Occurrence of pharmaceuticals and personal care products, and their associated environmental risks in Guanting Reservoir and its upstream rivers in north China

Eighteen selected pharmaceuticals and personal care products (PPCPs), consisting of five non-antibiotic pharmaceuticals (N-APs), four sulfonamides (SAs), four tetracyclines (TCs), four macrolides (MCs), and one quinolone (QN) were detected in surface water and sediments from Guanting Reservoir (GTR)...

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Veröffentlicht in:RSC advances 2018-01, Vol.8 (9), p.473-4712
Hauptverfasser: Zhang, Panwei, Zhou, Huaidong, Li, Kun, Zhao, Xiaohui, Liu, Qiaona, Li, Dongjiao, Zhao, Gaofeng, Wang, Liang
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container_issue 9
container_start_page 473
container_title RSC advances
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creator Zhang, Panwei
Zhou, Huaidong
Li, Kun
Zhao, Xiaohui
Liu, Qiaona
Li, Dongjiao
Zhao, Gaofeng
Wang, Liang
description Eighteen selected pharmaceuticals and personal care products (PPCPs), consisting of five non-antibiotic pharmaceuticals (N-APs), four sulfonamides (SAs), four tetracyclines (TCs), four macrolides (MCs), and one quinolone (QN) were detected in surface water and sediments from Guanting Reservoir (GTR) and its upstream rivers in north China. Acetaminophen, caffeine, chlorotetracycline, and ofloxacin were detected with 100% frequency in the surface water of GTR and its upstream rivers, while diltiazem was also detected with 100% frequency in surface water from the reservoir's upstream rivers. Acetaminophen and caffeine were detected with 100% frequency in sediments from GTR and its upstream rivers, while high concentrations of ofloxacin in GTR, and carbamazepine, tetracycline, and chlortetracycline in upstream rivers were also detected in 100% of samples. Five N-APs, especially acetaminophen and caffeine, were prominent pollutants. The mean concentrations of acetaminophen were 155 and 302 ng L −1 in surface water and 529 and 202 ng g −1 in sediments from GTR and upstream rivers, respectively. The mean concentrations of caffeine were 208 and 338 ng L −1 in surface water samples and 1430 and 1020 ng g −1 in sediments from GTR and upstream rivers, respectively. The geographical differences in PPCP concentrations were largely due to anthropogenic activities. Sewage discharged from Zhangjiakou City and human activities around the GTR basin were the main sources of PPCPs in this area. An environmental risk assessment for the worst-case scenario was undertaken using calculated risk quotients, which indicated a medium risk from erythromycin in GTR and a high risk in its upstream rivers. Eighteen selected pharmaceuticals and personal care products (PPCPs) were detected in surface water and sediments from the Guanting Reservoir (GTR) and its upstream rivers.
doi_str_mv 10.1039/c7ra12945a
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Acetaminophen, caffeine, chlorotetracycline, and ofloxacin were detected with 100% frequency in the surface water of GTR and its upstream rivers, while diltiazem was also detected with 100% frequency in surface water from the reservoir's upstream rivers. Acetaminophen and caffeine were detected with 100% frequency in sediments from GTR and its upstream rivers, while high concentrations of ofloxacin in GTR, and carbamazepine, tetracycline, and chlortetracycline in upstream rivers were also detected in 100% of samples. Five N-APs, especially acetaminophen and caffeine, were prominent pollutants. The mean concentrations of acetaminophen were 155 and 302 ng L −1 in surface water and 529 and 202 ng g −1 in sediments from GTR and upstream rivers, respectively. The mean concentrations of caffeine were 208 and 338 ng L −1 in surface water samples and 1430 and 1020 ng g −1 in sediments from GTR and upstream rivers, respectively. 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Acetaminophen, caffeine, chlorotetracycline, and ofloxacin were detected with 100% frequency in the surface water of GTR and its upstream rivers, while diltiazem was also detected with 100% frequency in surface water from the reservoir's upstream rivers. Acetaminophen and caffeine were detected with 100% frequency in sediments from GTR and its upstream rivers, while high concentrations of ofloxacin in GTR, and carbamazepine, tetracycline, and chlortetracycline in upstream rivers were also detected in 100% of samples. Five N-APs, especially acetaminophen and caffeine, were prominent pollutants. The mean concentrations of acetaminophen were 155 and 302 ng L −1 in surface water and 529 and 202 ng g −1 in sediments from GTR and upstream rivers, respectively. The mean concentrations of caffeine were 208 and 338 ng L −1 in surface water samples and 1430 and 1020 ng g −1 in sediments from GTR and upstream rivers, respectively. 