Nanoscale Architectural Control and Macromolecular Engineering of Nonlinear Optical Dendrimers and Polymers for Electro-Optics

Nanoscale Architectural Control and Macromolecular Engineering of Nonlinear Optical Dendrimers and Polymers for Electro-Optics

Recent progress in developing highly efficient nonlinear optical dendrimers and polymers for high-performance electro-optic (EO) devices has been reviewed. Our efforts are focused on using nanoscale architectural control to tailor the size, shape, conformation, and functionality of NLO chromophores...

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Veröffentlicht in:The journal of physical chemistry. B 2004-06, Vol.108 (25), p.8523-8530
Hauptverfasser: Luo, Jingdong, Haller, Marnie, Ma, Hong, Liu, Sen, Kim, Tae-Dong, Tian, Yanqing, Chen, Baoquan, Jang, Sei-Hum, Dalton, Larry R, Jen, Alex K.-Y
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container_end_page 8530
container_issue 25
container_start_page 8523
container_title The journal of physical chemistry. B
container_volume 108
creator Luo, Jingdong
Haller, Marnie
Ma, Hong
Liu, Sen
Kim, Tae-Dong
Tian, Yanqing
Chen, Baoquan
Jang, Sei-Hum
Dalton, Larry R
Jen, Alex K.-Y
description Recent progress in developing highly efficient nonlinear optical dendrimers and polymers for high-performance electro-optic (EO) devices has been reviewed. Our efforts are focused on using nanoscale architectural control to tailor the size, shape, conformation, and functionality of NLO chromophores and macromolecules and studying their effects on poling efficiency. The structures of these materials vary from a 3-D-shaped dendritic chromophore, multifunctional dendrimers with the center core connected to NLO chromophores and cross-linkable functional groups at the periphery, to side-chain-dendronized NLO polymers. All the poling results from these systems have shown dramatically enhanced EO properties (a factor of 2−3) compared to conventional NLO polymers.
doi_str_mv 10.1021/jp036714o
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