Tetranuclear [Mn III Mn 3 IV O 4 ] Complexes as Spectroscopic Models of the S 2 State of the Oxygen Evolving Complex in Photosystem II

Despite extensive biochemical, spectroscopic, and computational studies, the mechanism of biological water oxidation by the oxygen evolving complex (OEC) of Photosystem II remains a subject of significant debate. Mechanistic proposals are guided by the characterization of reaction intermediates such...

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Veröffentlicht in:	Journal of the American Chemical Society 2018-12, Vol.140 (49), p.17175-17187
Hauptverfasser:	Lee, Heui Beom, Shiau, Angela A, Oyala, Paul H, Marchiori, David A, Gul, Sheraz, Chatterjee, Ruchira, Yano, Junko, Britt, R David, Agapie, Theodor
Format:	Artikel
Sprache:	eng
Schlagworte:	Biomimetic Materials - chemical synthesis Biomimetic Materials - chemistry Coordination Complexes - chemical synthesis Coordination Complexes - chemistry Electrochemistry Electron Spin Resonance Spectroscopy Magnetic Phenomena Manganese - chemistry Molecular Structure Oxidation-Reduction Oxygen - chemistry Photosystem II Protein Complex - chemistry Temperature
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