Enhanced chirality in a dielectric metasurface without breaking symmetry
We propose a dielectric metasurface constructed by quadrumer silicon nano-disks with crossed slots in the middle. This metasurface can support the excitation of bound states in the continuum which are closely related to the toroidal dipole resonance. After introducing chiral enantiomers with weak ch...
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Veröffentlicht in: | Physical chemistry chemical physics : PCCP 2023-01, Vol.25 (3), p.25-255 |
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creator | Liu, Xingguang Li, Junqing Zhao, Rui Zhang, Yingjie Dong, Yongkang |
description | We propose a dielectric metasurface constructed by quadrumer silicon nano-disks with crossed slots in the middle. This metasurface can support the excitation of bound states in the continuum which are closely related to the toroidal dipole resonance. After introducing chiral enantiomers with weak chirality into the surrounding medium, due to the bound states in the continuum, the chiroptical effect of the metasurface can be greatly enhanced. In particular, this metasurface breaks neither the in-plane nor out-plane symmetry, which has lower requirements of spatial processing capabilities. The proposed metasurface can be used in the trace analysis of chiral enantiomers and may lead to potential applications for tailored phase control and ultra-integrated molar chiral sensing metadevices.
The proposed dielectric metasurface supports the excitation of bound states in the continuum. After introducing chiral enantiomers with weak chirality into the surrounding medium, the chiroptical effect of the metasurface can be greatly enhanced. |
doi_str_mv | 10.1039/d2cp04833g |
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The proposed dielectric metasurface supports the excitation of bound states in the continuum. After introducing chiral enantiomers with weak chirality into the surrounding medium, the chiroptical effect of the metasurface can be greatly enhanced.</description><identifier>ISSN: 1463-9076</identifier><identifier>EISSN: 1463-9084</identifier><identifier>DOI: 10.1039/d2cp04833g</identifier><identifier>PMID: 36546559</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Broken symmetry ; Chirality ; Dipoles ; Disks ; Enantiomers ; Metasurfaces ; Phase control</subject><ispartof>Physical chemistry chemical physics : PCCP, 2023-01, Vol.25 (3), p.25-255</ispartof><rights>Copyright Royal Society of Chemistry 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c337t-e0149636f87077b76dbd4940f68787b57776bbd79d4cceec4660b9937f8673963</citedby><cites>FETCH-LOGICAL-c337t-e0149636f87077b76dbd4940f68787b57776bbd79d4cceec4660b9937f8673963</cites><orcidid>0000-0001-8659-3983 ; 0000-0001-6288-5762</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27923,27924</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36546559$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liu, Xingguang</creatorcontrib><creatorcontrib>Li, Junqing</creatorcontrib><creatorcontrib>Zhao, Rui</creatorcontrib><creatorcontrib>Zhang, Yingjie</creatorcontrib><creatorcontrib>Dong, Yongkang</creatorcontrib><title>Enhanced chirality in a dielectric metasurface without breaking symmetry</title><title>Physical chemistry chemical physics : PCCP</title><addtitle>Phys Chem Chem Phys</addtitle><description>We propose a dielectric metasurface constructed by quadrumer silicon nano-disks with crossed slots in the middle. This metasurface can support the excitation of bound states in the continuum which are closely related to the toroidal dipole resonance. After introducing chiral enantiomers with weak chirality into the surrounding medium, due to the bound states in the continuum, the chiroptical effect of the metasurface can be greatly enhanced. In particular, this metasurface breaks neither the in-plane nor out-plane symmetry, which has lower requirements of spatial processing capabilities. The proposed metasurface can be used in the trace analysis of chiral enantiomers and may lead to potential applications for tailored phase control and ultra-integrated molar chiral sensing metadevices.
