Scale-Up of a Rotating Packed Bed Reactor with a Mesh-Pin Rotor: (II) Mass Transfer and Application
A systematic scale-up study on a rotating packed bed (RPB) reactor is essential before the industrial application. However, the mass transfer and application performance of the RPB reactor with a scale-up mesh-pin rotor (MPR) are still unclear. In this work, the mass transfer, including effective in...
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Veröffentlicht in: | Industrial & engineering chemistry research 2020-03, Vol.59 (11), p.5124-5132 |
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description | A systematic scale-up study on a rotating packed bed (RPB) reactor is essential before the industrial application. However, the mass transfer and application performance of the RPB reactor with a scale-up mesh-pin rotor (MPR) are still unclear. In this work, the mass transfer, including effective interfacial area (a e) and liquid-side volume mass transfer coefficient (k L a e), of the RPB reactor with scale-up MPR was investigated. An amendatory k L a e model for the scale-up MPR was established based on hydrodynamic studies. The calculation results from the amended model were validated by experimental data under deviations of ±20%. Taking H2S removal as an application case, the removal efficiency by scale-up MPR was not lower than 96.98%. No obvious scale-up effect was observed in the RPB reactor with two different-sized MPRs, which can be regarded as a scale-up strategy for this kind of RPB reactor. |
doi_str_mv | 10.1021/acs.iecr.9b06684 |
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However, the mass transfer and application performance of the RPB reactor with a scale-up mesh-pin rotor (MPR) are still unclear. In this work, the mass transfer, including effective interfacial area (a e) and liquid-side volume mass transfer coefficient (k L a e), of the RPB reactor with scale-up MPR was investigated. An amendatory k L a e model for the scale-up MPR was established based on hydrodynamic studies. The calculation results from the amended model were validated by experimental data under deviations of ±20%. Taking H2S removal as an application case, the removal efficiency by scale-up MPR was not lower than 96.98%. No obvious scale-up effect was observed in the RPB reactor with two different-sized MPRs, which can be regarded as a scale-up strategy for this kind of RPB reactor.</description><identifier>ISSN: 0888-5885</identifier><identifier>EISSN: 1520-5045</identifier><identifier>DOI: 10.1021/acs.iecr.9b06684</identifier><language>eng</language><publisher>American Chemical Society</publisher><ispartof>Industrial & engineering chemistry research, 2020-03, Vol.59 (11), p.5124-5132</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a280t-6b71096b64c7356f70e3eb11e660d946dc264bc26675c0741ccfb197a98bfc8b3</citedby><cites>FETCH-LOGICAL-a280t-6b71096b64c7356f70e3eb11e660d946dc264bc26675c0741ccfb197a98bfc8b3</cites><orcidid>0000-0001-8300-5277 ; 0000-0002-3047-7024</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acs.iecr.9b06684$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acs.iecr.9b06684$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,2765,27076,27924,27925,56738,56788</link.rule.ids></links><search><creatorcontrib>Liu, Wei</creatorcontrib><creatorcontrib>Luo, Yong</creatorcontrib><creatorcontrib>Li, Yan-Bin</creatorcontrib><creatorcontrib>Chu, Guang-Wen</creatorcontrib><title>Scale-Up of a Rotating Packed Bed Reactor with a Mesh-Pin Rotor: (II) Mass Transfer and Application</title><title>Industrial & engineering chemistry research</title><addtitle>Ind. Eng. Chem. Res</addtitle><description>A systematic scale-up study on a rotating packed bed (RPB) reactor is essential before the industrial application. However, the mass transfer and application performance of the RPB reactor with a scale-up mesh-pin rotor (MPR) are still unclear. In this work, the mass transfer, including effective interfacial area (a e) and liquid-side volume mass transfer coefficient (k L a e), of the RPB reactor with scale-up MPR was investigated. An amendatory k L a e model for the scale-up MPR was established based on hydrodynamic studies. The calculation results from the amended model were validated by experimental data under deviations of ±20%. Taking H2S removal as an application case, the removal efficiency by scale-up MPR was not lower than 96.98%. No obvious scale-up effect was observed in the RPB reactor with two different-sized MPRs, which can be regarded as a scale-up strategy for this kind of RPB reactor.