NiFe-LDH/g-C 3 N 4 binary heterostructures with 2D/2D configuration for highly efficient photocatalytic degradation of antibiotics and hydrogen production

NiFe-LDH/g-C 3 N 4 binary heterostructures with 2D/2D configuration for highly efficient photocatalytic degradation of antibiotics and hydrogen production

NiFe-LDH/g-C 3 N 4 (LDH/CN) heterostructures with different amounts of NiFe-LDH (LDH) were prepared by a hydrothermal method and characterized using different experimental techniques. Their photocatalytic properties were investigated using the degradation of tetracycline hydrochloride (TC) and the p...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:CrystEngComm 2024-01, Vol.26 (4), p.532-542
Hauptverfasser: Jia, Yujie, Jiang, Shuhan, Ou, Qianchen, Liu, Yanan, Zhang, Jian, Zhou, Yangjie, Lian, Yuan, Wang, Hongmei
Format: Artikel
Sprache:eng
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 542
container_issue 4
container_start_page 532
container_title CrystEngComm
container_volume 26
creator Jia, Yujie
Jiang, Shuhan
Ou, Qianchen
Liu, Yanan
Zhang, Jian
Zhou, Yangjie
Lian, Yuan
Wang, Hongmei
description NiFe-LDH/g-C 3 N 4 (LDH/CN) heterostructures with different amounts of NiFe-LDH (LDH) were prepared by a hydrothermal method and characterized using different experimental techniques. Their photocatalytic properties were investigated using the degradation of tetracycline hydrochloride (TC) and the production of hydrogen from water splitting. Experimental results showed that the hydrogen production rate (780.5 μmol g −1 h −1 ) was 2.29 times that of pristine CN, and the TC removal rate (76.3%) of 1.8LDH/CN was 3.71 times that of CN. According to the detailed study of the structural, optical, and photoelectrochemical properties, a type II charge transfer mechanism was proposed to explain the improved photocatalytic performance of LDH/CN.
doi_str_mv 10.1039/D3CE01133J
format Article
fullrecord <record><control><sourceid>crossref</sourceid><recordid>TN_cdi_crossref_primary_10_1039_D3CE01133J</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>10_1039_D3CE01133J</sourcerecordid><originalsourceid>FETCH-LOGICAL-c76J-c39347a2da831e2f788e1267dfa7fcecc564f0ad4c699ff7621366899cae7d323</originalsourceid><addsrcrecordid>eNpNkM1Kw0AUhQdRsFY3PsFdC7HzE2eSpSSttYS66T5M5ycZqZkyM0XyKj6tkQq6ugfu4RzOh9A9wY8Es3JRs2qJCWFsc4FmJOc8KzBjl__0NbqJ8R1jkhOCZ-hr61Yma-r1ossqYLCFHPZukGGE3iQTfEzhpNIpmAifLvVA6wWtQfnBuu4UZHJ-AOsD9K7rDyMYa51yZkhw7H3ySiZ5GJNToE0XpD77vQU5JLd3fvrESWvoRx18ZwY4Bq-nwsl2i66sPERz93vnaLda7qp11ry9vFbPTaYE32SKlSwXkmpZMGKoFUVhCOVCWymsMko98dxiqXPFy9JawSlhnBdlqaQRmlE2Rw_nWDWNjcHY9hjcxwSgJbj9gdr-QWXfkQRsNA</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>NiFe-LDH/g-C 3 N 4 binary heterostructures with 2D/2D configuration for highly efficient photocatalytic degradation of antibiotics and hydrogen production</title><source>Royal Society Of Chemistry Journals 2008-</source><source>Alma/SFX Local Collection</source><creator>Jia, Yujie ; Jiang, Shuhan ; Ou, Qianchen ; Liu, Yanan ; Zhang, Jian ; Zhou, Yangjie ; Lian, Yuan ; Wang, Hongmei</creator><creatorcontrib>Jia, Yujie ; Jiang, Shuhan ; Ou, Qianchen ; Liu, Yanan ; Zhang, Jian ; Zhou, Yangjie ; Lian, Yuan ; Wang, Hongmei</creatorcontrib><description>NiFe-LDH/g-C 3 N 4 (LDH/CN) heterostructures with different amounts of NiFe-LDH (LDH) were prepared by a hydrothermal method and characterized using different experimental techniques. Their photocatalytic