Amplitude- and Phase-Resolved Near-Field Mapping of Infrared Antenna Modes by Transmission-Mode Scattering-Type Near-Field Microscopy
We describe transmission-mode scattering-type near-field optical microscopy (s-SNOM) with interferometric detection. Using this technique, we map the near-field modes of infrared antennas in both amplitude and phase. The use of dielectric probing tips, higher-harmonic demodulation, and a complex-val...
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Veröffentlicht in: | Journal of physical chemistry. C 2010-04, Vol.114 (16), p.7341-7345 |
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creator | Schnell, Martin Garcia-Etxarri, Aitzol Huber, Andreas J Crozier, Kenneth B Borisov, Andrei Aizpurua, Javier Hillenbrand, Rainer |
description | We describe transmission-mode scattering-type near-field optical microscopy (s-SNOM) with interferometric detection. Using this technique, we map the near-field modes of infrared antennas in both amplitude and phase. The use of dielectric probing tips, higher-harmonic demodulation, and a complex-valued subtraction of residual background yields accurate near-field images of the antenna modes. We map metallic nanorods, disks, and triangles, designed for antenna resonance at mid-infrared frequencies, in good agreement with numerical calculations of the modal field distribution. Furthermore, we show that transmission-mode s-SNOM can map the z-component of the antenna near fields. Our results establish a basis for future near-field characterization of complex antenna structures for molecular sensing and spectroscopy. |
doi_str_mv | 10.1021/jp909252z |
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Using this technique, we map the near-field modes of infrared antennas in both amplitude and phase. The use of dielectric probing tips, higher-harmonic demodulation, and a complex-valued subtraction of residual background yields accurate near-field images of the antenna modes. We map metallic nanorods, disks, and triangles, designed for antenna resonance at mid-infrared frequencies, in good agreement with numerical calculations of the modal field distribution. Furthermore, we show that transmission-mode s-SNOM can map the z-component of the antenna near fields. Our results establish a basis for future near-field characterization of complex antenna structures for molecular sensing and spectroscopy.</description><identifier>ISSN: 1932-7447</identifier><identifier>EISSN: 1932-7455</identifier><identifier>DOI: 10.1021/jp909252z</identifier><language>eng</language><publisher>American Chemical Society</publisher><ispartof>Journal of physical chemistry. 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C</title><addtitle>J. Phys. Chem. C</addtitle><description>We describe transmission-mode scattering-type near-field optical microscopy (s-SNOM) with interferometric detection. Using this technique, we map the near-field modes of infrared antennas in both amplitude and phase. The use of dielectric probing tips, higher-harmonic demodulation, and a complex-valued subtraction of residual background yields accurate near-field images of the antenna modes. We map metallic nanorods, disks, and triangles, designed for antenna resonance at mid-infrared frequencies, in good agreement with numerical calculations of the modal field distribution. Furthermore, we show that transmission-mode s-SNOM can map the z-component of the antenna near fields. 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C</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Schnell, Martin</au><au>Garcia-Etxarri, Aitzol</au><au>Huber, Andreas J</au><au>Crozier, Kenneth B</au><au>Borisov, Andrei</au><au>Aizpurua, Javier</au><au>Hillenbrand, Rainer</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Amplitude- and Phase-Resolved Near-Field Mapping of Infrared Antenna Modes by Transmission-Mode Scattering-Type Near-Field Microscopy</atitle><jtitle>Journal of physical chemistry. C</jtitle><addtitle>J. Phys. Chem. C</addtitle><date>2010-04-29</date><risdate>2010</risdate><volume>114</volume><issue>16</issue><spage>7341</spage><epage>7345</epage><pages>7341-7345</pages><issn>1932-7447</issn><eissn>1932-7455</eissn><abstract>We describe transmission-mode scattering-type near-field optical microscopy (s-SNOM) with interferometric detection. Using this technique, we map the near-field modes of infrared antennas in both amplitude and phase. The use of dielectric probing tips, higher-harmonic demodulation, and a complex-valued subtraction of residual background yields accurate near-field images of the antenna modes. We map metallic nanorods, disks, and triangles, designed for antenna resonance at mid-infrared frequencies, in good agreement with numerical calculations of the modal field distribution. Furthermore, we show that transmission-mode s-SNOM can map the z-component of the antenna near fields. Our results establish a basis for future near-field characterization of complex antenna structures for molecular sensing and spectroscopy.</abstract><pub>American Chemical Society</pub><doi>10.1021/jp909252z</doi><tpages>5</tpages><oa>free_for_read</oa></addata></record> |
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title | Amplitude- and Phase-Resolved Near-Field Mapping of Infrared Antenna Modes by Transmission-Mode Scattering-Type Near-Field Microscopy |
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