Laser ablation of bicomponent systems: A probe of molecular ejection mechanisms

A combined experimental and molecular dynamics simulation study of laser ablation of a model bicomponent system with solutes of different volatility provides a consistent picture of the mechanisms of material ejection. The comparison of the ejection yields shows that there are two distinct regimes o...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Applied physics letters 2001-03, Vol.78 (11), p.1631-1633
Hauptverfasser: Yingling, Yaroslava G., Zhigilei, Leonid V., Garrison, Barbara J., Koubenakis, Antonis, Labrakis, John, Georgiou, Savas
Format: Artikel
Sprache:eng
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 1633
container_issue 11
container_start_page 1631
container_title Applied physics letters
container_volume 78
creator Yingling, Yaroslava G.
Zhigilei, Leonid V.
Garrison, Barbara J.
Koubenakis, Antonis
Labrakis, John
Georgiou, Savas
description A combined experimental and molecular dynamics simulation study of laser ablation of a model bicomponent system with solutes of different volatility provides a consistent picture of the mechanisms of material ejection. The comparison of the ejection yields shows that there are two distinct regimes of molecular ejection, desorption at low laser fluences, and a collective ejection of a volume of material or ablation at higher fluences. Ejection of volatile solutes dominates in the desorption regime, whereas nonvolatile solutes are ejected only in the ablation regime.
doi_str_mv 10.1063/1.1353816
format Article
fullrecord <record><control><sourceid>crossref</sourceid><recordid>TN_cdi_crossref_primary_10_1063_1_1353816</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>10_1063_1_1353816</sourcerecordid><originalsourceid>FETCH-LOGICAL-c227t-af2b608c69548fb740b6242c4e9451d4054b7ebf5c4a55472b28692b054cab53</originalsourceid><addsrcrecordid>eNotUDtrwzAYFKWFummH_gOtHZzq09PuFkJfYMiS3UjqJ-pgWUZyh_z7Jm2m4-644zhCHoGtgWnxDGsQSjSgr0gFzJhaADTXpGKMiVq3Cm7JXSmHE1VciIrsOlswU-tGuwxpoilQN_gU5zThtNByLAvG8kI3dM7J4dmPaUT_M9pM8YD-LxXRf9tpKLHck5tgx4IPF1yR_dvrfvtRd7v3z-2mqz3nZqlt4E6zxp8WySY4I5nTXHIvsZUKviRT0hl0QXlplZKGO97olruT7q1TYkWe_mt9TqVkDP2ch2jzsQfWn4_oob8cIX4B8NxPwg</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Laser ablation of bicomponent systems: A probe of molecular ejection mechanisms</title><source>AIP Journals Complete</source><source>AIP Digital Archive</source><creator>Yingling, Yaroslava G. ; Zhigilei, Leonid V. ; Garrison, Barbara J. ; Koubenakis, Antonis ; Labrakis, John ; Georgiou, Savas</creator><creatorcontrib>Yingling, Yaroslava G. ; Zhigilei, Leonid V. ; Garrison, Barbara J. ; Koubenakis, Antonis ; Labrakis, John ; Georgiou, Savas</creatorcontrib><description>A combined experimental and molecular dynamics simulation study of laser ablation of a model bicomponent system with solutes of different volatility provides a consistent picture of the mechanisms of material ejection. The comparison of the ejection yields shows that there are two distinct regimes of molecular ejection, desorption at low laser fluences, and a collective ejection of a volume of material or ablation at higher fluences. Ejection of volatile solutes dominates in the desorption regime, whereas nonvolatile solutes are ejected only in the ablation regime.</description><identifier>ISSN: 0003-6951</identifier><identifier>EISSN: 1077-3118</identifier><identifier>DOI: 10.1063/1.1353816</identifier><language>eng</language><ispartof>Applied physics letters, 2001-03, Vol.78 (11), p.1631-1633</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c227t-af2b608c69548fb740b6242c4e9451d4054b7ebf5c4a55472b28692b054cab53</citedby><cites>FETCH-LOGICAL-c227t-af2b608c69548fb740b6242c4e9451d4054b7ebf5c4a55472b28692b054cab53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27903,27904</link.rule.ids></links><search><creatorcontrib>Yingling, Yaroslava G.</creatorcontrib><creatorcontrib>Zhigilei, Leonid V.</creatorcontrib><creatorcontrib>Garrison, Barbara J.