Mg ions intercalated with V 3 O 7 ·H 2 O to construct ultrastable cathode materials for aqueous zinc-ion batteries
V O ·H O (VO) stands out as a highly promising cathode material for aqueous zinc-ion batteries (AZIB). However, due to the instability of the VO structure and the limited ion transport rate, achieving the required specific capacity and extended cycling lifespan has been challenging. To tackle this i...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2024-08, Vol.60 (65), p.8597-8600 |
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| container_title | Chemical communications (Cambridge, England) |
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| creator | Shi, Yaowen Yin, Bosi Sun, Ying Ge, Rongyuan Hu, Yingfang Li, Jiazhuo Li, Hui Zhang, Siwen Ma, Tianyi |
| description | V
O
·H
O (VO) stands out as a highly promising cathode material for aqueous zinc-ion batteries (AZIB). However, due to the instability of the VO structure and the limited ion transport rate, achieving the required specific capacity and extended cycling lifespan has been challenging. To tackle this issue, we synthesized Mg-ion intercalated VO (MgVO) using a straightforward hydrothermal method. Introducing Mg
as an interlayer support enhanced the flexibility of MgVO within the confined layer space, stabilized its lamellar structure, and expanded the VO layer spacing. The AZIB employing the MgVO cathode demonstrated a high specific capacity of 382.7 mA h g
at a current density of 0.1 A g
and showed excellent cycling stability. The robust structural stability of MgVO suggests promising applications for large-scale energy storage, while the Mg
intercalation strategy presents a novel approach for exploring other potential cathode materials. |
| doi_str_mv | 10.1039/d4cc03201b |
| format | Article |
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O
·H
O (VO) stands out as a highly promising cathode material for aqueous zinc-ion batteries (AZIB). However, due to the instability of the VO structure and the limited ion transport rate, achieving the required specific capacity and extended cycling lifespan has been challenging. To tackle this issue, we synthesized Mg-ion intercalated VO (MgVO) using a straightforward hydrothermal method. Introducing Mg
as an interlayer support enhanced the flexibility of MgVO within the confined layer space, stabilized its lamellar structure, and expanded the VO layer spacing. The AZIB employing the MgVO cathode demonstrated a high specific capacity of 382.7 mA h g
at a current density of 0.1 A g
and showed excellent cycling stability. The robust structural stability of MgVO suggests promising applications for large-scale energy storage, while the Mg
intercalation strategy presents a novel approach for exploring other potential cathode materials.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d4cc03201b</identifier><identifier>PMID: 39045830</identifier><language>eng</language><publisher>England</publisher><ispartof>Chemical communications (Cambridge, England), 2024-08, Vol.60 (65), p.8597-8600</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c580-b8b069e46001f8420a1d5fb0e67075bf3c5d7762c66cddc3089a6e783e3d3f9c3</cites><orcidid>0000-0002-1042-8700</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27922,27923</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/39045830$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Shi, Yaowen</creatorcontrib><creatorcontrib>Yin, Bosi</creatorcontrib><creatorcontrib>Sun, Ying</creatorcontrib><creatorcontrib>Ge, Rongyuan</creatorcontrib><creatorcontrib>Hu, Yingfang</creatorcontrib><creatorcontrib>Li, Jiazhuo</creatorcontrib><creatorcontrib>Li, Hui</creatorcontrib><creatorcontrib>Zhang, Siwen</creatorcontrib><creatorcontrib>Ma, Tianyi</creatorcontrib><title>Mg ions intercalated with V 3 O 7 ·H 2 O to construct ultrastable cathode materials for aqueous zinc-ion batteries</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>V
O
·H
O (VO) stands out as a highly promising cathode material for aqueous zinc-ion batteries (AZIB). However, due to the instability of the VO structure and the limited ion transport rate, achieving the required specific capacity and extended cycling lifespan has been challenging. To tackle this issue, we synthesized Mg-ion intercalated VO (MgVO) using a straightforward hydrothermal method. Introducing Mg
