Giant second-order Zeeman effect in titanium (III) doped caesium gallium alum

Giant second-order Zeeman effect in titanium (III) doped caesium gallium alum

Low temperature magnetization data obtained for titanium (III) doped caesium gallium alum show a spectacular deviation from Brillouin behavior with the magnetization highly dependent on the strength of the applied field at a given value of B/T. This arises from unprecedented higher-order contributio...

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Veröffentlicht in:The Journal of chemical physics 1998-08, Vol.109 (8), p.2967-2970
Hauptverfasser: Tregenna-Piggott, Philip L. W., O’Brien, Mary C. M., Weihe, Ho/gni, Güdel, Hans U.
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container_end_page 2970
container_issue 8
container_start_page 2967
container_title The Journal of chemical physics
container_volume 109
creator Tregenna-Piggott, Philip L. W.
O’Brien, Mary C. M.
Weihe, Ho/gni
Güdel, Hans U.
description Low temperature magnetization data obtained for titanium (III) doped caesium gallium alum show a spectacular deviation from Brillouin behavior with the magnetization highly dependent on the strength of the applied field at a given value of B/T. This arises from unprecedented higher-order contributions to the magnetization and these measurements afford the determination of the Zeeman coefficients to third order. This anomalous magnetic behavior is a manifestation of Jahn-Teller coupling giving rise to low-lying vibronic states which mix into the ground state through the magnetic field.
doi_str_mv 10.1063/1.476885
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title Giant second-order Zeeman effect in titanium (III) doped caesium gallium alum
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