High-Performance Self-Powered Photoelectrochemical Ultraviolet Photodetectors Based on an In 2 O 3 Nanocube Film
Ultraviolet photodetectors (UV PDs) have attracted significant attention due to their wide range of applications, such as underwater communication, biological analysis, and early fire warning systems. Indium oxide (In O ) is a candidate for developing high-performance photoelectrochemical (PEC)-type...
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Veröffentlicht in: | ACS applied materials & interfaces 2024-04, Vol.16 (15), p.19167-19174 |
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creator | Zhang, Nana Cui, Mengqi Zhou, Junxin Shao, Zhitao Gao, Xinyu Liu, Jiaming Sun, Ruyu Zhang, Yuan Li, Wenhui Li, Xinghan Yao, Jing Gao, Feng Feng, Wei |
description | Ultraviolet photodetectors (UV PDs) have attracted significant attention due to their wide range of applications, such as underwater communication, biological analysis, and early fire warning systems. Indium oxide (In
O
) is a candidate for developing high-performance photoelectrochemical (PEC)-type UV PDs owing to its high UV absorption and good stability. However, the self-powered photoresponse of the previously reported In
O
-based PEC UV PDs is unsatisfactory. In this work, high-performance self-powered PEC UV PDs were constructed by using an In
O
nanocube film (NCF) as a photoanode. In
O
NCF photoanodes were synthesized on FTO by using hydrothermal methods with a calcining process. The influence of the electrolyte concentration, bias potential, and irradiation light on the photoresponse properties was systematically studied. In
O
NCF PEC UV PDs exhibit outstanding self-powered photoresponses to 365 nm UV light with a high responsivity of 44.43 mA/W and fast response speed (20/30 ms) under zero bias potential, these results are superior to those of previously reported In
O
-based PEC UV PDs. The improved self-powered photoresponse is attributed to the higher photogenerated carrier separation efficiency and faster charge transport of the in-situ grown In
O
NCF. In addition, these PDs exhibit excellent multicycle stability, maintaining the photocurrent at 98.69% of the initial value after 700 optical switching cycles. Therefore, our results prove the great promise of In
O
in self-powered PEC UV PDs. |
doi_str_mv | 10.1021/acsami.4c00801 |
format | Article |
fullrecord | <record><control><sourceid>pubmed_cross</sourceid><recordid>TN_cdi_crossref_primary_10_1021_acsami_4c00801</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>38569197</sourcerecordid><originalsourceid>FETCH-LOGICAL-c1077-c3b1429289a3ccedb4eb41705514ac5280af728f0c2013f48807c9bbc69d3a6e3</originalsourceid><addsrcrecordid>eNo9kE9PwkAQRzdGI4hePZr9AsXZP223RyUiJkRIlHOznU6lpu2S3aLx24spcpo5vPc7PMZuBUwFSHFvMdi2nmoEMCDO2FhkWkdGxvL89Gs9YlchfAIkSkJ8yUbKxEkmsnTMdov6YxutyVfOt7ZD4m_UVNHafZOnkq-3rnfUEPbe4ZbaGm3DN03v7VftGuoHoKT-QDgf-KMNB8t13Hb8peOSr7jir7ZzuC-Iz-umvWYXlW0C3RzvhG3mT--zRbRcPb_MHpYRCkjTCFUhtMykyaxCpLLQVGiRQhwLbTGWBmyVSlMBShCq0sZAillRYJKVyiakJmw67KJ3IXiq8p2vW-t_cgH5X7p8SJcf0x2Eu0HY7YuWyhP-30r9Ajhha7s</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>High-Performance Self-Powered Photoelectrochemical Ultraviolet Photodetectors Based on an In 2 O 3 Nanocube Film</title><source>American Chemical Society Journals</source><creator>Zhang, Nana ; Cui, Mengqi ; Zhou, Junxin ; Shao, Zhitao ; Gao, Xinyu ; Liu, Jiaming ; Sun, Ruyu ; Zhang, Yuan ; Li, Wenhui ; Li, Xinghan ; Yao, Jing ; Gao, Feng ; Feng, Wei</creator><creatorcontrib>Zhang, Nana ; Cui, Mengqi ; Zhou, Junxin ; Shao, Zhitao ; Gao, Xinyu ; Liu, Jiaming ; Sun, Ruyu ; Zhang, Yuan ; Li, Wenhui ; Li, Xinghan ; Yao, Jing ; Gao, Feng ; Feng, Wei</creatorcontrib><description>Ultraviolet photodetectors (UV PDs) have attracted significant attention due to their wide range of applications, such as underwater communication, biological analysis, and early fire warning systems. Indium oxide (In
O
) is a candidate for developing high-performance photoelectrochemical (PEC)-type UV PDs owing to its high UV absorption and good stability. However, the self-powered photoresponse of the previously reported In
O
-based PEC UV PDs is unsatisfactory. In this work, high-performance self-powered PEC UV PDs were constructed by using an In
O
nanocube film (NCF) as a photoanode. In
O
