Photo-induced mode change for CO 2 capture/release on spiropyran in a polar-gradient environment
Photo-induced mode change of CO capture/release was achieved by a rationally designed system composed of spiropyran introduced into a polar-gradient field in the interlayer of montmorillonite. DFT calculations and CO adsorption tests demonstrated that spiropyran can interact with CO through not only...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2023-04, Vol.59 (29), p.4304-4307 |
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| container_title | Chemical communications (Cambridge, England) |
| container_volume | 59 |
| creator | Tashiro, Keigo Otori, Masaki Satokawa, Shigeo |
| description | Photo-induced mode change of CO
capture/release was achieved by a rationally designed system composed of spiropyran introduced into a polar-gradient field in the interlayer of montmorillonite. DFT calculations and CO
adsorption tests demonstrated that spiropyran can interact with CO
through not only weak physical interaction such as Coulombic or van der Waals interactions but also electronic interaction, while photo-isomerized merocyanine was in the CO
release mode. Photo-induced CO
concentration systems highly contribute to the realization of carbon neutrality, hence, this study could be a breakthrough for the world's environmental issues. |
| doi_str_mv | 10.1039/d3cc00628j |
| format | Article |
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capture/release was achieved by a rationally designed system composed of spiropyran introduced into a polar-gradient field in the interlayer of montmorillonite. DFT calculations and CO
adsorption tests demonstrated that spiropyran can interact with CO
through not only weak physical interaction such as Coulombic or van der Waals interactions but also electronic interaction, while photo-isomerized merocyanine was in the CO
release mode. Photo-induced CO
concentration systems highly contribute to the realization of carbon neutrality, hence, this study could be a breakthrough for the world's environmental issues.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d3cc00628j</identifier><identifier>PMID: 36976545</identifier><language>eng</language><publisher>England</publisher><ispartof>Chemical communications (Cambridge, England), 2023-04, Vol.59 (29), p.4304-4307</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c995-96042eb2f6f71b484e9ff06bb8fd3131a4c7b7603e7bb8fff16307fa87bb7a203</citedby><cites>FETCH-LOGICAL-c995-96042eb2f6f71b484e9ff06bb8fd3131a4c7b7603e7bb8fff16307fa87bb7a203</cites><orcidid>0000-0002-3380-166X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27903,27904</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36976545$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Tashiro, Keigo</creatorcontrib><creatorcontrib>Otori, Masaki</creatorcontrib><creatorcontrib>Satokawa, Shigeo</creatorcontrib><title>Photo-induced mode change for CO 2 capture/release on spiropyran in a polar-gradient environment</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>Photo-induced mode change of CO
capture/release was achieved by a rationally designed system composed of spiropyran introduced into a polar-gradient field in the interlayer of montmorillonite. DFT calculations and CO
adsorption tests demonstrated that spiropyran can interact with CO
through not only weak physical interaction such as Coulombic or van der Waals interactions but also electronic interaction, while photo-isomerized merocyanine was in the CO
release mode. Photo-induced CO
concentration systems highly contribute to the realization of carbon neutrality, hence, this study could be a breakthrough for the world's environmental issues.</description><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNo9kD1PwzAQhi0EoqWw8AOQZ6RQO_6KRxS-VakMHdiCY5_bVI0dOS1S_z0pBW659-4e3fAgdE3JHSVMTx2zlhCZF-sTNKZM8kzw4uP0kIXOFONihC76fk2GoqI4RyMmtZKCizH6fF_Fbcya4HYWHG6jA2xXJiwB-5hwOcc5tqbb7hJME2zA9IBjwH3XpNjtkwm4CdjgLm5MypbJuAbCFkP4Gu6hHfIlOvNm08PVb5-gxdPjonzJZvPn1_J-llmtRaYl4TnUuZde0ZoXHLT3RNZ14R2jjBpuVa0kYaAOO--pZER5UwyjMjlhE3R7fGtT7PsEvupS05q0ryipDpaqB1aWP5beBvjmCHe7ugX3j_5pYd84ZmNy</recordid><startdate>20230406</startdate><enddate>20230406</enddate><creator>Tashiro, Keigo</creator><creator>Otori, Masaki</creator><creator>Satokawa, Shigeo</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-3380-166X</orcidid></search><sort><creationdate>20230406</creationdate><title>Photo-induced mode change for CO 2 capture/release on spiropyran in a polar-gradient environment</title><author>Tashiro, Keigo ; Otori, Masaki ; Satokawa, Shigeo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c995-96042eb2f6f71b484e9ff06bb8fd3131a4c7b7603e7bb8fff16307fa87bb7a203</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Tashiro, Keigo</creatorcontrib><creatorcontrib>Otori, Masaki</creatorcontrib><creatorcontrib>Satokawa, Shigeo</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tashiro, Keigo</au><au>Otori, Masaki</au><au>Satokawa, Shigeo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Photo-induced mode change for CO 2 capture/release on spiropyran in a polar-gradient environment</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2023-04-06</date><risdate>2023</risdate><volume>59</volume><issue>29</issue><spage>4304</spage><epage>4307</epage><pages>4304-4307</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>Photo-induced mode change of CO
capture/release was achieved by a rationally designed system composed of spiropyran introduced into a polar-gradient field in the interlayer of montmorillonite. DFT calculations and CO
adsorption tests demonstrated that spiropyran can interact with CO
through not only weak physical interaction such as Coulombic or van der Waals interactions but also electronic interaction, while photo-isomerized merocyanine was in the CO
release mode. Photo-induced CO
concentration systems highly contribute to the realization of carbon neutrality, hence, this study could be a breakthrough for the world's environmental issues.</abstract><cop>England</cop><pmid>36976545</pmid><doi>10.1039/d3cc00628j</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0002-3380-166X</orcidid></addata></record> |
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| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2023-04, Vol.59 (29), p.4304-4307 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_crossref_primary_10_1039_D3CC00628J |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | Photo-induced mode change for CO 2 capture/release on spiropyran in a polar-gradient environment |
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