as an interlayer support enhanced the flexibility of MgVO within the confined layer space, stabilized its lamellar structure, and expanded the VO layer spacing. The AZIB employing the MgVO cathode demonstrated a high specific capacity of 382.7 mA h g
at a current density of 0.1 A g
and showed excellent cycling stability. The robust structural stability of MgVO suggests promising applications for large-scale energy storage, while the Mg
intercalation strategy presents a novel approach for exploring other potential cathode materials.</description><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNo9kMtOwzAQRS0EoqWw4QPQrJECTvyIs4TwlIq6qRC7yE8alDbFdoTgx9jzZbgUmM1cac7MHV2EjnN8lmNSnRuqNSYFztUOGueE04xR8bS70azKSkLZCB2E8IJT5UzsoxGpMGWC4DEKD8_Q9qsA7Spar2UnozXw1sYFPAKBGZTw9XkHRVKxB53I6AcdYeiilyFK1VnQMi56Y2GZdn0ruwCu9yBfB9sPAT7alc6SBSgZN3MbDtGeS5Q9-u0TNL-5ntd32XR2e19fTDPNBM6UUJhXlvL0tBO0wDI3zClseYlLphzRzJQlLzTn2hhNsKgkt6UglhjiKk0m6HR7Vvs-BG9ds_btUvr3JsfNJrjmitb1T3CXCT7ZwutBLa35R_-SIt9L2GmA</recordid><startdate>20240809</startdate><enddate>20240809</enddate><creator>Shi, Yaowen</creator><creator>Yin, Bosi</creator><creator>Sun, Ying</creator><creator>Ge, Rongyuan</creator><creator>Hu, Yingfang</creator><creator>Li, Jiazhuo</creator><creator>Li, Hui</creator><creator>Zhang, Siwen</creator><creator>Ma, Tianyi</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-1042-8700</orcidid></search><sort><creationdate>20240809</creationdate><title>Mg ions intercalated with V 3 O 7 ·H 2 O to construct ultrastable cathode materials for aqueous zinc-ion batteries</title><author>Shi, Yaowen ; Yin, Bosi ; Sun, Ying ; Ge, Rongyuan ; Hu, Yingfang ; Li, Jiazhuo ; Li, Hui ; Zhang, Siwen ; Ma, Tianyi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c580-b8b069e46001f8420a1d5fb0e67075bf3c5d7762c66cddc3089a6e783e3d3f9c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Shi, Yaowen</creatorcontrib><creatorcontrib>Yin, Bosi</creatorcontrib><creatorcontrib>Sun, Ying</creatorcontrib><creatorcontrib>Ge, Rongyuan</creatorcontrib><creatorcontrib>Hu, Yingfang</creatorcontrib><creatorcontrib>Li, Jiazhuo</creatorcontrib><creatorcontrib>Li, Hui</creatorcontrib><creatorcontrib>Zhang, Siwen</creatorcontrib><creatorcontrib>Ma, Tianyi</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Shi, Yaowen</au><au>Yin, Bosi</au><au>Sun, Ying</au><au>Ge, Rongyuan</au><au>Hu, Yingfang</au><au>Li, Jiazhuo</au><au>Li, Hui</au><au>Zhang, Siwen</au><au>Ma, Tianyi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Mg ions intercalated with V 3 O 7 ·H 2 O to construct ultrastable cathode materials for aqueous zinc-ion batteries</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2024-08-09</date><risdate>2024</risdate><volume>60</volume><issue>65</issue><spage>8597</spage><epage>8600</epage><pages>8597-8600</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>V
O
·H
O (VO) stands out as a highly promising cathode material for aqueous zinc-ion batteries (AZIB). However, due to the instability of the VO structure and the limited ion transport rate, achieving the required specific capacity and extended cycling lifespan has been challenging. To tackle this issue, we synthesized Mg-ion intercalated VO (MgVO) using a straightforward hydrothermal method. Introducing Mg
as an interlayer support enhanced the flexibility of MgVO within the confined layer space, stabilized its lamellar structure, and expanded the VO layer spacing. The AZIB employing the MgVO cathode demonstrated a high specific capacity of 382.7 mA h g
at a current density of 0.1 A g
and showed excellent cycling stability. The robust structural stability of MgVO suggests promising applications for large-scale energy storage, while the Mg
intercalation strategy presents a novel approach for exploring other potential cathode materials.</abstract><cop>England</cop><pmid>39045830</pmid><doi>10.1039/d4cc03201b</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0002-1042-8700</orcidid></addata></record> |
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| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2024-08, Vol.60 (65), p.8597-8600 |
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| language | eng |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | Mg ions intercalated with V 3 O 7 ·H 2 O to construct ultrastable cathode materials for aqueous zinc-ion batteries |
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