Sunlight-assisted, biocatalytic formate synthesis from CO 2 and water using silicon-based photoelectrochemical cells
We report on a silicon-based photoelectrochemical cell that integrates a formate dehydrogenase from Thiobacillus sp. (TsFDH) to convert CO 2 to formate using water as an electron donor under visible light irradiation and an applied bias. Our current study suggests that the deliberate integration of...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2016, Vol.52 (62), p.9723-9726 |
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| container_issue | 62 |
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| container_title | Chemical communications (Cambridge, England) |
| container_volume | 52 |
| creator | Son, Eun Jin Ko, Jong Wan Kuk, Su Keun Choe, Hyunjun Lee, Sumi Kim, Jae Hong Nam, Dong Heon Ryu, Gyeong Min Kim, Yong Hwan Park, Chan Beum |
| description | We report on a silicon-based photoelectrochemical cell that integrates a formate dehydrogenase from
Thiobacillus
sp. (TsFDH) to convert CO
2
to formate using water as an electron donor under visible light irradiation and an applied bias. Our current study suggests that the deliberate integration of biocatalysis to a light-harvesting platform could provide an opportunity to synthesize valuable chemicals with the use of earth-abundant materials and sustainable resources. |
| doi_str_mv | 10.1039/C6CC04661D |
| format | Article |
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Thiobacillus
sp. (TsFDH) to convert CO
2
to formate using water as an electron donor under visible light irradiation and an applied bias. Our current study suggests that the deliberate integration of biocatalysis to a light-harvesting platform could provide an opportunity to synthesize valuable chemicals with the use of earth-abundant materials and sustainable resources.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/C6CC04661D</identifier><language>eng</language><ispartof>Chemical communications (Cambridge, England), 2016, Vol.52 (62), p.9723-9726</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c76D-94389c036edf27b1ccc1d83a413cb612af1899ac99338f1fd9c74a6eec0664cd3</citedby><cites>FETCH-LOGICAL-c76D-94389c036edf27b1ccc1d83a413cb612af1899ac99338f1fd9c74a6eec0664cd3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,4024,27923,27924,27925</link.rule.ids></links><search><creatorcontrib>Son, Eun Jin</creatorcontrib><creatorcontrib>Ko, Jong Wan</creatorcontrib><creatorcontrib>Kuk, Su Keun</creatorcontrib><creatorcontrib>Choe, Hyunjun</creatorcontrib><creatorcontrib>Lee, Sumi</creatorcontrib><creatorcontrib>Kim, Jae Hong</creatorcontrib><creatorcontrib>Nam, Dong Heon</creatorcontrib><creatorcontrib>Ryu, Gyeong Min</creatorcontrib><creatorcontrib>Kim, Yong Hwan</creatorcontrib><creatorcontrib>Park, Chan Beum</creatorcontrib><title>Sunlight-assisted, biocatalytic formate synthesis from CO 2 and water using silicon-based photoelectrochemical cells</title><title>Chemical communications (Cambridge, England)</title><description>We report on a silicon-based photoelectrochemical cell that integrates a formate dehydrogenase from
Thiobacillus
sp. (TsFDH) to convert CO
2
to formate using water as an electron donor under visible light irradiation and an applied bias. Our current study suggests that the deliberate integration of biocatalysis to a light-harvesting platform could provide an opportunity to synthesize valuable chemicals with the use of earth-abundant materials and sustainable resources.</description><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><recordid>eNpFkE1LAzEYhIMoWKsXf0HOYjRpstnNUbZ-QaEHe_C2ZN8k3Uh2U5IU6b-3RcG5zMAMc3gQumX0gVGuHlvZtlRIyZZnaMa4FKQSzef5KVeK1FxUl-gq5y96FKuaGSof-yn47VCIztnnYs097n0EXXQ4FA_YxTTqYnE-TGWwxwl2KY64XeMF1pPB38cy4X320xZnHzzEifQ6W4N3QyzRBgslRRjs6EEHDDaEfI0unA7Z3vz5HG1enjftG1mtX9_bpxWBWi6JErxRQLm0xi3qngEAMw3XgnHoJVtoxxqlNCjFeeOYMwpqoaW1QKUUYPgc3f3eQoo5J-u6XfKjToeO0e6Eq_vHxX8AemZf2g</recordid><startdate>2016</startdate><enddate>2016</enddate><creator>Son, Eun Jin</creator><creator>Ko, Jong Wan</creator><creator>Kuk, Su Keun</creator><creator>Choe, Hyunjun</creator><creator>Lee, Sumi</creator><creator>Kim, Jae Hong</creator><creator>Nam, Dong Heon</creator><creator>Ryu, Gyeong Min</creator><creator>Kim, Yong Hwan</creator><creator>Park, Chan Beum</creator><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>2016</creationdate><title>Sunlight-assisted, biocatalytic formate synthesis from CO 2 and water using silicon-based photoelectrochemical cells</title><author>Son, Eun Jin ; Ko, Jong Wan ; Kuk, Su Keun ; Choe, Hyunjun ; Lee, Sumi ; Kim, Jae Hong ; Nam, Dong Heon ; Ryu, Gyeong Min ; Kim, Yong Hwan ; Park, Chan Beum</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c76D-94389c036edf27b1ccc1d83a413cb612af1899ac99338f1fd9c74a6eec0664cd3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Son, Eun Jin</creatorcontrib><creatorcontrib>Ko, Jong Wan</creatorcontrib><creatorcontrib>Kuk, Su Keun</creatorcontrib><creatorcontrib>Choe, Hyunjun</creatorcontrib><creatorcontrib>Lee, Sumi</creatorcontrib><creatorcontrib>Kim, Jae Hong</creatorcontrib><creatorcontrib>Nam, Dong Heon</creatorcontrib><creatorcontrib>Ryu, Gyeong Min</creatorcontrib><creatorcontrib>Kim, Yong Hwan</creatorcontrib><creatorcontrib>Park, Chan Beum</creatorcontrib><collection>CrossRef</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Son, Eun Jin</au><au>Ko, Jong Wan</au><au>Kuk, Su Keun</au><au>Choe, Hyunjun</au><au>Lee, Sumi</au><au>Kim, Jae Hong</au><au>Nam, Dong Heon</au><au>Ryu, Gyeong Min</au><au>Kim, Yong Hwan</au><au>Park, Chan Beum</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Sunlight-assisted, biocatalytic formate synthesis from CO 2 and water using silicon-based photoelectrochemical cells</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><date>2016</date><risdate>2016</risdate><volume>52</volume><issue>62</issue><spage>9723</spage><epage>9726</epage><pages>9723-9726</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>We report on a silicon-based photoelectrochemical cell that integrates a formate dehydrogenase from
Thiobacillus
sp. (TsFDH) to convert CO
2
to formate using water as an electron donor under visible light irradiation and an applied bias. Our current study suggests that the deliberate integration of biocatalysis to a light-harvesting platform could provide an opportunity to synthesize valuable chemicals with the use of earth-abundant materials and sustainable resources.</abstract><doi>10.1039/C6CC04661D</doi><tpages>4</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2016, Vol.52 (62), p.9723-9726 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_crossref_primary_10_1039_C6CC04661D |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| title | Sunlight-assisted, biocatalytic formate synthesis from CO 2 and water using silicon-based photoelectrochemical cells |
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