Multiphase, Microdispersion Reactor for the Continuous Production of Methane Gas Hydrate
A continuous-jet hydrate reactor originally developed to generate a CO2 hydrate stream has been modified to continuously produce CH4 hydrate. The reactor has been tested in the Seafloor Process Simulator (SPS), a 72-L pressure vessel available at Oak Ridge National Laboratory. During experiments, th...
Gespeichert in:
| Veröffentlicht in: | Industrial & engineering chemistry research 2009-07, Vol.48 (13), p.6448-6452 |
|---|---|
| Hauptverfasser: | , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 6452 |
|---|---|
| container_issue | 13 |
| container_start_page | 6448 |
| container_title | Industrial & engineering chemistry research |
| container_volume | 48 |
| creator | Taboada-Serrano, Patricia Ulrich, Shannon Szymcek, Phillip McCallum, Scott D Phelps, Tommy J Palumbo, Anthony Tsouris, Costas |
| description | A continuous-jet hydrate reactor originally developed to generate a CO2 hydrate stream has been modified to continuously produce CH4 hydrate. The reactor has been tested in the Seafloor Process Simulator (SPS), a 72-L pressure vessel available at Oak Ridge National Laboratory. During experiments, the reactor was submerged in water inside the SPS and received water from the surrounding through a submersible pump and CH4 externally through a gas booster pump. Thermodynamic conditions in the hydrate stability regime were employed in the experiments. The reactor produced a continuous stream of CH4 hydrate, and based on pressure values and amount of gas injected, the conversion of gas to hydrate was estimated. A conversion of up to 70% was achieved using this reactor. |
| doi_str_mv | 10.1021/ie8019517 |
| format | Article |
| fullrecord | <record><control><sourceid>acs_cross</sourceid><recordid>TN_cdi_crossref_primary_10_1021_ie8019517</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>c521015029</sourcerecordid><originalsourceid>FETCH-LOGICAL-a326t-7dda3d759a0f9f49ac726c15f5b79286e8115f0eb54ea10aa8055a66e2962d0d3</originalsourceid><addsrcrecordid>eNptkE9LAzEQxYMoWKsHv0EuHgRXJ-kmmz1K0VZoUUTB2zLNH5pSN0uSPfTbu6VSPHgYhoHfPN57hFwzuGfA2YO3ClgtWHVCRkxwKASU4pSMQClVCKXEOblIaQMAQpTliHwt-2323RqTvaNLr2MwPnU2Jh9a-m5R5xCpGyavLZ2GNvu2D32ibwPY67yngqNLm9fYWjrDROc7EzHbS3LmcJvs1e8ek8_np4_pvFi8zl6mj4sCJ1zmojIGJ6YSNYKrXVmjrrjUTDixqmqupFVsOMCuRGmRAaIajKOUlteSGzCTMbk96A7WU4rWNV303xh3DYNmX0lzrGRgbw5sh0nj1kVstU_HB85BSVn_4VCnZhP62A4J_tH7AehCbN8</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Multiphase, Microdispersion Reactor for the Continuous Production of Methane Gas Hydrate</title><source>American Chemical Society Publications</source><creator>Taboada-Serrano, Patricia ; Ulrich, Shannon ; Szymcek, Phillip ; McCallum, Scott D ; Phelps, Tommy J ; Palumbo, Anthony ; Tsouris, Costas</creator><creatorcontrib>Taboada-Serrano, Patricia ; Ulrich, Shannon ; Szymcek, Phillip ; McCallum, Scott D ; Phelps, Tommy J ; Palumbo, Anthony ; Tsouris, Costas</creatorcontrib><description>A continuous-jet hydrate reactor originally developed to generate a CO2 hydrate stream has been modified to continuously produce CH4 hydrate. The reactor has been tested in the Seafloor Process Simulator (SPS), a 72-L pressure vessel available at Oak Ridge National Laboratory. During experiments, the reactor was submerged in water inside the SPS and received water from the surrounding through a submersible pump and CH4 externally through a gas booster pump. Thermodynamic conditions in the hydrate stability regime were employed in the experiments. The reactor produced a continuous stream of CH4 hydrate, and based on pressure values and amount of gas injected, the conversion of gas to hydrate was estimated. A conversion of up to 70% was achieved using this reactor.