Lightweight Ti 2 CT x MXene/Poly(vinyl alcohol) Composite Foams for Electromagnetic Wave Shielding with Absorption-Dominated Feature
Lightweight absorption-dominated electromagnetic interference (EMI) shielding materials are more attractive than conventional reflection-dominated counterparts because they minimize the twice pollution of the reflected electromagnetic (EM) wave. Here, porous Ti CT MXene/poly(vinyl alcohol) composite...
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Veröffentlicht in: | ACS applied materials & interfaces 2019-03, Vol.11 (10), p.10198-10207 |
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creator | Xu, Hailong Yin, Xiaowei Li, Xinliang Li, Minghang Liang, Shuang Zhang, Litong Cheng, Laifei |
description | Lightweight absorption-dominated electromagnetic interference (EMI) shielding materials are more attractive than conventional reflection-dominated counterparts because they minimize the twice pollution of the reflected electromagnetic (EM) wave. Here, porous Ti
CT
MXene/poly(vinyl alcohol) composite foams constructed by few-layered Ti
CT
(f-Ti
CT
) MXene and poly(vinyl alcohol) (PVA) are fabricated via a facile freeze-drying method. As superior EMI shielding materials, their calculated specific shielding effectiveness reaches up to 5136 dB cm
g
with an ultralow filler content of only 0.15 vol % and reflection effectiveness (SE
) of less than 2 dB, representing the excellent absorption-dominated shielding performance. Contrast experiment reveals that the good impedance matching derived from the multiple porous structures, internal reflection, and polarization effect (dipole and interfacial polarization) plays a synergistic role in the improved absorption efficiency and superior EMI shielding performance. Consequently, this work provides a promising MXene-based EMI shielding candidate with lightweight and high strength features. |
doi_str_mv | 10.1021/acsami.8b21671 |
format | Article |
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CT
MXene/poly(vinyl alcohol) composite foams constructed by few-layered Ti
CT
(f-Ti
CT
) MXene and poly(vinyl alcohol) (PVA) are fabricated via a facile freeze-drying method. As superior EMI shielding materials, their calculated specific shielding effectiveness reaches up to 5136 dB cm
g
with an ultralow filler content of only 0.15 vol % and reflection effectiveness (SE
) of less than 2 dB, representing the excellent absorption-dominated shielding performance. Contrast experiment reveals that the good impedance matching derived from the multiple porous structures, internal reflection, and polarization effect (dipole and interfacial polarization) plays a synergistic role in the improved absorption efficiency and superior EMI shielding performance. Consequently, this work provides a promising MXene-based EMI shielding candidate with lightweight and high strength features.</description><identifier>ISSN: 1944-8244</identifier><identifier>EISSN: 1944-8252</identifier><identifier>DOI: 10.1021/acsami.8b21671</identifier><identifier>PMID: 30689343</identifier><language>eng</language><publisher>United States</publisher><ispartof>ACS applied materials & interfaces, 2019-03, Vol.11 (10), p.10198-10207</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c177t-6e396c157dc3dc9821820c766d7e9497df124096d6745da21484cb0113783fa63</citedby><cites>FETCH-LOGICAL-c177t-6e396c157dc3dc9821820c766d7e9497df124096d6745da21484cb0113783fa63</cites><orcidid>0000-0001-6485-2614 ; 0000-0003-1223-1693 ; 0000-0001-8756-8624</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,2752,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30689343$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Xu, Hailong</creatorcontrib><creatorcontrib>Yin, Xiaowei</creatorcontrib><creatorcontrib>Li, Xinliang</creatorcontrib><creatorcontrib>Li, Minghang</creatorcontrib><creatorcontrib>Liang, Shuang</creatorcontrib><creatorcontrib>Zhang, Litong</creatorcontrib><creatorcontrib>Cheng, Laifei</creatorcontrib><title>Lightweight Ti 2 CT x MXene/Poly(vinyl alcohol) Composite Foams for Electromagnetic Wave Shielding with Absorption-Dominated Feature</title><title>ACS applied materials & interfaces</title><addtitle>ACS Appl Mater Interfaces</addtitle><description>Lightweight absorption-dominated electromagnetic interference (EMI) shielding materials are more attractive than conventional reflection-dominated counterparts because they minimize the twice pollution of the reflected electromagnetic (EM) wave. Here, porous Ti
CT
MXene/poly(vinyl alcohol) composite foams constructed by few-layered Ti
CT
(f-Ti
CT
) MXene and poly(vinyl alcohol) (PVA) are fabricated via a facile freeze-drying method. As superior EMI shielding materials, their calculated specific shielding effectiveness reaches up to 5136 dB cm
g
