Controlled electropositive catalytic sites on zeolites for achieving high CH 3 Cl selectivity via electrophilic CH 4 chlorination using Cl 2

The spontaneous homolytic Cl 2 cleavage to two reactive chlorine radicals is useful for activating the C–H bond in CH 4 to produce various chlorinated products (CH 3 Cl, CH 2 Cl 2 , CHCl 3 , and CCl 4 ), but it is noncatalytic and uncontrollable. Herein, zeolites with controlled electropositive Lewi...

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Veröffentlicht in:Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2022-11, Vol.10 (46), p.24475-24486
Hauptverfasser: Choi, Yuyeol, Park, Sunghyun, Kwon, Seungdon, Ko, Kyoung Chul
Format: Artikel
Sprache:eng
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