subject>Modal choice</subject><subject>Parameters</subject><subject>Phase control</subject><subject>Photochemical reactions</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNp9kM1LwzAUwIMoOKcH_4OAJ4XOpGna9CjDqTDwoueQ5oNlpE1NWqH7683c0IPg6fEev_d7HwBcY7TAqCT3eEERy2nFTsAMo6rKCMbsFMwQQiQra4rPwUWM25TSnJAZmFZ-DFnrlYbt6AabRe20HKzvoO3gsNFQjcLBfiOihtJ3Q_AOegMFbH0CRycCTLDdiWOPGqVWsJngXmx1yOLUJU20u1R2yRKgsdqpeAnOjHBRXx3jHLyvHt-Wz9n69ell-bDOZJGzIaubWhBT0EZRwiRSmCGq6zovKlYYhZXQSpRIS0yEpILlBRGNNkgKRFlZSkPm4Obg7YP_GHUc-DZt1qWRPMcVLVlRE5qo2wMlg48xaMP7YFsRJo4R33-WY378bGLvDmyUdvi--wf-9OEX5L0y_8F_zV-z-4ln</recordid><startdate>20190204</startdate><enddate>20190204</enddate><creator>Ohmura, Hideki</creator><creator>Yoshida, Tsuyoshi</creator><creator>Saito, Naoaki</creator><general>American Institute of Physics</general><scope>AJDQP</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-5418-164X</orcidid><orcidid>https://orcid.org/0000-0001-8727-0377</orcidid></search><sort><creationdate>20190204</creationdate><title>Four-mode multi-selection in the dual phase control of a molecular ionization induced by Fourier-synthesized laser fields</title><author>Ohmura, Hideki ; Yoshida, Tsuyoshi ; Saito, Naoaki</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c428t-9b9a3f45bd538c0d1805e9924784fd1daeda60ec13ac5a8243abef0ca05866cf3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Applied physics</topic><topic>Carbonyl sulfide</topic><topic>Carbonyls</topic><topic>Chemical synthesis</topic><topic>Ionization</topic><topic>Lasers</topic><topic>Modal choice</topic><topic>Parameters</topic><topic>Phase control</topic><topic>Photochemical reactions</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ohmura, Hideki</creatorcontrib><creatorcontrib>Yoshida, Tsuyoshi</creatorcontrib><creatorcontrib>Saito, Naoaki</creatorcontrib><collection>AIP Open Access Journals</collection><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ohmura, Hideki</au><au>Yoshida, Tsuyoshi</au><au>Saito, Naoaki</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Four-mode multi-selection in the dual phase control of a molecular ionization induced by Fourier-synthesized laser fields</atitle><jtitle>Applied physics letters</jtitle><date>2019-02-04</date><risdate>2019</risdate><volume>114</volume><issue>5</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>Coherent laser fields have been used to maximize the rate of a photochemical reaction or provide control over a single targeted property or function of matter by tuning of single-laser or multi-laser parameters. 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| ispartof | Applied physics letters, 2019-02, Vol.114 (5) |
| issn | 0003-6951 1077-3118 |
| language | eng |
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| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | Applied physics Carbonyl sulfide Carbonyls Chemical synthesis Ionization Lasers Modal choice Parameters Phase control Photochemical reactions |
| title | Four-mode multi-selection in the dual phase control of a molecular ionization induced by Fourier-synthesized laser fields |
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