</description><issn>0888-5885</issn><issn>1520-5045</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp1kL1PwzAQxS0EEqWwM3oECZdzajsOW6n4qNSKqrRzZDs2TSlxZAch_nsctSvD3Q333tPTD6FrCiMKGb1XJo5qa8Ko0CCEZCdoQHkGhAPjp2gAUkrCpeTn6CLGHQBwztgAmXej9pZsWuwdVnjlO9XVzQdeKvNpK_yYZmWV6XzAP3W3TZKFjVuyrJte68MDvpnNbvFCxYjXQTXR2YBVU-FJ2-5rk8J8c4nOnNpHe3W8Q7R5flpPX8n87WU2ncyJyiR0ROicQiG0YCYfc-FysGOrKbVCQFUwUZlMMJ2WyLmBnFFjnKZFrgqpnZF6PERwyDXBxxisK9tQf6nwW1Ioe0hlglT2kMojpGS5O1j6z85_hyYV_F_-B_lFab8</recordid><startdate>20200318</startdate><enddate>20200318</enddate><creator>Liu, Wei</creator><creator>Luo, Yong</creator><creator>Li, Yan-Bin</creator><creator>Chu, Guang-Wen</creator><general>American Chemical Society</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-8300-5277</orcidid><orcidid>https://orcid.org/0000-0002-3047-7024</orcidid></search><sort><creationdate>20200318</creationdate><title>Scale-Up of a Rotating Packed Bed Reactor with a Mesh-Pin Rotor: (II) Mass Transfer and Application</title><author>Liu, Wei ; Luo, Yong ; Li, Yan-Bin ; Chu, Guang-Wen</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a280t-6b71096b64c7356f70e3eb11e660d946dc264bc26675c0741ccfb197a98bfc8b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Liu, Wei</creatorcontrib><creatorcontrib>Luo, Yong</creatorcontrib><creatorcontrib>Li, Yan-Bin</creatorcontrib><creatorcontrib>Chu, Guang-Wen</creatorcontrib><collection>CrossRef</collection><jtitle>Industrial & engineering chemistry research</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, Wei</au><au>Luo, Yong</au><au>Li, Yan-Bin</au><au>Chu, Guang-Wen</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Scale-Up of a Rotating Packed Bed Reactor with a Mesh-Pin Rotor: (II) Mass Transfer and Application</atitle><jtitle>Industrial & engineering chemistry research</jtitle><addtitle>Ind. Eng. Chem. Res</addtitle><date>2020-03-18</date><risdate>2020</risdate><volume>59</volume><issue>11</issue><spage>5124</spage><epage>5132</epage><pages>5124-5132</pages><issn>0888-5885</issn><eissn>1520-5045</eissn><abstract>A systematic scale-up study on a rotating packed bed (RPB) reactor is essential before the industrial application. However, the mass transfer and application performance of the RPB reactor with a scale-up mesh-pin rotor (MPR) are still unclear. In this work, the mass transfer, including effective interfacial area (a e) and liquid-side volume mass transfer coefficient (k L a e), of the RPB reactor with scale-up MPR was investigated. An amendatory k L a e model for the scale-up MPR was established based on hydrodynamic studies. The calculation results from the amended model were validated by experimental data under deviations of ±20%. Taking H2S removal as an application case, the removal efficiency by scale-up MPR was not lower than 96.98%. No obvious scale-up effect was observed in the RPB reactor with two different-sized MPRs, which can be regarded as a scale-up strategy for this kind of RPB reactor.</abstract><pub>American Chemical Society</pub><doi>10.1021/acs.iecr.9b06684</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0001-8300-5277</orcidid><orcidid>https://orcid.org/0000-0002-3047-7024</orcidid></addata></record> |
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title | Scale-Up of a Rotating Packed Bed Reactor with a Mesh-Pin Rotor: (II) Mass Transfer and Application |
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