Temperature-assisted rapid nucleation: a facile method to optimize the film morphology for perovskite solar cells
The nucleation stage has an important influence on the lead halide perovskite film morphology, and therefore the solar cell performance. Here, we introduce a facile temperature-assisted rapid nucleation (TRN) method to improve the film crystallization process and the film morphology. By employing lo...
Gespeichert in:
| Veröffentlicht in: | Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2017, Vol.5 (38), p.20327-20333 |
|---|---|
| Hauptverfasser: | , , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 20333 |
|---|---|
| container_issue | 38 |
| container_start_page | 20327 |
| container_title | Journal of materials chemistry. A, Materials for energy and sustainability |
| container_volume | 5 |
| creator | Ren, Ying-Ke Ding, Xi-Hong Wu, Ya-Han Zhu, Jun Hayat, Tasawar Alsaedi, Ahmed Xu, Ya-Feng Li, Zhao-Qian Yang, Shang-Feng Dai, Song-Yuan |
| description | The nucleation stage has an important influence on the lead halide perovskite film morphology, and therefore the solar cell performance. Here, we introduce a facile temperature-assisted rapid nucleation (TRN) method to improve the film crystallization process and the film morphology. By employing low temperature anti-solvents (diethyl ether, chlorobenzene and toluene), we stimulate homogeneous nuclei growth, resulting in a highly dense perovskite thin layer. The TRN method prepared (FAPbI
3
)
0.85
(MAPbBr
3
)
0.15
devices exhibit a power conversion efficiency up to 19.2% and maintain over 85% of the original efficiency after 40 days of storage at room temperature under a relative humidity of 10–40%. |
| doi_str_mv | 10.1039/C7TA06334B |
| format | Article |
| fullrecord | <record><control><sourceid>crossref</sourceid><recordid>TN_cdi_crossref_primary_10_1039_C7TA06334B</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>10_1039_C7TA06334B</sourcerecordid><originalsourceid>FETCH-LOGICAL-c375t-f188cc2daf16324972e094cf2ed3310ec25878191e613c659c3559c2d21d1603</originalsourceid><addsrcrecordid>eNpFkE1LAzEURYMoWGo3_oK3FkbzMZOZuKtFq1BwM_shJC82mmnGJBXqr7ei6F3ce1dncQi5ZPSaUaFuVm2_pFKI-u6EzDhtaNXWSp7-_a47J4ucX-kxHaVSqRl573GcMOmyT1jpnH0uaCHpyVvY7U1AXXzc3YIGp40PCCOWbbRQIsSp-NF_IpQtgvNhhDGmaRtDfDmAiwmO3PiR33xByDHoBAZDyBfkzOmQcfG7c9I_3Perx2rzvH5aLTeVEW1TKse6zhhutWNS8Fq1HKmqjeNohWAUDW-6tmOKoWTCyEYZ0RyLW84sk1TMydUP1qSYc0I3TMmPOh0GRodvXcO_LvEF1_leZg</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Temperature-assisted rapid nucleation: a facile method to optimize the film morphology for perovskite solar cells</title><source>Royal Society Of Chemistry Journals 2008-</source><creator>Ren, Ying-Ke ; Ding, Xi-Hong ; Wu, Ya-Han ; Zhu, Jun ; Hayat, Tasawar ; Alsaedi, Ahmed ; Xu, Ya-Feng ; Li, Zhao-Qian ; Yang, Shang-Feng ; Dai, Song-Yuan</creator><creatorcontrib>Ren, Ying-Ke ; Ding, Xi-Hong ; Wu, Ya-Han ; Zhu, Jun ; Hayat, Tasawar ; Alsaedi, Ahmed ; Xu, Ya-Feng ; Li, Zhao-Qian ; Yang, Shang-Feng ; Dai, Song-Yuan</creatorcontrib><description>The nucleation stage has an important influence on the lead halide perovskite film morphology, and therefore the solar cell performance. Here, we introduce a facile temperature-assisted rapid nucleation (TRN) method to improve the film crystallization process and the film morphology. By employing low temperature anti-solvents (diethyl ether, chlorobenzene and toluene), we stimulate homogeneous nuclei growth, resulting in a highly dense perovskite thin layer. The TRN method prepared (FAPbI