NCF photoanodes were synthesized on FTO by using hydrothermal methods with a calcining process. The influence of the electrolyte concentration, bias potential, and irradiation light on the photoresponse properties was systematically studied. In
O
NCF PEC UV PDs exhibit outstanding self-powered photoresponses to 365 nm UV light with a high responsivity of 44.43 mA/W and fast response speed (20/30 ms) under zero bias potential, these results are superior to those of previously reported In
O
-based PEC UV PDs. The improved self-powered photoresponse is attributed to the higher photogenerated carrier separation efficiency and faster charge transport of the in-situ grown In
O
NCF. In addition, these PDs exhibit excellent multicycle stability, maintaining the photocurrent at 98.69% of the initial value after 700 optical switching cycles. Therefore, our results prove the great promise of In
O
in self-powered PEC UV PDs.</description><identifier>ISSN: 1944-8244</identifier><identifier>EISSN: 1944-8252</identifier><identifier>DOI: 10.1021/acsami.4c00801</identifier><identifier>PMID: 38569197</identifier><language>eng</language><publisher>United States</publisher><ispartof>ACS applied materials & interfaces, 2024-04, Vol.16 (15), p.19167-19174</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c1077-c3b1429289a3ccedb4eb41705514ac5280af728f0c2013f48807c9bbc69d3a6e3</citedby><cites>FETCH-LOGICAL-c1077-c3b1429289a3ccedb4eb41705514ac5280af728f0c2013f48807c9bbc69d3a6e3</cites><orcidid>0000-0001-6902-0024</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,2765,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38569197$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhang, Nana</creatorcontrib><creatorcontrib>Cui, Mengqi</creatorcontrib><creatorcontrib>Zhou, Junxin</creatorcontrib><creatorcontrib>Shao, Zhitao</creatorcontrib><creatorcontrib>Gao, Xinyu</creatorcontrib><creatorcontrib>Liu, Jiaming</creatorcontrib><creatorcontrib>Sun, Ruyu</creatorcontrib><creatorcontrib>Zhang, Yuan</creatorcontrib><creatorcontrib>Li, Wenhui</creatorcontrib><creatorcontrib>Li, Xinghan</creatorcontrib><creatorcontrib>Yao, Jing</creatorcontrib><creatorcontrib>Gao, Feng</creatorcontrib><creatorcontrib>Feng, Wei</creatorcontrib><title>High-Performance Self-Powered Photoelectrochemical Ultraviolet Photodetectors Based on an In 2 O 3 Nanocube Film</title><title>ACS applied materials & interfaces</title><addtitle>ACS Appl Mater Interfaces</addtitle><description>Ultraviolet photodetectors (UV PDs) have attracted significant attention due to their wide range of applications, such as underwater communication, biological analysis, and early fire warning systems. Indium oxide (In
O
) is a candidate for developing high-performance photoelectrochemical (PEC)-type UV PDs owing to its high UV absorption and good stability. However, the self-powered photoresponse of the previously reported In
O
-based PEC UV PDs is unsatisfactory. In this work, high-performance self-powered PEC UV PDs were constructed by using an In
O
nanocube film (NCF) as a photoanode. In
O
NCF photoanodes were synthesized on FTO by using hydrothermal methods with a calcining process. The influence of the electrolyte concentration, bias potential, and irradiation light on the photoresponse properties was systematically studied. In
O
NCF PEC UV PDs exhibit outstanding self-powered photoresponses to 365 nm UV light with a high responsivity of 44.43 mA/W and fast response speed (20/30 ms) under zero bias potential, these results are superior to those of previously reported In
O
-based PEC UV PDs. The improved self-powered photoresponse is attributed to the higher photogenerated carrier separation efficiency and faster charge transport of the in-situ grown In
O
NCF. In addition, these PDs exhibit excellent multicycle stability, maintaining the photocurrent at 98.69% of the initial value after 700 optical switching cycles. Therefore, our results prove the great promise of In
O
