Phase control of plasmon enhanced two-photon photoluminescence in resonant gold nanoantennas

Plasmonic nanoantennas emit two-photon photoluminescence, which is much stronger than their second harmonic generation. Unfortunately, luminescence is an incoherent process and therefore generally not explored for nanoscale coherent control of the antenna response. Here, we demonstrate that, in reso...

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Veröffentlicht in:Applied physics letters 2018-11, Vol.113 (21)
Hauptverfasser: Remesh, Vikas, Stührenberg, Michael, Saemisch, Lisa, Accanto, Nicolò, van Hulst, Niek F.
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container_issue 21
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container_title Applied physics letters
container_volume 113
creator Remesh, Vikas
Stührenberg, Michael
Saemisch, Lisa
Accanto, Nicolò
van Hulst, Niek F.
description Plasmonic nanoantennas emit two-photon photoluminescence, which is much stronger than their second harmonic generation. Unfortunately, luminescence is an incoherent process and therefore generally not explored for nanoscale coherent control of the antenna response. Here, we demonstrate that, in resonant gold nanoantennas, the two-photon absorption process can be coherent, provided that the excitation pulse duration is shorter than the dephasing time of plasmon mode oscillation. Exploiting this coherent response, we show the pure spectral phase control of resonant gold nanoantennas, with effective read-out of the two-photon photoluminescence.
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subjects Applied physics
Coherence
Gold
Nanoantennas
Phase control
Photoluminescence
Photon absorption
Pulse duration
Second harmonic generation
title Phase control of plasmon enhanced two-photon photoluminescence in resonant gold nanoantennas
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