Hubbard Gap Closure‐Induced Dual‐Redox Li‐Storage Mechanism as the Origin of Anomalously High Capacity and Fast Ion Diffusivity in MOFs‐Like Polyoxometalates

MOFs‐like polyoxometalate (POMs) electrodes, harvesting combined advantages of interlocking porosity and multi‐electron transfer reaction, have already emerged as promising candidates for lithium‐ion batteries (LIBs), yet the origins of the underlying redox mechanism in such materials remain a matte...

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