New small-molecule acceptors based on hexacyclic naphthalene(cyclopentadithiophene) for efficient non-fullerene organic solar cells
A series of new non-fullerene small molecule acceptors ( NTIC , NTIC-Me , NTIC-OMe and NTIC-F ) based on the acceptor–donor–acceptor (A–D–A) architecture, using hexacyclic naphthalene-(cyclopentadithiophene) as the central unit, were designed and synthesized. The non-fullerene OSC device based on PB...
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| Veröffentlicht in: | Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2017, Vol.5 (33), p.17204-17210 |
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| container_end_page | 17210 |
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| container_issue | 33 |
| container_start_page | 17204 |
| container_title | Journal of materials chemistry. A, Materials for energy and sustainability |
| container_volume | 5 |
| creator | Yi, Yuan-Qiu-Qiang Feng, Huanran Chang, Meijia Zhang, Hongtao Wan, Xiangjian Li, Chenxi Chen, Yongsheng |
| description | A series of new non-fullerene small molecule acceptors (
NTIC
,
NTIC-Me
,
NTIC-OMe
and
NTIC-F
) based on the acceptor–donor–acceptor (A–D–A) architecture, using hexacyclic naphthalene-(cyclopentadithiophene) as the central unit, were designed and synthesized. The non-fullerene OSC device based on PBDB-T:
NTIC
showed a highest PCE of 8.63%. With a relatively high-lying LUMO level of
NTIC-OMe
, the PBDB-T:
NTIC-OMe
based device obtained a comparatively high
V
oc
of 0.965 V and a PCE of 8.61% simultaneously. The results demonstrate that the naphthalene core is a promising building block for constructing highly efficient non-fullerene acceptors and further boosting the photovoltaic performance of the devices. |
| doi_str_mv | 10.1039/C7TA05809H |
| format | Article |
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NTIC
,
NTIC-Me
,
NTIC-OMe
and
NTIC-F
) based on the acceptor–donor–acceptor (A–D–A) architecture, using hexacyclic naphthalene-(cyclopentadithiophene) as the central unit, were designed and synthesized. The non-fullerene OSC device based on PBDB-T:
NTIC
showed a highest PCE of 8.63%. With a relatively high-lying LUMO level of
NTIC-OMe
, the PBDB-T:
NTIC-OMe
based device obtained a comparatively high
V
oc
of 0.965 V and a PCE of 8.61% simultaneously. The results demonstrate that the naphthalene core is a promising building block for constructing highly efficient non-fullerene acceptors and further boosting the photovoltaic performance of the devices.</description><identifier>ISSN: 2050-7488</identifier><identifier>EISSN: 2050-7496</identifier><identifier>DOI: 10.1039/C7TA05809H</identifier><language>eng</language><ispartof>Journal of materials chemistry. A, Materials for energy and sustainability, 2017, Vol.5 (33), p.17204-17210</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c297t-b62705a41cde594d937885770e58bca88da6123e3cd9ec61b0707bf5b9ff5dd73</citedby><cites>FETCH-LOGICAL-c297t-b62705a41cde594d937885770e58bca88da6123e3cd9ec61b0707bf5b9ff5dd73</cites><orcidid>0000-0001-5266-8510 ; 0000-0003-3522-7056 ; 0000-0003-1448-8177</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,781,785,4025,27928,27929,27930</link.rule.ids></links><search><creatorcontrib>Yi, Yuan-Qiu-Qiang</creatorcontrib><creatorcontrib>Feng, Huanran</creatorcontrib><creatorcontrib>Chang, Meijia</creatorcontrib><creatorcontrib>Zhang, Hongtao</creatorcontrib><creatorcontrib>Wan, Xiangjian</creatorcontrib><creatorcontrib>Li, Chenxi</creatorcontrib><creatorcontrib>Chen, Yongsheng</creatorcontrib><title>New small-molecule acceptors based on hexacyclic naphthalene(cyclopentadithiophene) for efficient non-fullerene organic solar cells</title><title>Journal of materials chemistry. A, Materials for energy and sustainability</title><description>A series of new non-fullerene small molecule acceptors (
NTIC
,
NTIC-Me
,
NTIC-OMe
and
NTIC-F
) based on the acceptor–donor–acceptor (A–D–A) architecture, using hexacyclic naphthalene-(cyclopentadithiophene) as the central unit, were designed and synthesized. The non-fullerene OSC device based on PBDB-T:
NTIC
showed a highest PCE of 8.63%. With a relatively high-lying LUMO level of