3
)
0.85
(MAPbBr
3
)
0.15
devices exhibit a power conversion efficiency up to 19.2% and maintain over 85% of the original efficiency after 40 days of storage at room temperature under a relative humidity of 10–40%.</description><identifier>ISSN: 2050-7488</identifier><identifier>EISSN: 2050-7496</identifier><identifier>DOI: 10.1039/C7TA06334B</identifier><language>eng</language><ispartof>Journal of materials chemistry. A, Materials for energy and sustainability, 2017, Vol.5 (38), p.20327-20333</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c375t-f188cc2daf16324972e094cf2ed3310ec25878191e613c659c3559c2d21d1603</citedby><cites>FETCH-LOGICAL-c375t-f188cc2daf16324972e094cf2ed3310ec25878191e613c659c3559c2d21d1603</cites><orcidid>0000-0003-1938-4705 ; 0000-0002-6931-9613 ; 0000-0002-4921-0979</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,4010,27900,27901,27902</link.rule.ids></links><search><creatorcontrib>Ren, Ying-Ke</creatorcontrib><creatorcontrib>Ding, Xi-Hong</creatorcontrib><creatorcontrib>Wu, Ya-Han</creatorcontrib><creatorcontrib>Zhu, Jun</creatorcontrib><creatorcontrib>Hayat, Tasawar</creatorcontrib><creatorcontrib>Alsaedi, Ahmed</creatorcontrib><creatorcontrib>Xu, Ya-Feng</creatorcontrib><creatorcontrib>Li, Zhao-Qian</creatorcontrib><creatorcontrib>Yang, Shang-Feng</creatorcontrib><creatorcontrib>Dai, Song-Yuan</creatorcontrib><title>Temperature-assisted rapid nucleation: a facile method to optimize the film morphology for perovskite solar cells</title><title>Journal of materials chemistry. A, Materials for energy and sustainability</title><description>The nucleation stage has an important influence on the lead halide perovskite film morphology, and therefore the solar cell performance. Here, we introduce a facile temperature-assisted rapid nucleation (TRN) method to improve the film crystallization process and the film morphology. By employing low temperature anti-solvents (diethyl ether, chlorobenzene and toluene), we stimulate homogeneous nuclei growth, resulting in a highly dense perovskite thin layer. The TRN method prepared (FAPbI
3
)
0.85
(MAPbBr
3
)
0.15
devices exhibit a power conversion efficiency up to 19.2% and maintain over 85% of the original efficiency after 40 days of storage at room temperature under a relative humidity of 10–40%.</description><issn>2050-7488</issn><issn>2050-7496</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNpFkE1LAzEURYMoWGo3_oK3FkbzMZOZuKtFq1BwM_shJC82mmnGJBXqr7ei6F3ce1dncQi5ZPSaUaFuVm2_pFKI-u6EzDhtaNXWSp7-_a47J4ucX-kxHaVSqRl573GcMOmyT1jpnH0uaCHpyVvY7U1AXXzc3YIGp40PCCOWbbRQIsSp-NF_IpQtgvNhhDGmaRtDfDmAiwmO3PiR33xByDHoBAZDyBfkzOmQcfG7c9I_3Perx2rzvH5aLTeVEW1TKse6zhhutWNS8Fq1HKmqjeNohWAUDW-6tmOKoWTCyEYZ0RyLW84sk1TMydUP1qSYc0I3TMmPOh0GRodvXcO_LvEF1_leZg</recordid><startdate>2017</startdate><enddate>2017</enddate><creator>Ren, Ying-Ke</creator><creator>Ding, Xi-Hong</creator><creator>Wu, Ya-Han</creator><creator>Zhu, Jun</creator><creator>Hayat, Tasawar</creator><creator>Alsaedi, Ahmed</creator><creator>Xu, Ya-Feng</creator><creator>Li, Zhao-Qian</creator><creator>Yang, Shang-Feng</creator><creator>Dai, Song-Yuan</creator><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0003-1938-4705</orcidid><orcidid>https://orcid.org/0000-0002-6931-9613</orcidid><orcidid>https://orcid.org/0000-0002-4921-0979</orcidid></search><sort><creationdate>2017</creationdate><title>Temperature-assisted rapid nucleation: a facile method to optimize the film morphology for perovskite solar cells</title><author>Ren, Ying-Ke ; Ding, Xi-Hong ; Wu, Ya-Han ; Zhu, Jun ; Hayat, Tasawar ; Alsaedi, Ahmed ; Xu, Ya-Feng ; Li, Zhao-Qian ; Yang, Shang-Feng ; Dai, Song-Yuan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c375t-f188cc2daf16324972e094cf2ed3310ec25878191e613c659c3559c2d21d1603</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ren, Ying-Ke</creatorcontrib><creatorcontrib>Ding, Xi-Hong</creatorcontrib><creatorcontrib>Wu, Ya-Han</creatorcontrib><creatorcontrib>Zhu, Jun</creatorcontrib><creatorcontrib>Hayat, Tasawar</creatorcontrib><creatorcontrib>Alsaedi, Ahmed</creatorcontrib><creatorcontrib>Xu, Ya-Feng</creatorcontrib><creatorcontrib>Li, Zhao-Qian</creatorcontrib><creatorcontrib>Yang, Shang-Feng</creatorcontrib><creatorcontrib>Dai, Song-Yuan</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ren, Ying-Ke</au><au>Ding, Xi-Hong</au><au>Wu, Ya-Han</au><au>Zhu, Jun</au><au>Hayat, Tasawar</au><au>Alsaedi, Ahmed</au><au>Xu, Ya-Feng</au><au>Li, Zhao-Qian</au><au>Yang, Shang-Feng</au><au>Dai, Song-Yuan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Temperature-assisted rapid nucleation: a facile method to optimize the film morphology for perovskite solar cells</atitle><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle><date>2017</date><risdate>2017</risdate><volume>5</volume><issue>38</issue><spage>20327</spage><epage>20333</epage><pages>20327-20333</pages><issn>2050-7488</issn><eissn>2050-7496</eissn><abstract>The nucleation stage has an important influence on the lead halide perovskite film morphology, and therefore the solar cell performance. Here, we introduce a facile temperature-assisted rapid nucleation (TRN) method to improve the film crystallization process and the film morphology. By employing low temperature anti-solvents (diethyl ether, chlorobenzene and toluene), we stimulate homogeneous nuclei growth, resulting in a highly dense perovskite thin layer. The TRN method prepared (FAPbI
3
)
0.85
(MAPbBr
3
)
0.15
devices exhibit a power conversion efficiency up to 19.2% and maintain over 85% of the original efficiency after 40 days of storage at room temperature under a relative humidity of 10–40%.</abstract><doi>10.1039/C7TA06334B</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0003-1938-4705</orcidid><orcidid>https://orcid.org/0000-0002-6931-9613</orcidid><orcidid>https://orcid.org/0000-0002-4921-0979</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 2050-7488 |
| ispartof | Journal of materials chemistry. A, Materials for energy and sustainability, 2017, Vol.5 (38), p.20327-20333 |
| issn | 2050-7488 2050-7496 |
| language | eng |
| recordid | cdi_crossref_primary_10_1039_C7TA06334B |
| source | Royal Society Of Chemistry Journals 2008- |
| title | Temperature-assisted rapid nucleation: a facile method to optimize the film morphology for perovskite solar cells |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-05T20%3A59%3A54IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-crossref&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Temperature-assisted%20rapid%20nucleation:%20a%20facile%20method%20to%20optimize%20the%20film%20morphology%20for%20perovskite%20solar%20cells&rft.jtitle=Journal%20of%20materials%20chemistry.%20A,%20Materials%20for%20energy%20and%20sustainability&rft.au=Ren,%20Ying-Ke&rft.date=2017&rft.volume=5&rft.issue=38&rft.spage=20327&rft.epage=20333&rft.pages=20327-20333&rft.issn=2050-7488&rft.eissn=2050-7496&rft_id=info:doi/10.1039/C7TA06334B&rft_dat=%3Ccrossref%3E10_1039_C7TA06334B%3C/crossref%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |