Photocatalytic activity of silver oxide capped Ag nanoparticles constructed by air plasma irradiation

Photocatalytic activity of silver oxide capped Ag nanoparticles constructed by air plasma irradiation

We construct a kind of structure of silver oxide capped silver nanoparticles (AgNPs) by cost-efficient air plasma irradiation, and study its visible-light driven photocatalytic activity (PA). By controlling the oxidization time, the relationship between the intensity of the localized surface plasmon...

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Veröffentlicht in:Applied physics letters 2018-04, Vol.112 (16)
Hauptverfasser: Fang, Yingcui, Wu, Qingmeng, Li, Huanhuan, Zhang, Bing, Yan, Rong, Chen, Junling, Sun, Mengtao
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container_issue 16
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container_title Applied physics letters
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creator Fang, Yingcui
Wu, Qingmeng
Li, Huanhuan
Zhang, Bing
Yan, Rong
Chen, Junling
Sun, Mengtao
description We construct a kind of structure of silver oxide capped silver nanoparticles (AgNPs) by cost-efficient air plasma irradiation, and study its visible-light driven photocatalytic activity (PA). By controlling the oxidization time, the relationship between the intensity of the localized surface plasmon resonance (LSPR) and the PA is well established. The PA reaches the maximum when the LSPR of AgNPs is nearly completely damped (according to absorption spectra); however, under this condition, the LSPR still works, confirmed with the high efficient selective transformation of p-Aminothiophenol (PATP) to p, p′-dimercaptoazobenzene (DMAB) under visible light. The mechanism of the LSPR damping induced PA improvement is discussed. We not only provide a cost-efficient approach to construct a LSPR strong damping structure but also promote the understanding of LSPR strong damping and its relationship with photocatalysis.
doi_str_mv 10.1063/1.5024770
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title Photocatalytic activity of silver oxide capped Ag nanoparticles constructed by air plasma irradiation
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