Ultrathin MXene/aramid nanofiber composite paper with excellent mechanical properties for efficient electromagnetic interference shielding
MXenes, new two-dimensional compounds with hydrophilic surfaces and high metallic conductivity, have attracted significant interest in the electromagnetic interference shielding field in recent years. Nevertheless, poor mechanical properties and brittle nature are bottlenecks for their commercial ap...
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| Veröffentlicht in: | Nanoscale 2019-12, Vol.11 (48), p.23382-23391 |
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| creator | Xie, Fan Jia, Fengfeng Zhuo, Longhai Lu, Zhaoqing Si, Lianmeng Huang, Jizhen Zhang, Meiyun Ma, Qin |
| description | MXenes, new two-dimensional compounds with hydrophilic surfaces and high metallic conductivity, have attracted significant interest in the electromagnetic interference shielding field in recent years. Nevertheless, poor mechanical properties and brittle nature are bottlenecks for their commercial application. Herein, one-dimensional ANFs were designed as the intermolecular cross-linker between d-Ti
3
C
2
T
x
flakes and MXene (d-Ti
3
C
2
T
x
)/aramid nanofiber (ANF) composite paper with a multi-layered structure was fabricated
via
the vacuum-assisted filtration approach. Further investigation revealed that the ANFs and MXene displayed good combination by hydrogen bonding, and MXene/ANF composite papers exhibited excellent mechanical properties and superior electrical conductivity. The MXene/ANF composite paper possessed a favorable shielding effectiveness (SE) which reached ∼28 dB in 8.2-12.4 GHz (X band) with an ultra-thin thickness ∼17 μm and showed potential application prospects as an advanced composite in sensitive electronic products.
ANFs were designed as an intermolecular cross-linker to reinforce MXene and the composite paper exhibited excellent EMI shielding performance with a multi-layered structure. |
| doi_str_mv | 10.1039/c9nr07331k |
| format | Article |
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3
C
2
T
x
flakes and MXene (d-Ti
3
C
2
T
x
)/aramid nanofiber (ANF) composite paper with a multi-layered structure was fabricated
via
the vacuum-assisted filtration approach. Further investigation revealed that the ANFs and MXene displayed good combination by hydrogen bonding, and MXene/ANF composite papers exhibited excellent mechanical properties and superior electrical conductivity. The MXene/ANF composite paper possessed a favorable shielding effectiveness (SE) which reached ∼28 dB in 8.2-12.4 GHz (X band) with an ultra-thin thickness ∼17 μm and showed potential application prospects as an advanced composite in sensitive electronic products.
ANFs were designed as an intermolecular cross-linker to reinforce MXene and the composite paper exhibited excellent EMI shielding performance with a multi-layered structure.</description><identifier>ISSN: 2040-3364</identifier><identifier>EISSN: 2040-3372</identifier><identifier>DOI: 10.1039/c9nr07331k</identifier><identifier>PMID: 31793611</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Crosslinking ; Electrical resistivity ; Electromagnetic shielding ; Hydrogen bonding ; Hydrogen embrittlement ; Mechanical properties ; Multilayers ; MXenes ; Nanofibers ; Superhigh frequencies</subject><ispartof>Nanoscale, 2019-12, Vol.11 (48), p.23382-23391</ispartof><rights>Copyright Royal Society of Chemistry 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c337t-edeb3db56ad804310f742b4cfbf5b688705966f62c9b28772df5d367682a1ce3</citedby><cites>FETCH-LOGICAL-c337t-edeb3db56ad804310f742b4cfbf5b688705966f62c9b28772df5d367682a1ce3</cites><orcidid>0000-0002-2095-4405 ; 