Strain engineering of magnetocaloric effect in W/Gd/W/MgO structures
[Display omitted] •Mechanical strain at interface affects magnetocaloric effect in Gd films.•Magnetic entropy and RCP depend on substrate orientation.•Increase in internal mechanical strain causes increase in RCP.•Maximal magnetocaloric effect appears at (111) orientation of MgO substrate.•Metastabl...
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Veröffentlicht in: | Journal of magnetism and magnetic materials 2022-12, Vol.564, p.170164, Article 170164 |
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Sprache: | eng |
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•Mechanical strain at interface affects magnetocaloric effect in Gd films.•Magnetic entropy and RCP depend on substrate orientation.•Increase in internal mechanical strain causes increase in RCP.•Maximal magnetocaloric effect appears at (111) orientation of MgO substrate.•Metastable fcc phase is present in the films.
Strain controlled magnetocaloric effect (MCE) accompanying a transition between ferromagnetic and paramagnetic phases has been revealed in multilayered W/Gd/W/MgO structures at Tc = 293 K. Mechanical stresses at the Gd/W interface controlled by internal stresses at the MgO substrate and depending on its crystallographic orientation, strongly affect magnetic part of entropy ΔSM and relative cooling power (RCP). Increase in thickness of Gd films from 100 nm up to 300 nm approaches the ΔSM and RCP values to those known for the bulk Gd samples. We found that higher internal stresses widen the temperature range in which a ferromagnet-paramagnet transition occurs. Since Gd based alloys are very perspective for magnetic refrigeration, obtained data can be used to predict how local internal stresses in the vicinity of structural defects (dislocations, twins etc) can affect MCE even in bulk Gd samples. |
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ISSN: | 0304-8853 |
DOI: | 10.1016/j.jmmm.2022.170164 |