Toward Combined Carbon Capture and Recycling: Addition of an Amine Alters Product Selectivity from CO to Formic Acid in Manganese Catalyzed Reduction of CO 2

Owing to the energetic cost associated with CO release in carbon capture (CC), the combination of carbon capture and recycling (CCR) is an emerging area of research. In this approach, "captured CO ," typically generated by addition of amines, serves as a substrate for subsequent reduction....

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Veröffentlicht in:	Journal of the American Chemical Society 2020-10, Vol.142 (41), p.17589-17597
Hauptverfasser:	Bhattacharya, Moumita, Sebghati, Sepehr, VanderLinden, Ryan T, Saouma, Caroline T
Format:	Artikel
Sprache:	eng
Schlagworte:	Amines - chemistry Carbamates - chemistry Carbon - chemistry Carbon Dioxide - chemistry Carbon Monoxide - chemistry Catalysis Coordination Complexes - chemistry Electrochemical Techniques Formates - chemistry Hydrogen - chemistry Hydrogenation Ligands Manganese - chemistry Oxidation-Reduction Structure-Activity Relationship
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