Hot Hydrocarbon‐Solvent Slot‐Die Coating Enables High‐Efficiency Organic Solar Cells with Temperature‐Dependent Aggregation Behavior
Organic solar cells (OSCs) have made rapid progress in terms of their development as a sustainable energy source. However, record‐breaking devices have not shown compatibility with large‐scale production via solution processing in particular due to the use of halogenated environment‐threatening solv...
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| Veröffentlicht in: | Advanced materials (Weinheim) 2020-10, Vol.32 (39), p.e2002302-n/a, Article 2002302 |
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| creator | Zhao, Heng Naveed, Hafiz Bilal Lin, Baojun Zhou, Xiaobo Yuan, Jian Zhou, Ke Wu, Hongbo Guo, Renjun Scheel, Manuel A. Chumakov, Andrei Roth, Stephan V. Tang, Zheng Müller‐Buschbaum, Peter Ma, Wei |
| description | Organic solar cells (OSCs) have made rapid progress in terms of their development as a sustainable energy source. However, record‐breaking devices have not shown compatibility with large‐scale production via solution processing in particular due to the use of halogenated environment‐threatening solvents. Here, slot‐die fabrication with processing involving hydrocarbon‐based solvents is used to realize highly efficient and environmentally friendly OSCs. Highly compatible slot‐die coating with roll‐to‐roll processing using halogenated (chlorobenzene (CB)) and hydrocarbon solvents (1,2,4‐trimethylbenzene (TMB) and ortho‐xylene (o‐XY)) is used to fabricate photoactive films. Controlled solution and substrate temperatures enable similar aggregation states in the solution and similar kinetics processes during film formation. The optimized blend film nanostructures for different solvents in the highly efficient PM6:Y6 blend is adopted to show a similar morphology, which results in device efficiencies of 15.2%, 15.4%, and 15.6% for CB, TMB, and o‐XY solvents. This approach is successfully extended to other donor–acceptor combinations to demonstrate the excellent universality of this method. The results combine a method to optimize the aggregation state and film formation kinetics with the fabrication of OSCs with environmentally friendly solvents by slot‐die coating, which is a critical finding for the future development of OSCs in terms of their scalable production and high‐performance.
Highly efficient temperature‐dependent‐aggregation polymer‐based organic solar cells are fabricated by hot slot‐die coating with hydrocarbon solvents. Power conversion efficiencies of 15.2%, 15.4%, and 15.6% are obtained when chlorobenzene, 1,2,4‐trimethylbenzene (TMB), and ortho‐xylene are used, respectively. |
| doi_str_mv | 10.1002/adma.202002302 |
| format | Article |
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Highly efficient temperature‐dependent‐aggregation polymer‐based organic solar cells are fabricated by hot slot‐die coating with hydrocarbon solvents. Power conversion efficiencies of 15.2%, 15.4%, and 15.6% are obtained when chlorobenzene, 1,2,4‐trimethylbenzene (TMB), and ortho‐xylene are used, respectively.</description><identifier>ISSN: 0935-9648</identifier><identifier>ISSN: 1521-4095</identifier><identifier>EISSN: 1521-4095</identifier><identifier>DOI: 10.1002/adma.202002302</identifier><identifier>PMID: 32812287</identifier><language>eng</language><publisher>WEINHEIM: Wiley</publisher><subject>4-trimethylbenzene ; Agglomeration ; Aggregation behavior ; Chemistry ; Chemistry, Multidisciplinary ; Chemistry, Physical ; Chlorobenzene ; Coating ; Coatings ; Dies ; Entertainment industry ; Environmentally friendly solvents ; Green manufacturing ; Halogenation ; hot slot-die coating ; Hydrocarbon refining ; hydrocarbon solvents ; Hydrocarbons ; Kinetics ; Large scale productions ; Materials Science ; Materials Science, Multidisciplinary ; Morphology ; Nanoscience & Nanotechnology ; organic solar cells ; Photovoltaic cells ; Physical Sciences ; Physics ; Physics, Applied ; Physics, Condensed Matter ; Roll-to-roll processing ; Science & Technology ; Science & Technology - Other Topics ; Slot dies ; Solar cells ; Solvents ; Substrate temperature ; Substrates ; Sustainable development ; Sustainable energy sources ; Technology ; Temperature dependence ; Temperature dependent ; temperature-dependent aggregation ; Trimethylbenzene ; Xylene</subject><ispartof>Advanced materials (Weinheim), 2020-10, Vol.32 (39), p.e2002302-n/a, Article 2002302</ispartof><rights>2020 Wiley‐VCH GmbH</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>157</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000560352000001</woscitedreferencesoriginalsourcerecordid><citedby>FETCH-LOGICAL-c4252-4420cd80552e4fd7698fe7381bc5a529622408807b58491ea23a26702c92844a3</citedby><cites>FETCH-LOGICAL-c4252-4420cd80552e4fd7698fe7381bc5a529622408807b58491ea23a26702c92844a3</cites><orcidid>0000-0002-7239-2010 ; 0000-0001-6323-8401 ; 0000-0003-0036-2362</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fadma.202002302$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fadma.202002302$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>230,315,782,786,887,1419,27931,27932,28255,45581,45582</link.rule.ids><backlink>$$Uhttps://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-286554$$DView record from Swedish Publication Index$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhao, Heng</creatorcontrib><creatorcontrib>Naveed, Hafiz Bilal</creatorcontrib><creatorcontrib>Lin, Baojun</creatorcontrib><creatorcontrib>Zhou, Xiaobo</creatorcontrib><creatorcontrib>Yuan, Jian</creatorcontrib><creatorcontrib>Zhou, Ke</creatorcontrib><creatorcontrib>Wu, Hongbo</creatorcontrib><creatorcontrib>Guo, Renjun</creatorcontrib><creatorcontrib>Scheel, Manuel A.</creatorcontrib><creatorcontrib>Chumakov, Andrei</creatorcontrib><creatorcontrib>Roth, Stephan V.</creatorcontrib><creatorcontrib>Tang, Zheng</creatorcontrib><creatorcontrib>Müller‐Buschbaum, Peter</creatorcontrib><creatorcontrib>Ma, Wei</creatorcontrib><title>Hot Hydrocarbon‐Solvent Slot‐Die Coating Enables High‐Efficiency Organic Solar Cells with Temperature‐Dependent Aggregation Behavior</title><title>Advanced materials (Weinheim)</title><addtitle>ADV MATER</addtitle><description>Organic solar cells (OSCs) have made rapid progress in terms of their development as a sustainable energy source. However, record‐breaking devices have not shown compatibility with large‐scale production via solution processing in particular due to the use of halogenated environment‐threatening solvents. Here, slot‐die fabrication with processing involving hydrocarbon‐based solvents is used to realize highly efficient and environmentally friendly OSCs. Highly compatible slot‐die coating with roll‐to‐roll processing using halogenated (chlorobenzene (CB)) and hydrocarbon solvents (1,2,4‐trimethylbenzene (TMB) and ortho‐xylene (o‐XY)) is used to fabricate photoactive films. Controlled solution and substrate temperatures enable similar aggregation states in the solution and similar kinetics processes during film formation. The optimized blend film nanostructures for different solvents in the highly efficient PM6:Y6 blend is adopted to show a similar morphology, which results in device efficiencies of 15.2%, 15.4%, and 15.6% for CB, TMB, and o‐XY solvents. This approach is successfully extended to other donor–acceptor combinations to demonstrate the excellent universality of this method. The results combine a method to optimize the aggregation state and film formation kinetics with the fabrication of OSCs with environmentally friendly solvents by slot‐die coating, which is a critical finding for the future development of OSCs in terms of their scalable production and high‐performance.