properties were investigated using the degradation of tetracycline hydrochloride (TC) and the production of hydrogen from water splitting. Experimental results showed that the hydrogen production rate (780.5 μmol g −1 h −1 ) was 2.29 times that of pristine CN, and the TC removal rate (76.3%) of 1.8LDH/CN was 3.71 times that of CN. According to the detailed study of the structural, optical, and photoelectrochemical properties, a type II charge transfer mechanism was proposed to explain the improved photocatalytic performance of LDH/CN.</description><identifier>ISSN: 1466-8033</identifier><identifier>EISSN: 1466-8033</identifier><identifier>DOI: 10.1039/D3CE01133J</identifier><language>eng</language><ispartof>CrystEngComm, 2024-01, Vol.26 (4), p.532-542</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c76J-c39347a2da831e2f788e1267dfa7fcecc564f0ad4c699ff7621366899cae7d323</citedby><cites>FETCH-LOGICAL-c76J-c39347a2da831e2f788e1267dfa7fcecc564f0ad4c699ff7621366899cae7d323</cites><orcidid>0000-0002-9881-9553 ; 0000-0003-0792-1681</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Jia, Yujie</creatorcontrib><creatorcontrib>Jiang, Shuhan</creatorcontrib><creatorcontrib>Ou, Qianchen</creatorcontrib><creatorcontrib>Liu, Yanan</creatorcontrib><creatorcontrib>Zhang, Jian</creatorcontrib><creatorcontrib>Zhou, Yangjie</creatorcontrib><creatorcontrib>Lian, Yuan</creatorcontrib><creatorcontrib>Wang, Hongmei</creatorcontrib><title>NiFe-LDH/g-C 3 N 4 binary heterostructures with 2D/2D configuration for highly efficient photocatalytic degradation of antibiotics and hydrogen production</title><title>CrystEngComm</title><description>NiFe-LDH/g-C 3 N 4 (LDH/CN) heterostructures with different amounts of NiFe-LDH (LDH) were prepared by a hydrothermal method and characterized using different experimental techniques. Their photocatalytic properties were investigated using the degradation of tetracycline hydrochloride (TC) and the production of hydrogen from water splitting. Experimental results showed that the hydrogen production rate (780.5 μmol g −1 h −1 ) was 2.29 times that of pristine CN, and the TC removal rate (76.3%) of 1.8LDH/CN was 3.71 times that of CN. According to the detailed study of the structural, optical, and photoelectrochemical properties, a type II charge transfer mechanism was proposed to explain the improved photocatalytic performance of LDH/CN.</description><issn>1466-8033</issn><issn>1466-8033</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNpNkM1Kw0AUhQdRsFY3PsFdC7HzE2eSpSSttYS66T5M5ycZqZkyM0XyKj6tkQq6ugfu4RzOh9A9wY8Es3JRs2qJCWFsc4FmJOc8KzBjl__0NbqJ8R1jkhOCZ-hr61Yma-r1ossqYLCFHPZukGGE3iQTfEzhpNIpmAifLvVA6wWtQfnBuu4UZHJ-AOsD9K7rDyMYa51yZkhw7H3ySiZ5GJNToE0XpD77vQU5JLd3fvrESWvoRx18ZwY4Bq-nwsl2i66sPERz93vnaLda7qp11ry9vFbPTaYE32SKlSwXkmpZMGKoFUVhCOVCWymsMko98dxiqXPFy9JawSlhnBdlqaQRmlE2Rw_nWDWNjcHY9hjcxwSgJbj9gdr-QWXfkQRsNA</recordid><startdate>20240122</startdate><enddate>20240122</enddate><creator>Jia, Yujie</creator><creator>Jiang, Shuhan</creator><creator>Ou, Qianchen</creator><creator>Liu, Yanan</creator><creator>Zhang, Jian</creator><creator>Zhou, Yangjie</creator><creator>Lian, Yuan</creator><creator>Wang, Hongmei</creator><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-9881-9553</orcidid><orcidid>https://orcid.org/0000-0003-0792-1681</orcidid></search><sort><creationdate>20240122</creationdate><title>NiFe-LDH/g-C 3 N 4 binary heterostructures with 2D/2D configuration for highly