Phase control of plasmon enhanced two-photon photoluminescence in resonant gold nanoantennas
Plasmonic nanoantennas emit two-photon photoluminescence, which is much stronger than their second harmonic generation. Unfortunately, luminescence is an incoherent process and therefore generally not explored for nanoscale coherent control of the antenna response. Here, we demonstrate that, in reso...
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Veröffentlicht in: | Applied physics letters 2018-11, Vol.113 (21) |
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creator | Remesh, Vikas Stührenberg, Michael Saemisch, Lisa Accanto, Nicolò van Hulst, Niek F. |
description | Plasmonic nanoantennas emit two-photon photoluminescence, which is much stronger than their second harmonic generation. Unfortunately, luminescence is an incoherent process and therefore generally not explored for nanoscale coherent control of the antenna response. Here, we demonstrate that, in resonant gold nanoantennas, the two-photon absorption process can be coherent, provided that the excitation pulse duration is shorter than the dephasing time of plasmon mode oscillation. Exploiting this coherent response, we show the pure spectral phase control of resonant gold nanoantennas, with effective read-out of the two-photon photoluminescence. |
doi_str_mv | 10.1063/1.5051381 |
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Exploiting this coherent response, we show the pure spectral phase control of resonant gold nanoantennas, with effective read-out of the two-photon photoluminescence.</description><subject>Applied physics</subject><subject>Coherence</subject><subject>Gold</subject><subject>Nanoantennas</subject><subject>Phase control</subject><subject>Photoluminescence</subject><subject>Photon absorption</subject><subject>Pulse duration</subject><subject>Second harmonic generation</subject><issn>0003-6951</issn><issn>1077-3118</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>D8T</sourceid><recordid>eNqdkV1rFTEQhoNY8Fi98B8EvFLYOslsPvZSilWhYEG9E0I2O-tu2ZOsyZ6W_ntTz0HvvXrn4-GdGYaxVwIuBGh8Jy4UKIFWPGE7AcY0KIR9ynYAgI3ulHjGnpdyW1MlEXfsx83kC_GQ4pbTwtPI18WXfYqc4uRjoIFv96lZp7TV2h9ZDvs5UglUu3yOPFNJ0ceN_0zLwGuUakIx-vKCnY1-KfTypOfs-9WHb5efmusvHz9fvr9uQot2a4QF1EoqDYMF2bUy6EH0hmTfWU8yiA56OahWK98CSexHoF4HP-pK9GjwnH09-pZ7Wg-9W_O89_nBJT-7uh35HCYXJr_sKRdXyLXCgGw77dAiulYP5OxgvEM1ku7BmmpdXV8fXdecfh2obO42HXKshzgpUBkLpn2k3hypkFMpmca_0wW4x5c44U4vqezb055h3vw2p_h_8F3K_0C3DiP-Bilamf0</recordid><startdate>20181119</startdate><enddate>20181119</enddate><creator>Remesh, Vikas</creator><creator>Stührenberg, Michael</creator><creator>Saemisch, Lisa</creator><creator>Accanto, Nicolò</creator><creator>van Hulst, Niek F.</creator><general>American Institute of Physics</general><scope>AJDQP</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>ABBSD</scope><scope>ADTPV</scope><scope>AOWAS</scope><scope>D8T</scope><scope>F1S</scope><scope>ZZAVC</scope><orcidid>https://orcid.org/0000-0003-4630-1776</orcidid></search><sort><creationdate>20181119</creationdate><title>Phase control of plasmon enhanced two-photon photoluminescence in resonant gold nanoantennas</title><author>Remesh, Vikas ; Stührenberg, Michael ; Saemisch, Lisa ; Accanto, Nicolò ; van Hulst, Niek F.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c438t-1803652560d802942c6d1b7e2b98ae2c190b2d5465a40e23bf0eb6caf62b9b373</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Applied physics</topic><topic>Coherence</topic><topic>Gold</topic><topic>Nanoantennas</topic><topic>Phase control</topic><topic>Photoluminescence</topic><topic>Photon absorption</topic><topic>Pulse duration</topic><topic>Second harmonic generation</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Remesh, Vikas</creatorcontrib><creatorcontrib>Stührenberg, Michael</creatorcontrib><creatorcontrib>Saemisch, Lisa</creatorcontrib><creatorcontrib>Accanto, Nicolò</creatorcontrib><creatorcontrib>van Hulst, Niek F.</creatorcontrib><collection>AIP Open Access Journals</collection><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>SWEPUB Chalmers tekniska högskola full text</collection><collection>SwePub</collection><collection>SwePub Articles</collection><collection>SWEPUB Freely available online</collection><collection>SWEPUB Chalmers tekniska högskola</collection><collection>SwePub Articles full text</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Remesh, Vikas</au><au>Stührenberg, Michael</au><au>Saemisch, Lisa</au><au>Accanto, Nicolò</au><au>van Hulst, Niek F.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Phase control of plasmon enhanced two-photon photoluminescence in resonant gold nanoantennas</atitle><jtitle>Applied physics letters</jtitle><date>2018-11-19</date><risdate>2018</risdate><volume>113</volume><issue>21</issue><issn>0003-6951</issn><issn>1077-3118</issn><eissn>1077-3118</eissn><coden>APPLAB</coden><abstract>Plasmonic nanoantennas emit two-photon photoluminescence, which is much stronger than their second harmonic generation. Unfortunately, luminescence is an incoherent process and therefore generally not explored for nanoscale coherent control of the antenna response. Here, we demonstrate that, in resonant gold nanoantennas, the two-photon absorption process can be coherent, provided that the excitation pulse duration is shorter than the dephasing time of plasmon mode oscillation. Exploiting this coherent response, we show the pure spectral phase control of resonant gold nanoantennas, with effective read-out of the two-photon photoluminescence.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/1.5051381</doi><tpages>5</tpages><orcidid>https://orcid.org/0000-0003-4630-1776</orcidid><oa>free_for_read</oa></addata></record> |
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subjects | Applied physics Coherence Gold Nanoantennas Phase control Photoluminescence Photon absorption Pulse duration Second harmonic generation |
title | Phase control of plasmon enhanced two-photon photoluminescence in resonant gold nanoantennas |
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