Dynamic Monte Carlo simulations of dense polymer systems on the tetrahedral lattice: a liquid-glass-type transition
The mean square displacement of chain beads, 〈R2i (t)〉 has been studied for systems having total bead densities in the range 0.875 to 0.980. On increasing the density, the bead diffusion presents a sharp step from a liquid-like behavior to a glass-like one. Such a transition is observed for systems...
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| Veröffentlicht in: | The Journal of chemical physics 1984-01, Vol.81 (1), p.567-570 |
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| container_end_page | 570 |
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| container_issue | 1 |
| container_start_page | 567 |
| container_title | The Journal of chemical physics |
| container_volume | 81 |
| creator | DEJEAN DE LA BATIE, R VIOVY, J.-L MONNERIE, L |
| description | The mean square displacement of chain beads, 〈R2i (t)〉 has been studied for systems having total bead densities in the range 0.875 to 0.980. On increasing the density, the bead diffusion presents a sharp step from a liquid-like behavior to a glass-like one. Such a transition is observed for systems containing either chains only or chains and free beads, but in this latter case it occurs at a higher total density. Furthermore, this transition has some geometrical features of a dynamic percolation and shows similarities to the equilibrium liquid-glass transition theory proposed by Cohen and Grest. |
| doi_str_mv | 10.1063/1.447339 |
| format | Article |
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| fulltext | fulltext |
| identifier | ISSN: 0021-9606 |
| ispartof | The Journal of chemical physics, 1984-01, Vol.81 (1), p.567-570 |
| issn | 0021-9606 1089-7690 |
| language | eng |
| recordid | cdi_crossref_primary_10_1063_1_447339 |
| source | AIP Digital Archive |
| subjects | Applied sciences Exact sciences and technology Organic polymers Physicochemistry of polymers Properties and characterization |
| title | Dynamic Monte Carlo simulations of dense polymer systems on the tetrahedral lattice: a liquid-glass-type transition |
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