Perovskites as Catalysts for the Selective Catalytic Reduction of Nitric Oxide with Propene: Relationship between Solid State Properties and Catalytic Activity
The influence of the solid state properties of manganese- and iron-based perovskites on the activity for the selective catalytic reduction of nitric oxide with propene under oxidizing conditions has been investigated. By substituting manganese for iron in the solid solution series La0.6Sr0.4Fe1−yMny...
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| Veröffentlicht in: | Journal of catalysis 2001-04, Vol.199 (1), p.132-140 |
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| container_title | Journal of catalysis |
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| creator | Hansen, K.Kammer Skou, E.M Christensen, H Turek, T |
| description | The influence of the solid state properties of manganese- and iron-based perovskites on the activity for the selective catalytic reduction of nitric oxide with propene under oxidizing conditions has been investigated. By substituting manganese for iron in the solid solution series La0.6Sr0.4Fe1−yMnyO3±δ (0 ≤ y ≤ 1) and by substituting strontium for lanthanum in the solid solution series La1−xSrxMnO3+δ(0.05 ≤ x ≤ 0.50) it is shown that the catalytic activity of the perovskites depends mainly on the redox properties of the transition metal and on the number of oxygen vacancies. |
| doi_str_mv | 10.1006/jcat.2000.3153 |
| format | Article |
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By substituting manganese for iron in the solid solution series La0.6Sr0.4Fe1−yMnyO3±δ (0 ≤ y ≤ 1) and by substituting strontium for lanthanum in the solid solution series La1−xSrxMnO3+δ(0.05 ≤ x ≤ 0.50) it is shown that the catalytic activity of the perovskites depends mainly on the redox properties of the transition metal and on the number of oxygen vacancies.</description><identifier>ISSN: 0021-9517</identifier><identifier>EISSN: 1090-2694</identifier><identifier>DOI: 10.1006/jcat.2000.3153</identifier><identifier>CODEN: JCTLA5</identifier><language>eng</language><publisher>Amsterdam: Elsevier Inc</publisher><subject>Catalysis ; Catalytic reactions ; Chemistry ; Exact sciences and technology ; General and physical chemistry ; iron ; manganese ; nitric oxide ; perovskite ; propene ; Theory of reactions, general kinetics. Catalysis. 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By substituting manganese for iron in the solid solution series La0.6Sr0.4Fe1−yMnyO3±δ (0 ≤ y ≤ 1) and by substituting strontium for lanthanum in the solid solution series La1−xSrxMnO3+δ(0.05 ≤ x ≤ 0.50) it is shown that the catalytic activity of the perovskites depends mainly on the redox properties of the transition metal and on the number of oxygen vacancies.</description><subject>Catalysis</subject><subject>Catalytic reactions</subject><subject>Chemistry</subject><subject>Exact sciences and technology</subject><subject>General and physical chemistry</subject><subject>iron</subject><subject>manganese</subject><subject>nitric oxide</subject><subject>perovskite</subject><subject>propene</subject><subject>Theory of reactions, general kinetics. Catalysis. 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Nomenclature, chemical documentation, computer chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Hansen, K.Kammer</creatorcontrib><creatorcontrib>Skou, E.M</creatorcontrib><creatorcontrib>Christensen, H</creatorcontrib><creatorcontrib>Turek, T</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><jtitle>Journal of catalysis</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Hansen, K.Kammer</au><au>Skou, E.M</au><au>Christensen, H</au><au>Turek, T</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Perovskites as Catalysts for the Selective Catalytic Reduction of Nitric Oxide with Propene: Relationship between Solid State Properties and Catalytic Activity</atitle><jtitle>Journal of catalysis</jtitle><date>2001-04-01</date><risdate>2001</risdate><volume>199</volume><issue>1</issue><spage>132</spage><epage>140</epage><pages>132-140</pages><issn>0021-9517</issn><eissn>1090-2694</eissn><coden>JCTLA5</coden><abstract>The influence of the solid state properties of manganese- and iron-based perovskites on the activity for the selective catalytic reduction of nitric oxide with propene under oxidizing conditions has been investigated. By substituting manganese for iron in the solid solution series La0.6Sr0.4Fe1−yMnyO3±δ (0 ≤ y ≤ 1) and by substituting strontium for lanthanum in the solid solution series La1−xSrxMnO3+δ(0.05 ≤ x ≤ 0.50) it is shown that the catalytic activity of the perovskites depends mainly on the redox properties of the transition metal and on the number of oxygen vacancies.</abstract><cop>Amsterdam</cop><pub>Elsevier Inc</pub><doi>10.1006/jcat.2000.3153</doi><tpages>9</tpages></addata></record> |
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| subjects | Catalysis Catalytic reactions Chemistry Exact sciences and technology General and physical chemistry iron manganese nitric oxide perovskite propene Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry |
| title | Perovskites as Catalysts for the Selective Catalytic Reduction of Nitric Oxide with Propene: Relationship between Solid State Properties and Catalytic Activity |
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