efficient photocatalytic degradation of antibiotics and hydrogen production</title><author>Jia, Yujie ; Jiang, Shuhan ; Ou, Qianchen ; Liu, Yanan ; Zhang, Jian ; Zhou, Yangjie ; Lian, Yuan ; Wang, Hongmei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c76J-c39347a2da831e2f788e1267dfa7fcecc564f0ad4c699ff7621366899cae7d323</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Jia, Yujie</creatorcontrib><creatorcontrib>Jiang, Shuhan</creatorcontrib><creatorcontrib>Ou, Qianchen</creatorcontrib><creatorcontrib>Liu, Yanan</creatorcontrib><creatorcontrib>Zhang, Jian</creatorcontrib><creatorcontrib>Zhou, Yangjie</creatorcontrib><creatorcontrib>Lian, Yuan</creatorcontrib><creatorcontrib>Wang, Hongmei</creatorcontrib><collection>CrossRef</collection><jtitle>CrystEngComm</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Jia, Yujie</au><au>Jiang, Shuhan</au><au>Ou, Qianchen</au><au>Liu, Yanan</au><au>Zhang, Jian</au><au>Zhou, Yangjie</au><au>Lian, Yuan</au><au>Wang, Hongmei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>NiFe-LDH/g-C 3 N 4 binary heterostructures with 2D/2D configuration for highly efficient photocatalytic degradation of antibiotics and hydrogen production</atitle><jtitle>CrystEngComm</jtitle><date>2024-01-22</date><risdate>2024</risdate><volume>26</volume><issue>4</issue><spage>532</spage><epage>542</epage><pages>532-542</pages><issn>1466-8033</issn><eissn>1466-8033</eissn><abstract>NiFe-LDH/g-C 3 N 4 (LDH/CN) heterostructures with different amounts of NiFe-LDH (LDH) were prepared by a hydrothermal method and characterized using different experimental techniques. Their photocatalytic properties were investigated using the degradation of tetracycline hydrochloride (TC) and the production of hydrogen from water splitting. Experimental results showed that the hydrogen production rate (780.5 μmol g −1 h −1 ) was 2.29 times that of pristine CN, and the TC removal rate (76.3%) of 1.8LDH/CN was 3.71 times that of CN. According to the detailed study of the structural, optical, and photoelectrochemical properties, a type II charge transfer mechanism was proposed to explain the improved photocatalytic performance of LDH/CN.</abstract><doi>10.1039/D3CE01133J</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0002-9881-9553</orcidid><orcidid>https://orcid.org/0000-0003-0792-1681</orcidid></addata></record>
fulltext fulltext
identifier ISSN: 1466-8033
ispartof CrystEngComm, 2024-01, Vol.26 (4), p.532-542
issn 1466-8033
1466-8033
language eng
recordid cdi_crossref_primary_10_1039_D3CE01133J
source Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection
title NiFe-LDH/g-C 3 N 4 binary heterostructures with 2D/2D configuration for highly efficient photocatalytic degradation of antibiotics and hydrogen production
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-02T01%3A26%3A21IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-crossref&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=NiFe-LDH/g-C%203%20N%204%20binary%20heterostructures%20with%202D/2D%20configuration%20for%20highly%20efficient%20photocatalytic%20degradation%20of%20antibiotics%20and%20hydrogen%20production&rft.jtitle=CrystEngComm&rft.au=Jia,%20Yujie&rft.date=2024-01-22&rft.volume=26&rft.issue=4&rft.spage=532&rft.epage=542&rft.pages=532-542&rft.issn=1466-8033&rft.eissn=1466-8033&rft_id=info:doi/10.1039/D3CE01133J&rft_dat=%3Ccrossref%3E10_1039_D3CE01133J%3C/crossref%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true