Highly efficient temperature‐dependent‐aggregation polymer‐based organic solar cells are fabricated by hot slot‐die coating with hydrocarbon solvents. Power conversion efficiencies of 15.2%, 15.4%, and 15.6% are obtained when chlorobenzene, 1,2,4‐trimethylbenzene (TMB), and ortho‐xylene are used, respectively.</description><subject>4-trimethylbenzene</subject><subject>Agglomeration</subject><subject>Aggregation behavior</subject><subject>Chemistry</subject><subject>Chemistry, Multidisciplinary</subject><subject>Chemistry, Physical</subject><subject>Chlorobenzene</subject><subject>Coating</subject><subject>Coatings</subject><subject>Dies</subject><subject>Entertainment industry</subject><subject>Environmentally friendly solvents</subject><subject>Green manufacturing</subject><subject>Halogenation</subject><subject>hot slot-die coating</subject><subject>Hydrocarbon refining</subject><subject>hydrocarbon solvents</subject><subject>Hydrocarbons</subject><subject>Kinetics</subject><subject>Large scale productions</subject><subject>Materials Science</subject><subject>Materials Science, Multidisciplinary</subject><subject>Morphology</subject><subject>Nanoscience & Nanotechnology</subject><subject>organic solar cells</subject><subject>Photovoltaic cells</subject><subject>Physical Sciences</subject><subject>Physics</subject><subject>Physics, Applied</subject><subject>Physics, Condensed Matter</subject><subject>Roll-to-roll processing</subject><subject>Science & Technology</subject><subject>Science & Technology - Other Topics</subject><subject>Slot dies</subject><subject>Solar cells</subject><subject>Solvents</subject><subject>Substrate temperature</subject><subject>Substrates</subject><subject>Sustainable development</subject><subject>Sustainable energy sources</subject><subject>Technology</subject><subject>Temperature dependence</subject><subject>Temperature dependent</subject><subject>temperature-dependent aggregation</subject><subject>Trimethylbenzene</subject><subject>Xylene</subject><issn>0935-9648</issn><issn>1521-4095</issn><issn>1521-4095</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>AOWDO</sourceid><recordid>eNqNkUFv0zAYhiMEYmVw5WyJCxJKcb7YiXMMaaFIQztscLWc9EvqkdrBTlb1xg_YYb-RX4K7TkXiAr7Ylp_31fv5jaLXCZ0nlMJ7td6qOVAI55TCk2iWcEhiRgv-NJrRIuVxkTFxFr3w_oZSWmQ0ex6dpSASAJHPoruVHclqv3a2Ua625tfP-yvb36IZyVVvx3BdaCSVVaM2HVkaVffoyUp3m_C0bFvdaDTNnly6ThndkCBWjlTY957s9Lgh17gd0KlxcngwwwHN-uBedp3DLthaQz7gRt1q615Gz1rVe3z1uJ9HXz8ur6tVfHH56XNVXsQNAw4xY0CbtaCcA7J2nWeFaDFPRVI3XHEoMgBGhaB5zQUrElSQKshyCk0BgjGVnkfx0dfvcJhqOTi9VW4vrdJyob-V0rpOfh83EkTGOQv82yM_OPtjQj_KrfZNmFEZtJOXwFLO04QKCOibv9AbOzkTpgkUy1lBOUsCNT9SjbPeO2xPERIqD73KQ6_y1GsQvDsKdljb1j98Op5EoVie0ZQHOqyDvfh_utLjQwuVncwYpMWjVPe4_0csWS6-lH9C_gaAa8jt</recordid><startdate>20201001</startdate><enddate>20201001</enddate><creator>Zhao, Heng</creator><creator>Naveed, Hafiz Bilal</creator><creator>Lin, Baojun</creator><creator>Zhou, Xiaobo</creator><creator>Yuan, Jian</creator><creator>Zhou, Ke</creator><creator>Wu, Hongbo</creator><creator>Guo, Renjun</creator><creator>Scheel, Manuel A.</creator><creator>Chumakov, Andrei</creator><creator>Roth, Stephan V.</creator><creator>Tang, Zheng</creator><creator>Müller‐Buschbaum, Peter</creator><creator>Ma, Wei</creator><general>Wiley</general><general>Wiley Subscription Services, Inc</general><scope>AOWDO</scope><scope>BLEPL</scope><scope>DTL</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>7X8</scope><scope>ADTPV</scope><scope>AOWAS</scope><scope>D8V</scope><orcidid>https://orcid.org/0000-0002-7239-2010</orcidid><orcidid>https://orcid.org/0000-0001-6323-8401</orcidid><orcidid>https://orcid.org/0000-0003-0036-2362</orcidid></search><sort><creationdate>20201001</creationdate><title>Hot Hydrocarbon‐Solvent Slot‐Die Coating Enables High‐Efficiency Organic Solar Cells with Temperature‐Dependent Aggregation Behavior</title><author>Zhao, Heng ; Naveed, Hafiz Bilal ; Lin, Baojun ; Zhou, Xiaobo ; Yuan, Jian ; Zhou, Ke ; Wu, Hongbo ; Guo, Renjun ; Scheel, Manuel A. ; Chumakov, Andrei ; Roth, Stephan V. ; Tang, Zheng ; Müller‐Buschbaum, Peter ; Ma, Wei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c4252-4420cd80552e4fd7698fe7381bc5a529622408807b58491ea23a26702c92844a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>4-trimethylbenzene</topic><topic>Agglomeration</topic><topic>Aggregation behavior</topic><topic>Chemistry</topic><topic>Chemistry, Multidisciplinary</topic><topic>Chemistry, Physical</topic><topic>Chlorobenzene</topic><topic>Coating</topic><topic>Coatings</topic><topic>Dies</topic><topic>Entertainment industry</topic><topic>Environmentally friendly solvents</topic><topic>Green manufacturing</topic><topic>Halogenation</topic><topic>hot slot-die coating</topic><topic>Hydrocarbon refining</topic><topic>hydrocarbon solvents</topic><topic>Hydrocarbons</topic><topic>Kinetics</topic><topic>Large scale productions</topic><topic>Materials Science</topic><topic>Materials Science, Multidisciplinary</topic><topic>Morphology</topic><topic>Nanoscience & Nanotechnology</topic><topic>organic solar cells</topic><topic>Photovoltaic cells</topic><topic>Physical Sciences</topic><topic>Physics</topic><topic>Physics, Applied</topic><topic>Physics, Condensed Matter</topic><topic>Roll-to-roll processing</topic><topic>Science & Technology</topic><topic>Science & Technology - Other Topics</topic><topic>Slot dies</topic><topic>Solar cells</topic><topic>Solvents</topic><topic>Substrate temperature</topic><topic>Substrates</topic><topic>Sustainable development</topic><topic>Sustainable energy sources</topic><topic>Technology</topic><topic>Temperature dependence</topic><topic>Temperature dependent</topic><topic>temperature-dependent aggregation</topic><topic>Trimethylbenzene</topic><topic>Xylene</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhao, Heng</creatorcontrib><creatorcontrib>Naveed, Hafiz Bilal</creatorcontrib><creatorcontrib>Lin, Baojun</creatorcontrib><creatorcontrib>Zhou, Xiaobo</creatorcontrib><creatorcontrib>Yuan, Jian</creatorcontrib><creatorcontrib>Zhou, Ke</creatorcontrib><creatorcontrib>Wu, Hongbo</creatorcontrib><creatorcontrib>Guo, Renjun</creatorcontrib><creatorcontrib>Scheel, Manuel A.</creatorcontrib><creatorcontrib>Chumakov, Andrei</creatorcontrib><creatorcontrib>Roth, Stephan V.</creatorcontrib><creatorcontrib>Tang, Zheng</creatorcontrib><creatorcontrib>Müller‐Buschbaum, Peter</creatorcontrib><creatorcontrib>Ma, Wei</creatorcontrib><collection>Web of Science - Science Citation Index Expanded - 2020</collection><collection>Web of Science Core Collection</collection><collection>Science Citation Index Expanded</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>MEDLINE - Academic</collection><collection>SwePub</collection><collection>SwePub Articles</collection><collection>SWEPUB Kungliga Tekniska Högskolan</collection><jtitle>Advanced materials (Weinheim)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhao, Heng</au><au>Naveed, Hafiz Bilal</au><au>Lin, Baojun</au><au>Zhou, Xiaobo</au><au>Yuan, Jian</au><au>Zhou, Ke</au><au>Wu, Hongbo</au><au>Guo, Renjun</au><au>Scheel, Manuel A.</au><au>Chumakov, Andrei</au><au>Roth, Stephan V.