</creatorcontrib><creatorcontrib>Koubenakis, Antonis</creatorcontrib><creatorcontrib>Labrakis, John</creatorcontrib><creatorcontrib>Georgiou, Savas</creatorcontrib><title>Laser ablation of bicomponent systems: A probe of molecular ejection mechanisms</title><title>Applied physics letters</title><description>A combined experimental and molecular dynamics simulation study of laser ablation of a model bicomponent system with solutes of different volatility provides a consistent picture of the mechanisms of material ejection. The comparison of the ejection yields shows that there are two distinct regimes of molecular ejection, desorption at low laser fluences, and a collective ejection of a volume of material or ablation at higher fluences. Ejection of volatile solutes dominates in the desorption regime, whereas nonvolatile solutes are ejected only in the ablation regime.</description><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2001</creationdate><recordtype>article</recordtype><recordid>eNotUDtrwzAYFKWFummH_gOtHZzq09PuFkJfYMiS3UjqJ-pgWUZyh_z7Jm2m4-644zhCHoGtgWnxDGsQSjSgr0gFzJhaADTXpGKMiVq3Cm7JXSmHE1VciIrsOlswU-tGuwxpoilQN_gU5zThtNByLAvG8kI3dM7J4dmPaUT_M9pM8YD-LxXRf9tpKLHck5tgx4IPF1yR_dvrfvtRd7v3z-2mqz3nZqlt4E6zxp8WySY4I5nTXHIvsZUKviRT0hl0QXlplZKGO97olruT7q1TYkWe_mt9TqVkDP2ch2jzsQfWn4_oob8cIX4B8NxPwg</recordid><startdate>20010312</startdate><enddate>20010312</enddate><creator>Yingling, Yaroslava G.</creator><creator>Zhigilei, Leonid V.</creator><creator>Garrison, Barbara J.</creator><creator>Koubenakis, Antonis</creator><creator>Labrakis, John</creator><creator>Georgiou, Savas</creator><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20010312</creationdate><title>Laser ablation of bicomponent systems: A probe of molecular ejection mechanisms</title><author>Yingling, Yaroslava G. ; Zhigilei, Leonid V. ; Garrison, Barbara J. ; Koubenakis, Antonis ; Labrakis, John ; Georgiou, Savas</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c227t-af2b608c69548fb740b6242c4e9451d4054b7ebf5c4a55472b28692b054cab53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2001</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yingling, Yaroslava G.</creatorcontrib><creatorcontrib>Zhigilei, Leonid V.</creatorcontrib><creatorcontrib>Garrison, Barbara J.</creatorcontrib><creatorcontrib>Koubenakis, Antonis</creatorcontrib><creatorcontrib>Labrakis, John</creatorcontrib><creatorcontrib>Georgiou, Savas</creatorcontrib><collection>CrossRef</collection><jtitle>Applied physics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yingling, Yaroslava G.</au><au>Zhigilei, Leonid V.</au><au>Garrison, Barbara J.</au><au>Koubenakis, Antonis</au><au>Labrakis, John</au><au>Georgiou, Savas</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Laser ablation of bicomponent systems: A probe of molecular ejection mechanisms</atitle><jtitle>Applied physics letters</jtitle><date>2001-03-12</date><risdate>2001</risdate><volume>78</volume><issue>11</issue><spage>1631</spage><epage>1633</epage><pages>1631-1633</pages><issn>0003-6951</issn><eissn>1077-3118</eissn><abstract>A combined experimental and molecular dynamics simulation study of laser ablation of a model bicomponent system with solutes of different volatility provides a consistent picture of the mechanisms of material ejection. The comparison of the ejection yields shows that there are two distinct regimes of molecular ejection, desorption at low laser fluences, and a collective ejection of a volume of material or ablation at higher fluences. Ejection of volatile solutes dominates in the desorption regime, whereas nonvolatile solutes are ejected only in the ablation regime.</abstract><doi>10.1063/1.1353816</doi><tpages>3</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0003-6951
ispartof Applied physics letters, 2001-03, Vol.78 (11), p.1631-1633
issn 0003-6951
1077-3118
language eng
recordid cdi_crossref_primary_10_1063_1_1353816
source AIP Journals Complete; AIP Digital Archive
title Laser ablation of bicomponent systems: A probe of molecular ejection mechanisms
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-23T10%3A56%3A58IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-crossref&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Laser%20ablation%20of%20bicomponent%20systems:%20A%20probe%20of%20molecular%20ejection%20mechanisms&rft.jtitle=Applied%20physics%20letters&rft.au=Yingling,%20Yaroslava%20G.&rft.date=2001-03-12&rft.volume=78&rft.issue=11&rft.spage=1631&rft.epage=1633&rft.pages=1631-1633&rft.issn=0003-6951&rft.eissn=1077-3118&rft_id=info:doi/10.1063/1.1353816&rft_dat=%3Ccrossref%3E10_1063_1_1353816%3C/crossref%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true