0000-0001-5721-3048</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31793611$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Xie, Fan</creatorcontrib><creatorcontrib>Jia, Fengfeng</creatorcontrib><creatorcontrib>Zhuo, Longhai</creatorcontrib><creatorcontrib>Lu, Zhaoqing</creatorcontrib><creatorcontrib>Si, Lianmeng</creatorcontrib><creatorcontrib>Huang, Jizhen</creatorcontrib><creatorcontrib>Zhang, Meiyun</creatorcontrib><creatorcontrib>Ma, Qin</creatorcontrib><title>Ultrathin MXene/aramid nanofiber composite paper with excellent mechanical properties for efficient electromagnetic interference shielding</title><title>Nanoscale</title><addtitle>Nanoscale</addtitle><description>MXenes, new two-dimensional compounds with hydrophilic surfaces and high metallic conductivity, have attracted significant interest in the electromagnetic interference shielding field in recent years. Nevertheless, poor mechanical properties and brittle nature are bottlenecks for their commercial application. Herein, one-dimensional ANFs were designed as the intermolecular cross-linker between d-Ti
3
C
2
T
x
flakes and MXene (d-Ti
3
C
2
T
x
)/aramid nanofiber (ANF) composite paper with a multi-layered structure was fabricated
via
the vacuum-assisted filtration approach. Further investigation revealed that the ANFs and MXene displayed good combination by hydrogen bonding, and MXene/ANF composite papers exhibited excellent mechanical properties and superior electrical conductivity. The MXene/ANF composite paper possessed a favorable shielding effectiveness (SE) which reached ∼28 dB in 8.2-12.4 GHz (X band) with an ultra-thin thickness ∼17 μm and showed potential application prospects as an advanced composite in sensitive electronic products.
ANFs were designed as an intermolecular cross-linker to reinforce MXene and the composite paper exhibited excellent EMI shielding performance with a multi-layered structure.</description><subject>Crosslinking</subject><subject>Electrical resistivity</subject><subject>Electromagnetic shielding</subject><subject>Hydrogen bonding</subject><subject>Hydrogen embrittlement</subject><subject>Mechanical properties</subject><subject>Multilayers</subject><subject>MXenes</subject><subject>Nanofibers</subject><subject>Superhigh frequencies</subject><issn>2040-3364</issn><issn>2040-3372</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNpd0VtLHDEUB_BQKt7qS98rgb6IsJrLTDLzKEu9oLZQLPRtyGRO3NiZZEyyVL-Cn9pMd12hTzkhPw7n5I_QZ0pOKOH1qa5dIJJz-ucD2mWkIDPOJfu4qUWxg_ZifCBE1FzwbbTDqcwVpbvo5VefgkoL6_Dtb3BwqoIabIedct7YFgLWfhh9tAnwqMZ8_2vTAsOThr4Hl_AAeqGc1arHY_AZJAsRGx8wGGO1nQz0oFPwg7p3kKzG1iUIBgI4DTguLPSddfef0JZRfYSD9bmP7s6_3c0vZzc_Lq7mZzcznddKM-ig5V1bCtVVpOCUGFmwttCmNWUrqkqSshbCCKbrllVSss6UHRdSVExRDXwfHa3a5nEflxBTM9g4baMc-GVsGGekkiVhJNOv_9EHvwwuDzepop6-cVLHK6WDjzGAacZgBxWeG0qaKaBmXn__-S-g64wP1y2X7QDdhr4lksGXFQhRb17fE-avusmYZw</recordid><startdate>20191228</startdate><enddate>20191228</enddate><creator>Xie, Fan</creator><creator>Jia, Fengfeng</creator><creator>Zhuo, Longhai</creator><creator>Lu, Zhaoqing</creator><creator>Si, Lianmeng</creator><creator>Huang, Jizhen</creator><creator>Zhang, Meiyun</creator><creator>Ma, Qin</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>F28</scope><scope>FR3</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-2095-4405</orcidid><orcidid>https://orcid.org/0000-0001-5721-3048</orcidid></search><sort><creationdate>20191228</creationdate><title>Ultrathin MXene/aramid nanofiber composite paper with excellent mechanical properties for efficient electromagnetic interference shielding</title><author>Xie, Fan ; Jia, Fengfeng ; Zhuo, Longhai ; Lu, Zhaoqing ; Si, Lianmeng ; Huang, Jizhen ; Zhang, Meiyun ; Ma, Qin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-edeb3db56ad804310f742b4cfbf5b688705966f62c9b28772df5d367682a1ce3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Crosslinking</topic><topic>Electrical resistivity</topic><topic>Electromagnetic shielding</topic><topic>Hydrogen bonding</topic><topic>Hydrogen embrittlement</topic><topic>Mechanical properties</topic><topic>Multilayers</topic><topic>MXenes</topic><topic>Nanofibers</topic><topic>Superhigh frequencies</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Xie, Fan</creatorcontrib><creatorcontrib>Jia, Fengfeng</creatorcontrib><creatorcontrib>Zhuo, Longhai</creatorcontrib><creatorcontrib>Lu, Zhaoqing</creatorcontrib><creatorcontrib>Si, Lianmeng</creatorcontrib><creatorcontrib>Huang, Jizhen</creatorcontrib><creatorcontrib>Zhang, Meiyun</creatorcontrib><creatorcontrib>Ma, Qin</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Nanoscale</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Xie, Fan</au><au>Jia, Fengfeng</au><au>Zhuo, Longhai</au><au>Lu, Zhaoqing</au><au>Si, Lianmeng</au><au>Huang, Jizhen</au><au>Zhang, Meiyun</au><au>Ma, Qin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ultrathin MXene/aramid nanofiber composite paper with excellent mechanical properties for efficient electromagnetic interference shielding</atitle><jtitle>Nanoscale</jtitle><addtitle>Nanoscale</addtitle><date>2019-12-28</date><risdate>2019</risdate><volume>11</volume><issue>48</issue><spage>23382</spage><epage>23391</epage><pages>23382-23391</pages><issn>2040-3364</issn><eissn>2040-3372</eissn><abstract>MXenes, new two-dimensional compounds with hydrophilic surfaces and high metallic conductivity, have attracted significant interest in the electromagnetic interference shielding field in recent years. Nevertheless, poor mechanical properties and brittle nature are bottlenecks for their commercial application. Herein, one-dimensional ANFs were designed as the intermolecular cross-linker between d-Ti
3
C
2
T
x
flakes and MXene (d-Ti
3
C
2
T
x
)/aramid nanofiber (ANF) composite paper with a multi-layered structure was fabricated
via
the vacuum-assisted filtration approach. Further investigation revealed that the ANFs and MXene displayed good combination by hydrogen bonding, and MXene/ANF composite papers exhibited excellent mechanical properties and superior electrical conductivity. The MXene/ANF composite paper possessed a favorable shielding effectiveness (SE) which reached ∼28 dB in 8.2-12.4 GHz (X band) with an ultra-thin thickness ∼17 μm and showed potential application prospects as an advanced composite in sensitive electronic products.
ANFs were designed as an intermolecular cross-linker to reinforce MXene and the composite paper exhibited excellent EMI shielding performance with a multi-layered structure.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>31793611</pmid><doi>10.1039/c9nr07331k</doi><tpages>1</tpages><orcidid>https://orcid.org/0000-0002-2095-4405</orcidid><orcidid>https://orcid.org/0000-0001-5721-3048</orcidid></addata></record> |
| fulltext | fulltext |
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| ispartof | Nanoscale, 2019-12, Vol.11 (48), p.23382-23391 |
| issn | 2040-3364 2040-3372 |
| language | eng |
| recordid | cdi_crossref_primary_10_1039_C9NR07331K |
| source | Royal Society Of Chemistry Journals 2008- |
| subjects | Crosslinking Electrical resistivity Electromagnetic shielding Hydrogen bonding Hydrogen embrittlement Mechanical properties Multilayers MXenes Nanofibers Superhigh frequencies |
| title | Ultrathin MXene/aramid nanofiber composite paper with excellent mechanical properties for efficient electromagnetic interference shielding |
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