Why surface hydrophobicity promotes CO 2 electroreduction: a case study of hydrophobic polymer N -heterocyclic carbenes

We report the use of polymer N -heterocyclic carbenes (NHCs) to control the microenvironment surrounding metal nanocatalysts, thereby enhancing their catalytic performance in CO 2 electroreduction. Three polymer NHC ligands were designed with different hydrophobicity: hydrophilic poly(ethylene oxide...

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Veröffentlicht in:Chemical science (Cambridge) 2023-09, Vol.14 (36), p.9664-9677
Hauptverfasser: Luo, Qiang, Duan, Hanyi, McLaughlin, Michael C., Wei, Kecheng, Tapia, Joseph, Adewuyi, Joseph A., Shuster, Seth, Liaqat, Maham, Suib, Steven L., Ung, Gaël, Bai, Peng, Sun, Shouheng, He, Jie
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Sprache:eng
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