Collaborative hydrothermal and calcination fabrication of ZnOS heterostructures for visible-light-driven H 2 production
Photocatalytic water splitting is forecasted as a promising strategy for H production. In this work, novel zinc oxide/zinc sulfide (ZnOS- ) ( = 1, 2, 3 and 4) heterostructures were fabricated by a collaborative hydrothermal and calcination method with different amounts of trithiocyanuric acid. The f...
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| Veröffentlicht in: | Physical chemistry chemical physics : PCCP 2023-02, Vol.25 (5), p.3617-3621 |
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| container_title | Physical chemistry chemical physics : PCCP |
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| creator | Chen, XueLi Lin, ChenXiang Lai, LanHai Liu, MingRui Zheng, Kai Li, SongTao Li, HaiTao |
| description | Photocatalytic water splitting is forecasted as a promising strategy for H
production. In this work, novel zinc oxide/zinc sulfide (ZnOS-
) (
= 1, 2, 3 and 4) heterostructures were fabricated by a collaborative hydrothermal and calcination method with different amounts of trithiocyanuric acid. The formation of ZnOS-
heterostructures was confirmed by PXRD, XPS, and HRTEM. Moreover, ZnOS-3 nanoparticles exhibited homogeneous and smooth surface morphology structure. ZnOS-3 displayed efficient charge separation and transfer efficiency upon photoinduction. ZnOS-3 showed the highest average H
evolution reaction rate (78.87 μmol h
) under visible-light irradiation, which increased with increase in the ratio of trithiocyanuric acid in the ZnOS-
series. This work provides a new insight to prepare uniformly integrated heterostructures of metal oxides/sulfides for visible-light-driven H
generation. |
| doi_str_mv | 10.1039/d2cp05351a |
| format | Article |
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production. In this work, novel zinc oxide/zinc sulfide (ZnOS-
) (
= 1, 2, 3 and 4) heterostructures were fabricated by a collaborative hydrothermal and calcination method with different amounts of trithiocyanuric acid. The formation of ZnOS-
heterostructures was confirmed by PXRD, XPS, and HRTEM. Moreover, ZnOS-3 nanoparticles exhibited homogeneous and smooth surface morphology structure. ZnOS-3 displayed efficient charge separation and transfer efficiency upon photoinduction. ZnOS-3 showed the highest average H
evolution reaction rate (78.87 μmol h
) under visible-light irradiation, which increased with increase in the ratio of trithiocyanuric acid in the ZnOS-
series. This work provides a new insight to prepare uniformly integrated heterostructures of metal oxides/sulfides for visible-light-driven H
generation.</description><identifier>ISSN: 1463-9076</identifier><identifier>EISSN: 1463-9084</identifier><identifier>DOI: 10.1039/d2cp05351a</identifier><identifier>PMID: 36649128</identifier><language>eng</language><publisher>England</publisher><ispartof>Physical chemistry chemical physics : PCCP, 2023-02, Vol.25 (5), p.3617-3621</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c998-fb2d387ecbe70e50df27f8760e3d76e4cfed5dd95b192f8312189afec83f49533</citedby><cites>FETCH-LOGICAL-c998-fb2d387ecbe70e50df27f8760e3d76e4cfed5dd95b192f8312189afec83f49533</cites><orcidid>0000-0003-4246-5183</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27903,27904</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36649128$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Chen, XueLi</creatorcontrib><creatorcontrib>Lin, ChenXiang</creatorcontrib><creatorcontrib>Lai, LanHai</creatorcontrib><creatorcontrib>Liu, MingRui</creatorcontrib><creatorcontrib>Zheng, Kai</creatorcontrib><creatorcontrib>Li, SongTao</creatorcontrib><creatorcontrib>Li, HaiTao</creatorcontrib><title>Collaborative hydrothermal and calcination fabrication of ZnOS heterostructures for visible-light-driven H 2 production</title><title>Physical chemistry chemical physics : PCCP</title><addtitle>Phys Chem Chem Phys</addtitle><description>Photocatalytic water splitting is forecasted as a promising strategy for H
production. In this work, novel zinc oxide/zinc sulfide (ZnOS-
) (
= 1, 2, 3 and 4) heterostructures were fabricated by a collaborative hydrothermal and calcination method with different amounts of trithiocyanuric acid. The formation of ZnOS-
heterostructures was confirmed by PXRD, XPS, and HRTEM. Moreover, ZnOS-3 nanoparticles exhibited homogeneous and smooth surface morphology structure. ZnOS-3 displayed efficient charge separation and transfer efficiency upon photoinduction. ZnOS-3 showed the highest average H
evolution reaction rate (78.87 μmol h
) under visible-light irradiation, which increased with increase in the ratio of trithiocyanuric acid in the ZnOS-
series. This work provides a new insight to prepare uniformly integrated heterostructures of metal oxides/sulfides for visible-light-driven H
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production. In this work, novel zinc oxide/zinc sulfide (ZnOS-
) (
= 1, 2, 3 and 4) heterostructures were fabricated by a collaborative hydrothermal and calcination method with different amounts of trithiocyanuric acid. The formation of ZnOS-
heterostructures was confirmed by PXRD, XPS, and HRTEM. Moreover, ZnOS-3 nanoparticles exhibited homogeneous and smooth surface morphology structure. ZnOS-3 displayed efficient charge separation and transfer efficiency upon photoinduction. ZnOS-3 showed the highest average H
evolution reaction rate (78.87 μmol h
) under visible-light irradiation, which increased with increase in the ratio of trithiocyanuric acid in the ZnOS-
series. This work provides a new insight to prepare uniformly integrated heterostructures of metal oxides/sulfides for visible-light-driven H
generation.</abstract><cop>England</cop><pmid>36649128</pmid><doi>10.1039/d2cp05351a</doi><tpages>5</tpages><orcidid>https://orcid.org/0000-0003-4246-5183</orcidid></addata></record> |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | Collaborative hydrothermal and calcination fabrication of ZnOS heterostructures for visible-light-driven H 2 production |
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