Nanopore/Nanosphere‐Induced Optical Enhancement of Monolayer MoS 2
Heterostructured transition metal dichalcogenides (TMDs) have received much attention due to their tunable optical and electronic properties. Here, a strategy for facile fabrication of porous anodic alumina (PAA) membrane‐supported monolayer molybdenum disulfide (MoS 2 ) is described. PAA is either...
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Veröffentlicht in: | Advanced optical materials 2023-08, Vol.11 (16) |
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container_title | Advanced optical materials |
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creator | Li, Yueqi Chen, Zhexue Zhou, Xuanping Wu, Xianxin Zhou, Zhican Li, Zhangqiang Xiao, Liuyang Liu, Qian Liu, Xinfeng Zhang, Yong |
description | Heterostructured transition metal dichalcogenides (TMDs) have received much attention due to their tunable optical and electronic properties. Here, a strategy for facile fabrication of porous anodic alumina (PAA) membrane‐supported monolayer molybdenum disulfide (MoS
2
) is described. PAA is either empty or filled with gold nanoparticles (AuNPs). Such nanopore/nanosphere‐supported MoS
2
(i.e., PAA‐MoS
2
and PAA‐Au‐MoS
2
) exhibits greatly enhanced optical performances compared with those of silicon wafer‐supported MoS
2
(i.e., Si/SiO
2
‐MoS
2
). Notably, 11‐fold Raman enhancement, 13‐fold photoluminescence enhancement, and 419‐fold second‐harmonic generation enhancement are achieved in PAA‐Au‐MoS
2
. Moreover, the optical enhancement mechanism of this unique structure is proposed. This work provides a platform for the construction of curved/heterostructured TMDs and exploration of their strong light‐matter interactions. |
doi_str_mv | 10.1002/adom.202300120 |
format | Article |
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2
) is described. PAA is either empty or filled with gold nanoparticles (AuNPs). Such nanopore/nanosphere‐supported MoS
2
(i.e., PAA‐MoS
2
and PAA‐Au‐MoS
2
) exhibits greatly enhanced optical performances compared with those of silicon wafer‐supported MoS
2
(i.e., Si/SiO
2
‐MoS
2
). Notably, 11‐fold Raman enhancement, 13‐fold photoluminescence enhancement, and 419‐fold second‐harmonic generation enhancement are achieved in PAA‐Au‐MoS
2
. Moreover, the optical enhancement mechanism of this unique structure is proposed. This work provides a platform for the construction of curved/heterostructured TMDs and exploration of their strong light‐matter interactions.</description><identifier>ISSN: 2195-1071</identifier><identifier>EISSN: 2195-1071</identifier><identifier>DOI: 10.1002/adom.202300120</identifier><language>eng</language><ispartof>Advanced optical materials, 2023-08, Vol.11 (16)</ispartof><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c840-7304499f21eadb7ee526017a3f64200f07aeb2d8813050cb11cc353d4817e1033</citedby><cites>FETCH-LOGICAL-c840-7304499f21eadb7ee526017a3f64200f07aeb2d8813050cb11cc353d4817e1033</cites><orcidid>0000-0002-5914-1065</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Li, Yueqi</creatorcontrib><creatorcontrib>Chen, Zhexue</creatorcontrib><creatorcontrib>Zhou, Xuanping</creatorcontrib><creatorcontrib>Wu, Xianxin</creatorcontrib><creatorcontrib>Zhou, Zhican</creatorcontrib><creatorcontrib>Li, Zhangqiang</creatorcontrib><creatorcontrib>Xiao, Liuyang</creatorcontrib><creatorcontrib>Liu, Qian</creatorcontrib><creatorcontrib>Liu, Xinfeng</creatorcontrib><creatorcontrib>Zhang, Yong</creatorcontrib><title>Nanopore/Nanosphere‐Induced Optical Enhancement of Monolayer MoS 2</title><title>Advanced optical materials</title><description>Heterostructured transition metal dichalcogenides (TMDs) have received much attention due to their tunable optical and electronic properties. Here, a strategy for facile fabrication of porous anodic alumina (PAA) membrane‐supported monolayer molybdenum disulfide (MoS
2
) is described. PAA is either empty or filled with gold nanoparticles (AuNPs). Such nanopore/nanosphere‐supported MoS
2
(i.e., PAA‐MoS
2
and PAA‐Au‐MoS
2
) exhibits greatly enhanced optical performances compared with those of silicon wafer‐supported MoS