in self-powered PEC UV PDs.</description><issn>1944-8244</issn><issn>1944-8252</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNo9kE9PwkAQRzdGI4hePZr9AsXZP223RyUiJkRIlHOznU6lpu2S3aLx24spcpo5vPc7PMZuBUwFSHFvMdi2nmoEMCDO2FhkWkdGxvL89Gs9YlchfAIkSkJ8yUbKxEkmsnTMdov6YxutyVfOt7ZD4m_UVNHafZOnkq-3rnfUEPbe4ZbaGm3DN03v7VftGuoHoKT-QDgf-KMNB8t13Hb8peOSr7jir7ZzuC-Iz-umvWYXlW0C3RzvhG3mT--zRbRcPb_MHpYRCkjTCFUhtMykyaxCpLLQVGiRQhwLbTGWBmyVSlMBShCq0sZAillRYJKVyiakJmw67KJ3IXiq8p2vW-t_cgH5X7p8SJcf0x2Eu0HY7YuWyhP-30r9Ajhha7s</recordid><startdate>20240417</startdate><enddate>20240417</enddate><creator>Zhang, Nana</creator><creator>Cui, Mengqi</creator><creator>Zhou, Junxin</creator><creator>Shao, Zhitao</creator><creator>Gao, Xinyu</creator><creator>Liu, Jiaming</creator><creator>Sun, Ruyu</creator><creator>Zhang, Yuan</creator><creator>Li, Wenhui</creator><creator>Li, Xinghan</creator><creator>Yao, Jing</creator><creator>Gao, Feng</creator><creator>Feng, Wei</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-6902-0024</orcidid></search><sort><creationdate>20240417</creationdate><title>High-Performance Self-Powered Photoelectrochemical Ultraviolet Photodetectors Based on an In 2 O 3 Nanocube Film</title><author>Zhang, Nana ; Cui, Mengqi ; Zhou, Junxin ; Shao, Zhitao ; Gao, Xinyu ; Liu, Jiaming ; Sun, Ruyu ; Zhang, Yuan ; Li, Wenhui ; Li, Xinghan ; Yao, Jing ; Gao, Feng ; Feng, Wei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c1077-c3b1429289a3ccedb4eb41705514ac5280af728f0c2013f48807c9bbc69d3a6e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Nana</creatorcontrib><creatorcontrib>Cui, Mengqi</creatorcontrib><creatorcontrib>Zhou, Junxin</creatorcontrib><creatorcontrib>Shao, Zhitao</creatorcontrib><creatorcontrib>Gao, Xinyu</creatorcontrib><creatorcontrib>Liu, Jiaming</creatorcontrib><creatorcontrib>Sun, Ruyu</creatorcontrib><creatorcontrib>Zhang, Yuan</creatorcontrib><creatorcontrib>Li, Wenhui</creatorcontrib><creatorcontrib>Li, Xinghan</creatorcontrib><creatorcontrib>Yao, Jing</creatorcontrib><creatorcontrib>Gao, Feng</creatorcontrib><creatorcontrib>Feng, Wei</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><jtitle>ACS applied materials & interfaces</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Nana</au><au>Cui, Mengqi</au><au>Zhou, Junxin</au><au>Shao, Zhitao</au><au>Gao, Xinyu</au><au>Liu, Jiaming</au><au>Sun, Ruyu</au><au>Zhang, Yuan</au><au>Li, Wenhui</au><au>Li, Xinghan</au><au>Yao, Jing</au><au>Gao, Feng</au><au>Feng, Wei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>High-Performance Self-Powered Photoelectrochemical Ultraviolet Photodetectors Based on an In 2 O 3 Nanocube Film</atitle><jtitle>ACS applied materials & interfaces</jtitle><addtitle>ACS Appl Mater Interfaces</addtitle><date>2024-04-17</date><risdate>2024</risdate><volume>16</volume><issue>15</issue><spage>19167</spage><epage>19174</epage><pages>19167-19174</pages><issn>1944-8244</issn><eissn>1944-8252</eissn><abstract>Ultraviolet photodetectors (UV PDs) have attracted significant attention due to their wide range of applications, such as underwater communication, biological analysis, and early fire warning systems. Indium oxide (In
O
) is a candidate for developing high-performance photoelectrochemical (PEC)-type UV PDs owing to its high UV absorption and good stability. However, the self-powered photoresponse of the previously reported In
O
-based PEC UV PDs is unsatisfactory. In this work, high-performance self-powered PEC UV PDs were constructed by using an In
O
nanocube film (NCF) as a photoanode. In
O
NCF photoanodes were synthesized on FTO by using hydrothermal methods with a calcining process. The influence of the electrolyte concentration, bias potential, and irradiation light on the photoresponse properties was systematically studied. In
O
NCF PEC UV PDs exhibit outstanding self-powered photoresponses to 365 nm UV light with a high responsivity of 44.43 mA/W and fast response speed (20/30 ms) under zero bias potential, these results are superior to those of previously reported In
O
-based PEC UV PDs. The improved self-powered photoresponse is attributed to the higher photogenerated carrier separation efficiency and faster charge transport of the in-situ grown In
O
NCF. In addition, these PDs exhibit excellent multicycle stability, maintaining the photocurrent at 98.69% of the initial value after 700 optical switching cycles. Therefore, our results prove the great promise of In
O
in self-powered PEC UV PDs.</abstract><cop>United States</cop><pmid>38569197</pmid><doi>10.1021/acsami.4c00801</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0001-6902-0024</orcidid></addata></record> |
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title | High-Performance Self-Powered Photoelectrochemical Ultraviolet Photodetectors Based on an In 2 O 3 Nanocube Film |
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