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Zhou, Huaidong ; Li, Kun ; Zhao, Xiaohui ; Liu, Qiaona ; Li, Dongjiao ; Zhao, Gaofeng ; Wang, Liang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c428t-16acc498aabdd447eeabbe77ce8444cb020487c0352e011ee2c42cef9a23131a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Analgesics</topic><topic>Antibiotics</topic><topic>Caffeine</topic><topic>Chemistry</topic><topic>Cosmetics industry</topic><topic>Diltiazem</topic><topic>Ecological risk assessment</topic><topic>Erythromycin</topic><topic>Human influences</topic><topic>Personal grooming</topic><topic>Pharmaceuticals</topic><topic>Pollutants</topic><topic>Quotients</topic><topic>Risk assessment</topic><topic>Rivers</topic><topic>Sediments</topic><topic>Sewage</topic><topic>Sulfonamides</topic><topic>Surface water</topic><topic>Tetracyclines</topic><topic>Upstream</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Panwei</creatorcontrib><creatorcontrib>Zhou, Huaidong</creatorcontrib><creatorcontrib>Li, Kun</creatorcontrib><creatorcontrib>Zhao, Xiaohui</creatorcontrib><creatorcontrib>Liu, Qiaona</creatorcontrib><creatorcontrib>Li, Dongjiao</creatorcontrib><creatorcontrib>Zhao, Gaofeng</creatorcontrib><creatorcontrib>Wang, Liang</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>RSC advances</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Panwei</au><au>Zhou, Huaidong</au><au>Li, Kun</au><au>Zhao, Xiaohui</au><au>Liu, Qiaona</au><au>Li, Dongjiao</au><au>Zhao, Gaofeng</au><au>Wang, Liang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Occurrence of pharmaceuticals and personal care products, and their associated environmental risks in Guanting Reservoir and its upstream rivers in north China</atitle><jtitle>RSC advances</jtitle><addtitle>RSC Adv</addtitle><date>2018-01-01</date><risdate>2018</risdate><volume>8</volume><issue>9</issue><spage>473</spage><epage>4712</epage><pages>473-4712</pages><issn>2046-2069</issn><eissn>2046-2069</eissn><abstract>Eighteen selected pharmaceuticals and personal care products (PPCPs), consisting of five non-antibiotic pharmaceuticals (N-APs), four sulfonamides (SAs), four tetracyclines (TCs), four macrolides (MCs), and one quinolone (QN) were detected in surface water and sediments from Guanting Reservoir (GTR) and its upstream rivers in north China. Acetaminophen, caffeine, chlorotetracycline, and ofloxacin were detected with 100% frequency in the surface water of GTR and its upstream rivers, while diltiazem was also detected with 100% frequency in surface water from the reservoir's upstream rivers. Acetaminophen and caffeine were detected with 100% frequency in sediments from GTR and its upstream rivers, while high concentrations of ofloxacin in GTR, and carbamazepine, tetracycline, and chlortetracycline in upstream rivers were also detected in 100% of samples. Five N-APs, especially acetaminophen and caffeine, were prominent pollutants. The mean concentrations of acetaminophen were 155 and 302 ng L −1 in surface water and 529 and 202 ng g −1 in sediments from GTR and upstream rivers, respectively. The mean concentrations of caffeine were 208 and 338 ng L −1 in surface water samples and 1430 and 1020 ng g −1 in sediments from GTR and upstream rivers, respectively. The geographical differences in PPCP concentrations were largely due to anthropogenic activities. Sewage discharged from Zhangjiakou City and human activities around the GTR basin were the main sources of PPCPs in this area. An environmental risk assessment for the worst-case scenario was undertaken using calculated risk quotients, which indicated a medium risk from erythromycin in GTR and a high risk in its upstream rivers. Eighteen selected pharmaceuticals and personal care products (PPCPs) were detected in surface water and sediments from the Guanting Reservoir (GTR) and its upstream rivers.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>35539549</pmid><doi>10.1039/c7ra12945a</doi><tpages>1</tpages><orcidid>https://orcid.org/0000-0002-0573-2660</orcidid><oa>free_for_read</oa></addata></record>
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subjects Analgesics
Antibiotics
Caffeine
Chemistry
Cosmetics industry
Diltiazem
Ecological risk assessment
Erythromycin
Human influences
Personal grooming
Pharmaceuticals
Pollutants
Quotients
Risk assessment
Rivers
Sediments
Sewage
Sulfonamides
Surface water
Tetracyclines
Upstream
title Occurrence of pharmaceuticals and personal care products, and their associated environmental risks in Guanting Reservoir and its upstream rivers in north China
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