Spectroscopy and Laser Action of Anisotropic Single-Centered LiKYF5: Nd3+ Crystals Grown by the Hydrothermal Method

Spectroscopy and Laser Action of Anisotropic Single-Centered LiKYF5: Nd3+ Crystals Grown by the Hydrothermal Method

Spectroscopic investigations are made on new laser monoclinic single‐centered LiKYF5: Nd3+ crystals grown by the hydrothermal method. Stark levels of its activator ions for 37 2s+1 LJ manifolds lying up to ≈ 40000 cm−1 are established from luminescence and absorption spectra at 7 K. Using a new set...

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Veröffentlicht in:Physica status solidi. A, Applied research Applied research, 1994-09, Vol.145 (1), p.177-195
Hauptverfasser: Kaminskii, A. A., Mironov, V. S., Bagaev, S. N., Khaidukov, N. M., Joubert, M. F., Jacquier, B., Boulon, G.
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container_title Physica status solidi. A, Applied research
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creator Kaminskii, A. A.
Mironov, V. S.
Bagaev, S. N.
Khaidukov, N. M.
Joubert, M. F.
Jacquier, B.
Boulon, G.
description Spectroscopic investigations are made on new laser monoclinic single‐centered LiKYF5: Nd3+ crystals grown by the hydrothermal method. Stark levels of its activator ions for 37 2s+1 LJ manifolds lying up to ≈ 40000 cm−1 are established from luminescence and absorption spectra at 7 K. Using a new set of reduced‐matrix elements for electric‐dipole 4f3−4f3 transitions the intensity characteristics for LiKYF5: Nd3+ are calculated including phenomenological Judd‐Ofelt parmaeters Ω1, intermanifold absorption line strengths, as well as the radiative lifetime of the initial laser state 4F3/2 and branching ratios originated for its IR emitting channels. The kinetics of luminescence from four metastable states 2F(2)5/2, 4D3/2, 2P3/2, and 4F3/2 as function of Nd3+‐ion concentration and temperature are measured. Room‐temperture pulse, cw, and quasi‐cw stimulated emission of Nd3+ ions at two generating 4F3/2 → 4I11/2 and 4F3/2 → 4I13/2 channels under Xe‐flashlamp and laser‐diode pumpings are obtained. All observed induced inter‐Stark transitions are identified.
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title Spectroscopy and Laser Action of Anisotropic Single-Centered LiKYF5: Nd3+ Crystals Grown by the Hydrothermal Method
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