NTIC-OMe
, the PBDB-T:
NTIC-OMe
based device obtained a comparatively high
V
oc
of 0.965 V and a PCE of 8.61% simultaneously. The results demonstrate that the naphthalene core is a promising building block for constructing highly efficient non-fullerene acceptors and further boosting the photovoltaic performance of the devices.</description><issn>2050-7488</issn><issn>2050-7496</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNpFkMFLwzAYxYMoOOYu_gU5qlD92i5NchxFnTD0Ms8lTb7YSpaUpEN39h-3Q9F3eY_fg3d4hFzmcJtDKe9qvl0BEyDXJ2RWAIOML2V1-peFOCeLlN5hkgCopJyRr2f8oGmnnMt2waHeO6RKaxzGEBNtVUJDg6cdfip90K7X1KuhGzvl0OPVEYUB_ahMP3Z9GLqJXlMbIkVre91PFfXBZ3bvHMappCG-KT_NpOBUpBqdSxfkzCqXcPHrc_L6cL-t19nm5fGpXm0yXUg-Zm1VcGBqmWuDTC6NLLkQjHNAJlqthDCqyosSS20k6ipvgQNvLWultcwYXs7Jzc-ujiGliLYZYr9T8dDk0BwfbP4fLL8BtDVm8w</recordid><startdate>2017</startdate><enddate>2017</enddate><creator>Yi, Yuan-Qiu-Qiang</creator><creator>Feng, Huanran</creator><creator>Chang, Meijia</creator><creator>Zhang, Hongtao</creator><creator>Wan, Xiangjian</creator><creator>Li, Chenxi</creator><creator>Chen, Yongsheng</creator><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-5266-8510</orcidid><orcidid>https://orcid.org/0000-0003-3522-7056</orcidid><orcidid>https://orcid.org/0000-0003-1448-8177</orcidid></search><sort><creationdate>2017</creationdate><title>New small-molecule acceptors based on hexacyclic naphthalene(cyclopentadithiophene) for efficient non-fullerene organic solar cells</title><author>Yi, Yuan-Qiu-Qiang ; Feng, Huanran ; Chang, Meijia ; Zhang, Hongtao ; Wan, Xiangjian ; Li, Chenxi ; Chen, Yongsheng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c297t-b62705a41cde594d937885770e58bca88da6123e3cd9ec61b0707bf5b9ff5dd73</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yi, Yuan-Qiu-Qiang</creatorcontrib><creatorcontrib>Feng, Huanran</creatorcontrib><creatorcontrib>Chang, Meijia</creatorcontrib><creatorcontrib>Zhang, Hongtao</creatorcontrib><creatorcontrib>Wan, Xiangjian</creatorcontrib><creatorcontrib>Li, Chenxi</creatorcontrib><creatorcontrib>Chen, Yongsheng</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yi, Yuan-Qiu-Qiang</au><au>Feng, Huanran</au><au>Chang, Meijia</au><au>Zhang, Hongtao</au><au>Wan, Xiangjian</au><au>Li, Chenxi</au><au>Chen, Yongsheng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>New small-molecule acceptors based on hexacyclic naphthalene(cyclopentadithiophene) for efficient non-fullerene organic solar cells</atitle><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle><date>2017</date><risdate>2017</risdate><volume>5</volume><issue>33</issue><spage>17204</spage><epage>17210</epage><pages>17204-17210</pages><issn>2050-7488</issn><eissn>2050-7496</eissn><abstract>A series of new non-fullerene small molecule acceptors (
NTIC
,
NTIC-Me
,
NTIC-OMe
and
NTIC-F
) based on the acceptor–donor–acceptor (A–D–A) architecture, using hexacyclic naphthalene-(cyclopentadithiophene) as the central unit, were designed and synthesized. The non-fullerene OSC device based on PBDB-T:
NTIC
showed a highest PCE of 8.63%. With a relatively high-lying LUMO level of
NTIC-OMe
, the PBDB-T:
NTIC-OMe
based device obtained a comparatively high
V
oc
of 0.965 V and a PCE of 8.61% simultaneously. The results demonstrate that the naphthalene core is a promising building block for constructing highly efficient non-fullerene acceptors and further boosting the photovoltaic performance of the devices.</abstract><doi>10.1039/C7TA05809H</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0001-5266-8510</orcidid><orcidid>https://orcid.org/0000-0003-3522-7056</orcidid><orcidid>https://orcid.org/0000-0003-1448-8177</orcidid></addata></record> |
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| ispartof | Journal of materials chemistry. A, Materials for energy and sustainability, 2017, Vol.5 (33), p.17204-17210 |
| issn | 2050-7488 2050-7496 |
| language | eng |
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| source | Royal Society Of Chemistry Journals |
| title | New small-molecule acceptors based on hexacyclic naphthalene(cyclopentadithiophene) for efficient non-fullerene organic solar cells |
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