2
(i.e., Si/SiO
2
‐MoS
2
). Notably, 11‐fold Raman enhancement, 13‐fold photoluminescence enhancement, and 419‐fold second‐harmonic generation enhancement are achieved in PAA‐Au‐MoS
2
. Moreover, the optical enhancement mechanism of this unique structure is proposed. This work provides a platform for the construction of curved/heterostructured TMDs and exploration of their strong light‐matter interactions.</description><issn>2195-1071</issn><issn>2195-1071</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpNkLFOwzAURS0EElXpypwfSPqe7dTJiEqBSoUOdI8c-1ktSuzILkM3PoFv5EtoBEJM9wxXZziM3SIUCMDn2oa-4MAFAHK4YBOOdZkjKLz8x9dsltIbnD-gRC3VhN2_aB-GEGk-Qhr2FOnr43Pt7bshm22H48HoLlv5vfaGevLHLLjsOfjQ6RPFM71m_IZdOd0lmv3ulO0eVrvlU77ZPq6Xd5vcVBJyJUDKunYcSdtWEZV8Aai0cAvJARwoTS23VYUCSjAtojGiFFZWqAhBiCkrfrQmhpQiuWaIh17HU4PQjBWasULzV0F8A05JT4g</recordid><startdate>202308</startdate><enddate>202308</enddate><creator>Li, Yueqi</creator><creator>Chen, Zhexue</creator><creator>Zhou, Xuanping</creator><creator>Wu, Xianxin</creator><creator>Zhou, Zhican</creator><creator>Li, Zhangqiang</creator><creator>Xiao, Liuyang</creator><creator>Liu, Qian</creator><creator>Liu, Xinfeng</creator><creator>Zhang, Yong</creator><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-5914-1065</orcidid></search><sort><creationdate>202308</creationdate><title>Nanopore/Nanosphere‐Induced Optical Enhancement of Monolayer MoS 2</title><author>Li, Yueqi ; Chen, Zhexue ; Zhou, Xuanping ; Wu, Xianxin ; Zhou, Zhican ; Li, Zhangqiang ; Xiao, Liuyang ; Liu, Qian ; Liu, Xinfeng ; Zhang, Yong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c840-7304499f21eadb7ee526017a3f64200f07aeb2d8813050cb11cc353d4817e1033</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><toplevel>online_resources</toplevel><creatorcontrib>Li, Yueqi</creatorcontrib><creatorcontrib>Chen, Zhexue</creatorcontrib><creatorcontrib>Zhou, Xuanping</creatorcontrib><creatorcontrib>Wu, Xianxin</creatorcontrib><creatorcontrib>Zhou, Zhican</creatorcontrib><creatorcontrib>Li, Zhangqiang</creatorcontrib><creatorcontrib>Xiao, Liuyang</creatorcontrib><creatorcontrib>Liu, Qian</creatorcontrib><creatorcontrib>Liu, Xinfeng</creatorcontrib><creatorcontrib>Zhang, Yong</creatorcontrib><collection>CrossRef</collection><jtitle>Advanced optical materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Yueqi</au><au>Chen, Zhexue</au><au>Zhou, Xuanping</au><au>Wu, Xianxin</au><au>Zhou, Zhican</au><au>Li, Zhangqiang</au><au>Xiao, Liuyang</au><au>Liu, Qian</au><au>Liu, Xinfeng</au><au>Zhang, Yong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Nanopore/Nanosphere‐Induced Optical Enhancement of Monolayer MoS 2</atitle><jtitle>Advanced optical materials</jtitle><date>2023-08</date><risdate>2023</risdate><volume>11</volume><issue>16</issue><issn>2195-1071</issn><eissn>2195-1071</eissn><abstract>Heterostructured transition metal dichalcogenides (TMDs) have received much attention due to their tunable optical and electronic properties. Here, a strategy for facile fabrication of porous anodic alumina (PAA) membrane‐supported monolayer molybdenum disulfide (MoS
2
) is described. PAA is either empty or filled with gold nanoparticles (AuNPs). Such nanopore/nanosphere‐supported MoS
2
(i.e., PAA‐MoS
2
and PAA‐Au‐MoS
2
) exhibits greatly enhanced optical performances compared with those of silicon wafer‐supported MoS
2
(i.e., Si/SiO
2
‐MoS
2
). Notably, 11‐fold Raman enhancement, 13‐fold photoluminescence enhancement, and 419‐fold second‐harmonic generation enhancement are achieved in PAA‐Au‐MoS
2
. Moreover, the optical enhancement mechanism of this unique structure is proposed. This work provides a platform for the construction of curved/heterostructured TMDs and exploration of their strong light‐matter interactions.</abstract><doi>10.1002/adom.202300120</doi><orcidid>https://orcid.org/0000-0002-5914-1065</orcidid></addata></record> |
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title | Nanopore/Nanosphere‐Induced Optical Enhancement of Monolayer MoS 2 |
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