Dynamic and LHHW Kinetic Analysis of Heterogeneous Catalytic Hydroformylation

Heterogeneous ethylene hydroformylation on a 4 wt% Rh/SiO 2 catalyst was studied using a steady-state pulse transient method coupled with in situ infrared spectroscopy. Four independent quantities, including the rates of propionaldehyde and ethane formation and the surface coverages of adsorbed CO a...

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Veröffentlicht in:	Journal of Catalysis 1995-02, Vol.151 (2), p.266-278
Hauptverfasser:	Balakos, M.W., Chuang, S.S.C.
Format:	Artikel
Sprache:	eng
Schlagworte:	10 SYNTHETIC FUELS 40 CHEMISTRY ABSORPTION SPECTROSCOPY ALDEHYDES CARBON 13 CARBON MONOXIDE CARBONYLATION Catalysis CATALYSTS CATALYTIC EFFECTS Catalytic reactions CHEMICAL REACTION KINETICS Chemistry ETHANE ETHYLENE Exact sciences and technology General and physical chemistry HETEROGENEOUS CATALYSIS ISOTHERMS LABELLED COMPOUNDS MATHEMATICAL MODELS REACTION INTERMEDIATES RHODIUM SILICA Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
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