Evolution of Condensable Fine Particle Size Distribution in Simulated Flue Gas by External Regulation for Growth Enhancement

Condensation fine particles (CFPs) from coal-fired flue gas harm humans and the environment after being emitted into the atmosphere. Given their small size (1 was significantly broadened due to joint action of multiple mechanisms. Fly ash acted as the core, and CFPs adhered to the ash surface when f...

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Veröffentlicht in:Environmental science & technology 2020-04, Vol.54 (7), p.3840-3848
Hauptverfasser: Zheng, Chenghang, Zheng, Hao, Shen, Jiali, Gao, Wenchao, Yang, Zhengda, Zhao, Zhongyang, Wang, Yifan, Zhang, Hao, Gao, Xiang
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Sprache:eng
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Zusammenfassung:Condensation fine particles (CFPs) from coal-fired flue gas harm humans and the environment after being emitted into the atmosphere. Given their small size (1 was significantly broadened due to joint action of multiple mechanisms. Fly ash acted as the core, and CFPs adhered to the ash surface when forming ash–salt droplets. Cooling flue gas could also enhance the CFP growth due to vapor condensation. At decreased temperature from 45 to 30 °C, the median diameter of CFPs increased by 15%. Finally, the growth and agglomeration of CFPs can be further enhanced when an external electrical field was utilized. The size range of growth factor >1 can be broadened, and the peak growth factor significantly increased at 8 kV applied voltage. The research findings provide valuable guidance for effectively improving the CFP removal efficiency by external regulation for growth enhancement.
ISSN:0013-936X
1520-5851
DOI:10.1021/acs.est.9b06569