</description><identifier>ISSN: 0888-5885</identifier><identifier>EISSN: 1520-5045</identifier><identifier>DOI: 10.1021/ie8019517</identifier><identifier>CODEN: IECRED</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>Applied sciences ; Chemical engineering ; Exact sciences and technology ; Reactors</subject><ispartof>Industrial & engineering chemistry research, 2009-07, Vol.48 (13), p.6448-6452</ispartof><rights>Copyright © 2009 American Chemical Society</rights><rights>2009 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a326t-7dda3d759a0f9f49ac726c15f5b79286e8115f0eb54ea10aa8055a66e2962d0d3</citedby><cites>FETCH-LOGICAL-a326t-7dda3d759a0f9f49ac726c15f5b79286e8115f0eb54ea10aa8055a66e2962d0d3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/ie8019517$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/ie8019517$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,2765,27076,27924,27925,56738,56788</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=22086697$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Taboada-Serrano, Patricia</creatorcontrib><creatorcontrib>Ulrich, Shannon</creatorcontrib><creatorcontrib>Szymcek, Phillip</creatorcontrib><creatorcontrib>McCallum, Scott D</creatorcontrib><creatorcontrib>Phelps, Tommy J</creatorcontrib><creatorcontrib>Palumbo, Anthony</creatorcontrib><creatorcontrib>Tsouris, Costas</creatorcontrib><title>Multiphase, Microdispersion Reactor for the Continuous Production of Methane Gas Hydrate</title><title>Industrial & engineering chemistry research</title><addtitle>Ind. Eng. Chem. Res</addtitle><description>A continuous-jet hydrate reactor originally developed to generate a CO2 hydrate stream has been modified to continuously produce CH4 hydrate. The reactor has been tested in the Seafloor Process Simulator (SPS), a 72-L pressure vessel available at Oak Ridge National Laboratory. During experiments, the reactor was submerged in water inside the SPS and received water from the surrounding through a submersible pump and CH4 externally through a gas booster pump. Thermodynamic conditions in the hydrate stability regime were employed in the experiments. The reactor produced a continuous stream of CH4 hydrate, and based on pressure values and amount of gas injected, the conversion of gas to hydrate was estimated. A conversion of up to 70% was achieved using this reactor.</description><subject>Applied sciences</subject><subject>Chemical engineering</subject><subject>Exact sciences and technology</subject><subject>Reactors</subject><issn>0888-5885</issn><issn>1520-5045</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2009</creationdate><recordtype>article</recordtype><recordid>eNptkE9LAzEQxYMoWKsHv0EuHgRXJ-kmmz1K0VZoUUTB2zLNH5pSN0uSPfTbu6VSPHgYhoHfPN57hFwzuGfA2YO3ClgtWHVCRkxwKASU4pSMQClVCKXEOblIaQMAQpTliHwt-2323RqTvaNLr2MwPnU2Jh9a-m5R5xCpGyavLZ2GNvu2D32ibwPY67yngqNLm9fYWjrDROc7EzHbS3LmcJvs1e8ek8_np4_pvFi8zl6mj4sCJ1zmojIGJ6YSNYKrXVmjrrjUTDixqmqupFVsOMCuRGmRAaIajKOUlteSGzCTMbk96A7WU4rWNV303xh3DYNmX0lzrGRgbw5sh0nj1kVstU_HB85BSVn_4VCnZhP62A4J_tH7AehCbN8</recordid><startdate>20090701</startdate><enddate>20090701</enddate><creator>Taboada-Serrano, Patricia</creator><creator>Ulrich, Shannon</creator><creator>Szymcek, Phillip</creator><creator>McCallum, Scott D</creator><creator>Phelps, Tommy J</creator><creator>Palumbo, Anthony</creator><creator>Tsouris, Costas</creator><general>American Chemical Society</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20090701</creationdate><title>Multiphase, Microdispersion Reactor for the Continuous Production of Methane Gas