Understanding the structure and dynamics of hydrogenases by ultrafast and two-dimensional infrared spectroscopy

Hydrogenases are valuable model enzymes for sustainable energy conversion approaches using H 2 , but rational utilization of these base-metal biocatalysts requires a detailed understanding of the structure and dynamics of their complex active sites. The intrinsic CO and CN − ligands of these metallo...

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Veröffentlicht in:	Chemical science (Cambridge) 2019-10, Vol.1 (39), p.8981-8989
Hauptverfasser:	Horch, Marius, Schoknecht, Janna, Wrathall, Solomon L. D, Greetham, Gregory M, Lenz, Oliver, Hunt, Neil T
Format:	Artikel
Sprache:	eng
Schlagworte:	Chemistry Chromophores Energy conversion Energy dissipation Enzymes Hydrogenase Infrared spectroscopy Intermetallic compounds Iron compounds Ligands Nickel compounds Spectrum analysis Vibrational states
Online-Zugang:	Volltext
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