with an ultralow filler content of only 0.15 vol % and reflection effectiveness (SE
) of less than 2 dB, representing the excellent absorption-dominated shielding performance. Contrast experiment reveals that the good impedance matching derived from the multiple porous structures, internal reflection, and polarization effect (dipole and interfacial polarization) plays a synergistic role in the improved absorption efficiency and superior EMI shielding performance. Consequently, this work provides a promising MXene-based EMI shielding candidate with lightweight and high strength features.</description><issn>1944-8244</issn><issn>1944-8252</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNo9kM1PwjAAxRujEUSvHk2Pehj0a-12JAhqgtFEjN6Wru1YzbYuawG5-4crAbm89w7vvcMPgGuMhhgRPJLKy9oOk5xgLvAJ6OOUsSghMTk9ZsZ64ML7L4Q4JSg-Bz2KeJJSRvvgZ26XZdiYncKFhQROFvAbPn-axoxeXbW9XdtmW0FZKVe66g5OXN06b4OBMydrDwvXwWllVOhcLZeNCVbBD7k28K20ptK2WcKNDSUc5951bbCuie5dbRsZjIYzI8OqM5fgrJCVN1cHH4D32XQxeYzmLw9Pk_E8UliIEHFDU65wLLSiWqUJwQlBSnCuhUlZKnSBCUMp11ywWEuCWcJUjjCmIqGF5HQAhvtf1TnvO1NkbWdr2W0zjLIdzmyPMzvg_Bvc7AftKq-NPtb_-dFfmjlyjg</recordid><startdate>20190313</startdate><enddate>20190313</enddate><creator>Xu, Hailong</creator><creator>Yin, Xiaowei</creator><creator>Li, Xinliang</creator><creator>Li, Minghang</creator><creator>Liang, Shuang</creator><creator>Zhang, Litong</creator><creator>Cheng, Laifei</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-6485-2614</orcidid><orcidid>https://orcid.org/0000-0003-1223-1693</orcidid><orcidid>https://orcid.org/0000-0001-8756-8624</orcidid></search><sort><creationdate>20190313</creationdate><title>Lightweight Ti 2 CT x MXene/Poly(vinyl alcohol) Composite Foams for Electromagnetic Wave Shielding with Absorption-Dominated Feature</title><author>Xu, Hailong ; Yin, Xiaowei ; Li, Xinliang ; Li, Minghang ; Liang, Shuang ; Zhang, Litong ; Cheng, Laifei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c177t-6e396c157dc3dc9821820c766d7e9497df124096d6745da21484cb0113783fa63</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Xu, Hailong</creatorcontrib><creatorcontrib>Yin, Xiaowei</creatorcontrib><creatorcontrib>Li, Xinliang</creatorcontrib><creatorcontrib>Li, Minghang</creatorcontrib><creatorcontrib>Liang, Shuang</creatorcontrib><creatorcontrib>Zhang, Litong</creatorcontrib><creatorcontrib>Cheng, Laifei</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><jtitle>ACS applied materials & interfaces</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Xu, Hailong</au><au>Yin, Xiaowei</au><au>Li, Xinliang</au><au>Li, Minghang</au><au>Liang, Shuang</au><au>Zhang, Litong</au><au>Cheng, Laifei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Lightweight Ti 2 CT x MXene/Poly(vinyl alcohol) Composite Foams for Electromagnetic Wave Shielding with Absorption-Dominated Feature</atitle><jtitle>ACS applied materials & interfaces</jtitle><addtitle>ACS Appl Mater Interfaces</addtitle><date>2019-03-13</date><risdate>2019</risdate><volume>11</volume><issue>10</issue><spage>10198</spage><epage>10207</epage><pages>10198-10207</pages><issn>1944-8244</issn><eissn>1944-8252</eissn><abstract>Lightweight absorption-dominated electromagnetic interference (EMI) shielding materials are more attractive than conventional reflection-dominated counterparts because they minimize the twice pollution of the reflected electromagnetic (EM) wave. Here, porous Ti
CT
MXene/poly(vinyl alcohol) composite foams constructed by few-layered Ti
CT
(f-Ti
CT
) MXene and poly(vinyl alcohol) (PVA) are fabricated via a facile freeze-drying method. As superior EMI shielding materials, their calculated specific shielding effectiveness reaches up to 5136 dB cm
g
with an ultralow filler content of only 0.15 vol % and reflection effectiveness (SE
) of less than 2 dB, representing the excellent absorption-dominated shielding performance. Contrast experiment reveals that the good impedance matching derived from the multiple porous structures, internal reflection, and polarization effect (dipole and interfacial polarization) plays a synergistic role in the improved absorption efficiency and superior EMI shielding performance. Consequently, this work provides a promising MXene-based EMI shielding candidate with lightweight and high strength features.</abstract><cop>United States</cop><pmid>30689343</pmid><doi>10.1021/acsami.8b21671</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0001-6485-2614</orcidid><orcidid>https://orcid.org/0000-0003-1223-1693</orcidid><orcidid>https://orcid.org/0000-0001-8756-8624</orcidid></addata></record> |
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title | Lightweight Ti 2 CT x MXene/Poly(vinyl alcohol) Composite Foams for Electromagnetic Wave Shielding with Absorption-Dominated Feature |
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