Shubnikov-de Haas oscillations of biaxial-strain-tuned superconductors in pulsed magnetic field up to 60 T
Two-dimensional (2D) materials have gained increasing prominence not only in fundamental research but also in daily applications. However, to fully harness their potential, it is crucial to optimize their properties with an external parameter and track the electronic structure simultaneously. Magnet...
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creator | King Yau Yip Wang, Lingfei Tsz Fung Poon Kai Ham Yu Siu Tung Lam Kwing To Lai Singleton, John Balakirev, Fedor F Goh, Swee K |
description | Two-dimensional (2D) materials have gained increasing prominence not only in fundamental research but also in daily applications. However, to fully harness their potential, it is crucial to optimize their properties with an external parameter and track the electronic structure simultaneously. Magnetotransport over a wide magnetic field range is a powerful method to probe the electronic structure and, for metallic 2D materials, quantum oscillations superimposed on the transport signals encode Fermi surface parameters. In this manuscript, we utilize biaxial strain as an external tuning parameter and investigate the effects of strain on the electronic properties of two quasi-2D superconductors, MoTe\(_2\) and RbV\(_3\)Sb\(_5\), by measuring their magnetoresistance in pulsed magnetic fields up to 60 T. With a careful selection of insulating substrates, we demonstrate the possibility of both the compressive and tensile biaxial strain, imposed on MoTe\(_2\) and RbV\(_3\)Sb\(_5\), respectively. For both systems, the applied strain has led to superconducting critical temperature enhancement compared to their free-standing counterparts, proving the effectiveness of this biaxial strain method at cryogenic temperatures. Clear quantum oscillations in the magnetoresistance -- the Shubnikov-de Haas (SdH) effect -- are obtained in both samples. In strained MoTe\(_2\), the magnetoresistance exhibits a nearly quadratic dependence on the magnetic field and remains non-saturating even at the highest field. Whereas in strained RbV\(_3\)Sb\(_5\), two SdH frequencies showed a substantial enhancement in effective mass values, hinting at a possible enhancement of charge fluctuations. Our results demonstrate that combining biaxial strain and pulsed magnetic field paves the way for studying 2D materials under unprecedented conditions. |
doi_str_mv | 10.48550/arxiv.2402.14534 |
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However, to fully harness their potential, it is crucial to optimize their properties with an external parameter and track the electronic structure simultaneously. Magnetotransport over a wide magnetic field range is a powerful method to probe the electronic structure and, for metallic 2D materials, quantum oscillations superimposed on the transport signals encode Fermi surface parameters. In this manuscript, we utilize biaxial strain as an external tuning parameter and investigate the effects of strain on the electronic properties of two quasi-2D superconductors, MoTe\(_2\) and RbV\(_3\)Sb\(_5\), by measuring their magnetoresistance in pulsed magnetic fields up to 60 T. With a careful selection of insulating substrates, we demonstrate the possibility of both the compressive and tensile biaxial strain, imposed on MoTe\(_2\) and RbV\(_3\)Sb\(_5\), respectively. For both systems, the applied strain has led to superconducting critical temperature enhancement compared to their free-standing counterparts, proving the effectiveness of this biaxial strain method at cryogenic temperatures. Clear quantum oscillations in the magnetoresistance -- the Shubnikov-de Haas (SdH) effect -- are obtained in both samples. In strained MoTe\(_2\), the magnetoresistance exhibits a nearly quadratic dependence on the magnetic field and remains non-saturating even at the highest field. Whereas in strained RbV\(_3\)Sb\(_5\), two SdH frequencies showed a substantial enhancement in effective mass values, hinting at a possible enhancement of charge fluctuations. Our results demonstrate that combining biaxial strain and pulsed magnetic field paves the way for studying 2D materials under unprecedented conditions.</description><identifier>EISSN: 2331-8422</identifier><identifier>DOI: 10.48550/arxiv.2402.14534</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Compressive properties ; Critical temperature ; Cryogenic temperature ; Electronic properties ; Electronic structure ; Electrons ; Fermi surfaces ; Insulation ; Magnetic fields ; Magnetoresistance ; Magnetoresistivity ; Oscillations ; Parameters ; Physics - Materials Science ; Physics - Strongly Correlated Electrons ; Physics - Superconductivity ; Substrates ; Superconductors ; Two dimensional materials</subject><ispartof>arXiv.org, 2024-02</ispartof><rights>2024. This work is published under http://arxiv.org/licenses/nonexclusive-distrib/1.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>http://arxiv.org/licenses/nonexclusive-distrib/1.0</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>228,230,781,785,886,27929</link.rule.ids><backlink>$$Uhttps://doi.org/10.48550/arXiv.2402.14534$$DView paper in arXiv$$Hfree_for_read</backlink><backlink>$$Uhttps://doi.org/10.1063/5.0191185$$DView published paper (Access to full text may be restricted)$$Hfree_for_read</backlink></links><search><creatorcontrib>King Yau Yip</creatorcontrib><creatorcontrib>Wang, Lingfei</creatorcontrib><creatorcontrib>Tsz Fung Poon</creatorcontrib><creatorcontrib>Kai Ham Yu</creatorcontrib><creatorcontrib>Siu Tung Lam</creatorcontrib><creatorcontrib>Kwing To Lai</creatorcontrib><creatorcontrib>Singleton, John</creatorcontrib><creatorcontrib>Balakirev, Fedor F</creatorcontrib><creatorcontrib>Goh, Swee K</creatorcontrib><title>Shubnikov-de Haas oscillations of biaxial-strain-tuned superconductors in pulsed magnetic field up to 60 T</title><title>arXiv.org</title><description>Two-dimensional (2D) materials have gained increasing prominence not only in fundamental research but also in daily applications. 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For both systems, the applied strain has led to superconducting critical temperature enhancement compared to their free-standing counterparts, proving the effectiveness of this biaxial strain method at cryogenic temperatures. Clear quantum oscillations in the magnetoresistance -- the Shubnikov-de Haas (SdH) effect -- are obtained in both samples. In strained MoTe\(_2\), the magnetoresistance exhibits a nearly quadratic dependence on the magnetic field and remains non-saturating even at the highest field. Whereas in strained RbV\(_3\)Sb\(_5\), two SdH frequencies showed a substantial enhancement in effective mass values, hinting at a possible enhancement of charge fluctuations. Our results demonstrate that combining biaxial strain and pulsed magnetic field paves the way for studying 2D materials under unprecedented conditions.</description><subject>Compressive properties</subject><subject>Critical temperature</subject><subject>Cryogenic temperature</subject><subject>Electronic properties</subject><subject>Electronic structure</subject><subject>Electrons</subject><subject>Fermi surfaces</subject><subject>Insulation</subject><subject>Magnetic fields</subject><subject>Magnetoresistance</subject><subject>Magnetoresistivity</subject><subject>Oscillations</subject><subject>Parameters</subject><subject>Physics - Materials Science</subject><subject>Physics - Strongly Correlated Electrons</subject><subject>Physics - Superconductivity</subject><subject>Substrates</subject><subject>Superconductors</subject><subject>Two dimensional materials</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GOX</sourceid><recordid>eNotkE1LAzEURYMgWGp_gCsDrqfme8alFLVCwYXdDy-TRFOnyZhMSv33jq2rx-UdLpeD0A0lS9FISe4hHf1hyQRhSyokFxdoxjinVSMYu0KLnHeEEKZqJiWfod37Z9HBf8VDZSxeA2Qcc-f7HkYfwxQc1h6OHvoqjwl8qMYSrMG5DDZ1MZjSjTFl7AMeSp-nzx4-gh19h523vcFlwGPEiuDtNbp0MCGL_ztH2-en7Wpdbd5eXlePmwokYxUYVQuntKXANXWgLGdEGSm000KDbQB0Z4hyVlpSO0GBdJIYpkQNjtGGz9HtufYkoh2S30P6af-EtCchE3F3JoYUv4vNY7uLJYVpU8seOCWEy5rxX0vjZSY</recordid><startdate>20240222</startdate><enddate>20240222</enddate><creator>King Yau Yip</creator><creator>Wang, Lingfei</creator><creator>Tsz Fung Poon</creator><creator>Kai Ham Yu</creator><creator>Siu Tung Lam</creator><creator>Kwing To Lai</creator><creator>Singleton, John</creator><creator>Balakirev, Fedor F</creator><creator>Goh, Swee K</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><scope>GOX</scope></search><sort><creationdate>20240222</creationdate><title>Shubnikov-de Haas oscillations of biaxial-strain-tuned superconductors in pulsed magnetic field up to 60 T</title><author>King Yau Yip ; 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For both systems, the applied strain has led to superconducting critical temperature enhancement compared to their free-standing counterparts, proving the effectiveness of this biaxial strain method at cryogenic temperatures. Clear quantum oscillations in the magnetoresistance -- the Shubnikov-de Haas (SdH) effect -- are obtained in both samples. In strained MoTe\(_2\), the magnetoresistance exhibits a nearly quadratic dependence on the magnetic field and remains non-saturating even at the highest field. Whereas in strained RbV\(_3\)Sb\(_5\), two SdH frequencies showed a substantial enhancement in effective mass values, hinting at a possible enhancement of charge fluctuations. Our results demonstrate that combining biaxial strain and pulsed magnetic field paves the way for studying 2D materials under unprecedented conditions.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><doi>10.48550/arxiv.2402.14534</doi><oa>free_for_read</oa></addata></record> |
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subjects | Compressive properties Critical temperature Cryogenic temperature Electronic properties Electronic structure Electrons Fermi surfaces Insulation Magnetic fields Magnetoresistance Magnetoresistivity Oscillations Parameters Physics - Materials Science Physics - Strongly Correlated Electrons Physics - Superconductivity Substrates Superconductors Two dimensional materials |
title | Shubnikov-de Haas oscillations of biaxial-strain-tuned superconductors in pulsed magnetic field up to 60 T |
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