The proposed dielectric metasurface supports the excitation of bound states in the continuum. After introducing chiral enantiomers with weak chirality into the surrounding medium, the chiroptical effect of the metasurface can be greatly enhanced.</description><subject>Broken symmetry</subject><subject>Chirality</subject><subject>Dipoles</subject><subject>Disks</subject><subject>Enantiomers</subject><subject>Metasurfaces</subject><subject>Phase control</subject><issn>1463-9076</issn><issn>1463-9084</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpdkctLAzEQxoMotlYv3pWAFxFWs81rc5RaW6GgBz0veW2buo-a7CL73xttreBpBr7ffMx8A8B5im5ThMWdGesNIhnGywMwTAnDiUAZOdz3nA3ASQhrhFBKU3wMBphRwigVQzCf1itZa2ugXjkvS9f20NVQQuNsaXXrnYaVbWXofCG1hZ-uXTVdC5W38t3VSxj6Kuq-PwVHhSyDPdvVEXh7nL5O5sniefY0uV8kGmPeJhalRDDMiowjzhVnRhkiCCpYxjOuKOecKWW4MERrazVhDCkhMC8yxnGcHIHrre_GNx-dDW1euaBtWcraNl3Ix5xyRGm8NKJX_9B10_k6bhcpxggiKIY2AjdbSvsmBG-LfONdJX2fpyj_zjd_GE9efvKdRfhyZ9mpypo9-htoBC62gA96r_49CH8B7Hl-DA</recordid><startdate>20230118</startdate><enddate>20230118</enddate><creator>Liu, Xingguang</creator><creator>Li, Junqing</creator><creator>Zhao, Rui</creator><creator>Zhang, Yingjie</creator><creator>Dong, Yongkang</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0001-8659-3983</orcidid><orcidid>https://orcid.org/0000-0001-6288-5762</orcidid></search><sort><creationdate>20230118</creationdate><title>Enhanced chirality in a dielectric metasurface without breaking symmetry</title><author>Liu, Xingguang ; Li, Junqing ; Zhao, Rui ; Zhang, Yingjie ; Dong, Yongkang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-e0149636f87077b76dbd4940f68787b57776bbd79d4cceec4660b9937f8673963</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Broken symmetry</topic><topic>Chirality</topic><topic>Dipoles</topic><topic>Disks</topic><topic>Enantiomers</topic><topic>Metasurfaces</topic><topic>Phase control</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Liu, Xingguang</creatorcontrib><creatorcontrib>Li, Junqing</creatorcontrib><creatorcontrib>Zhao, Rui</creatorcontrib><creatorcontrib>Zhang, Yingjie</creatorcontrib><creatorcontrib>Dong, Yongkang</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Physical chemistry chemical physics : PCCP</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, Xingguang</au><au>Li, Junqing</au><au>Zhao, Rui</au><au>Zhang, Yingjie</au><au>Dong, Yongkang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced chirality in a dielectric metasurface without breaking symmetry</atitle><jtitle>Physical chemistry chemical physics : PCCP</jtitle><addtitle>Phys Chem Chem Phys</addtitle><date>2023-01-18</date><risdate>2023</risdate><volume>25</volume><issue>3</issue><spage>25</spage><epage>255</epage><pages>25-255</pages><issn>1463-9076</issn><eissn>1463-9084</eissn><abstract>We propose a dielectric metasurface constructed by quadrumer silicon nano-disks with crossed slots in the middle. This metasurface can support the excitation of bound states in the continuum which are closely related to the toroidal dipole resonance. After introducing chiral enantiomers with weak chirality into the surrounding medium, due to the bound states in the continuum, the chiroptical effect of the metasurface can be greatly enhanced. In particular, this metasurface breaks neither the in-plane nor out-plane symmetry, which has lower requirements of spatial processing capabilities. The proposed metasurface can be used in the trace analysis of chiral enantiomers and may lead to potential applications for tailored phase control and ultra-integrated molar chiral sensing metadevices.
The proposed dielectric metasurface supports the excitation of bound states in the continuum. After introducing chiral enantiomers with weak chirality into the surrounding medium, the chiroptical effect of the metasurface can be greatly enhanced.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>36546559</pmid><doi>10.1039/d2cp04833g</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0001-8659-3983</orcidid><orcidid>https://orcid.org/0000-0001-6288-5762</orcidid></addata></record> |
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source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
subjects | Broken symmetry Chirality Dipoles Disks Enantiomers Metasurfaces Phase control |
title | Enhanced chirality in a dielectric metasurface without breaking symmetry |
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