Wavelength-resolved stimulated photon echoes: Direct observation of ultrafast intramolecular vibrational contributions to electronic dephasing

Novel wavelength-resolved stimulated photon echo measurements on a dye molecule in solution are presented. Data are simulated within the multimode Brownian oscillator model using the spectral density of de Boeij et al. [J. Phys. Chem. 100, 11806 (1996)] for the same solute–solvent system. For photon...

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Veröffentlicht in:The Journal of chemical physics 1999-07, Vol.111 (3), p.792-795
Hauptverfasser: Book, Lewis D., Scherer, Norbert F.
Format: Artikel
Sprache:eng
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Zusammenfassung:Novel wavelength-resolved stimulated photon echo measurements on a dye molecule in solution are presented. Data are simulated within the multimode Brownian oscillator model using the spectral density of de Boeij et al. [J. Phys. Chem. 100, 11806 (1996)] for the same solute–solvent system. For photon echo population times
ISSN:0021-9606
1089-7690
DOI:10.1063/1.479366