</au><au>Tang, Zheng</au><au>Müller‐Buschbaum, Peter</au><au>Ma, Wei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Hot Hydrocarbon‐Solvent Slot‐Die Coating Enables High‐Efficiency Organic Solar Cells with Temperature‐Dependent Aggregation Behavior</atitle><jtitle>Advanced materials (Weinheim)</jtitle><stitle>ADV MATER</stitle><date>2020-10-01</date><risdate>2020</risdate><volume>32</volume><issue>39</issue><spage>e2002302</spage><epage>n/a</epage><pages>e2002302-n/a</pages><artnum>2002302</artnum><issn>0935-9648</issn><issn>1521-4095</issn><eissn>1521-4095</eissn><abstract>Organic solar cells (OSCs) have made rapid progress in terms of their development as a sustainable energy source. However, record‐breaking devices have not shown compatibility with large‐scale production via solution processing in particular due to the use of halogenated environment‐threatening solvents. Here, slot‐die fabrication with processing involving hydrocarbon‐based solvents is used to realize highly efficient and environmentally friendly OSCs. Highly compatible slot‐die coating with roll‐to‐roll processing using halogenated (chlorobenzene (CB)) and hydrocarbon solvents (1,2,4‐trimethylbenzene (TMB) and ortho‐xylene (o‐XY)) is used to fabricate photoactive films. Controlled solution and substrate temperatures enable similar aggregation states in the solution and similar kinetics processes during film formation. The optimized blend film nanostructures for different solvents in the highly efficient PM6:Y6 blend is adopted to show a similar morphology, which results in device efficiencies of 15.2%, 15.4%, and 15.6% for CB, TMB, and o‐XY solvents. This approach is successfully extended to other donor–acceptor combinations to demonstrate the excellent universality of this method. The results combine a method to optimize the aggregation state and film formation kinetics with the fabrication of OSCs with environmentally friendly solvents by slot‐die coating, which is a critical finding for the future development of OSCs in terms of their scalable production and high‐performance.
Highly efficient temperature‐dependent‐aggregation polymer‐based organic solar cells are fabricated by hot slot‐die coating with hydrocarbon solvents. Power conversion efficiencies of 15.2%, 15.4%, and 15.6% are obtained when chlorobenzene, 1,2,4‐trimethylbenzene (TMB), and ortho‐xylene are used, respectively.</abstract><cop>WEINHEIM</cop><pub>Wiley</pub><pmid>32812287</pmid><doi>10.1002/adma.202002302</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-7239-2010</orcidid><orcidid>https://orcid.org/0000-0001-6323-8401</orcidid><orcidid>https://orcid.org/0000-0003-0036-2362</orcidid></addata></record> |
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| subjects | 4-trimethylbenzene Agglomeration Aggregation behavior Chemistry Chemistry, Multidisciplinary Chemistry, Physical Chlorobenzene Coating Coatings Dies Entertainment industry Environmentally friendly solvents Green manufacturing Halogenation hot slot-die coating Hydrocarbon refining hydrocarbon solvents Hydrocarbons Kinetics Large scale productions Materials Science Materials Science, Multidisciplinary Morphology Nanoscience & Nanotechnology organic solar cells Photovoltaic cells Physical Sciences Physics Physics, Applied Physics, Condensed Matter Roll-to-roll processing Science & Technology Science & Technology - Other Topics Slot dies Solar cells Solvents Substrate temperature Substrates Sustainable development Sustainable energy sources Technology Temperature dependence Temperature dependent temperature-dependent aggregation Trimethylbenzene Xylene |
| title | Hot Hydrocarbon‐Solvent Slot‐Die Coating Enables High‐Efficiency Organic Solar Cells with Temperature‐Dependent Aggregation Behavior |
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