Hydrate</title><author>Taboada-Serrano, Patricia ; Ulrich, Shannon ; Szymcek, Phillip ; McCallum, Scott D ; Phelps, Tommy J ; Palumbo, Anthony ; Tsouris, Costas</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a326t-7dda3d759a0f9f49ac726c15f5b79286e8115f0eb54ea10aa8055a66e2962d0d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2009</creationdate><topic>Applied sciences</topic><topic>Chemical engineering</topic><topic>Exact sciences and technology</topic><topic>Reactors</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Taboada-Serrano, Patricia</creatorcontrib><creatorcontrib>Ulrich, Shannon</creatorcontrib><creatorcontrib>Szymcek, Phillip</creatorcontrib><creatorcontrib>McCallum, Scott D</creatorcontrib><creatorcontrib>Phelps, Tommy J</creatorcontrib><creatorcontrib>Palumbo, Anthony</creatorcontrib><creatorcontrib>Tsouris, Costas</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><jtitle>Industrial & engineering chemistry research</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Taboada-Serrano, Patricia</au><au>Ulrich, Shannon</au><au>Szymcek, Phillip</au><au>McCallum, Scott D</au><au>Phelps, Tommy J</au><au>Palumbo, Anthony</au><au>Tsouris, Costas</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Multiphase, Microdispersion Reactor for the Continuous Production of Methane Gas Hydrate</atitle><jtitle>Industrial & engineering chemistry research</jtitle><addtitle>Ind. Eng. Chem. Res</addtitle><date>2009-07-01</date><risdate>2009</risdate><volume>48</volume><issue>13</issue><spage>6448</spage><epage>6452</epage><pages>6448-6452</pages><issn>0888-5885</issn><eissn>1520-5045</eissn><coden>IECRED</coden><abstract>A continuous-jet hydrate reactor originally developed to generate a CO2 hydrate stream has been modified to continuously produce CH4 hydrate. The reactor has been tested in the Seafloor Process Simulator (SPS), a 72-L pressure vessel available at Oak Ridge National Laboratory. During experiments, the reactor was submerged in water inside the SPS and received water from the surrounding through a submersible pump and CH4 externally through a gas booster pump. Thermodynamic conditions in the hydrate stability regime were employed in the experiments. The reactor produced a continuous stream of CH4 hydrate, and based on pressure values and amount of gas injected, the conversion of gas to hydrate was estimated. A conversion of up to 70% was achieved using this reactor.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><doi>10.1021/ie8019517</doi><tpages>5</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0888-5885 |
| ispartof | Industrial & engineering chemistry research, 2009-07, Vol.48 (13), p.6448-6452 |
| issn | 0888-5885 1520-5045 |
| language | eng |
| recordid | cdi_crossref_primary_10_1021_ie8019517 |
| source | American Chemical Society Publications |
| subjects | Applied sciences Chemical engineering Exact sciences and technology Reactors |
| title | Multiphase, Microdispersion Reactor for the Continuous Production of Methane Gas Hydrate |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-28T09%3A34%3A41IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-acs_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Multiphase,%20Microdispersion%20Reactor%20for%20the%20Continuous%20Production%20of%20Methane%20Gas%20Hydrate&rft.jtitle=Industrial%20&%20engineering%20chemistry%20research&rft.au=Taboada-Serrano,%20Patricia&rft.date=2009-07-01&rft.volume=48&rft.issue=13&rft.spage=6448&rft.epage=6452&rft.pages=6448-6452&rft.issn=0888-5885&rft.eissn=1520-5045&rft.coden=IECRED&rft_id=info:doi/10.1021/ie8019517&rft_dat=%3Cacs_cross%3Ec521015029%3C/acs_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |