Decoherence and Revival in Attosecond Charge Migration Driven by Non-adiabatic Dynamics

Attosecond charge migration is a periodic evolution of the charge density of a molecule on a time scale defined by the energy intervals between the electronic states involved. Here, we report the observation of charge migration in neutral silane (SiH\(_4\)) in 690~as, its decoherence within 15~fs, a...

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Veröffentlicht in:	arXiv.org 2021-10
Hauptverfasser:	Matselyukh, Danylo, Despré, Victor, Golubev, Nikolay, Kuleff, Alexander, Hans Jakob Wörner
Format:	Artikel
Sprache:	eng
Schlagworte:	Adiabatic flow Charge density Coherence Electron states Physics - Chemical Physics Valence
Online-Zugang:	Volltext
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