Note: Vibronic coupling in light-harvesting complex II revisited
We discuss our recent theoretical work on vibronic coupling mechanisms in a model energy transfer system in the context of previous 2DEV experiments on a natural light-harvesting system, light-harvesting complex II (LHCII), where vibronic signatures were suggested to be involved in energy transfer....
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creator | Arsenault, Eric A Schile, Addison J Limmer, David T Fleming, Graham R |
description | We discuss our recent theoretical work on vibronic coupling mechanisms in a model energy transfer system in the context of previous 2DEV experiments on a natural light-harvesting system, light-harvesting complex II (LHCII), where vibronic signatures were suggested to be involved in energy transfer. In this comparison, we directly assign the vibronic coupling mechanism in LHCII as arising from Herzberg-Teller activity and show how this coupling modulates the energy transfer dynamics in this photosynthetic system. |
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subjects | Coupling Energy transfer Natural lighting Photosynthesis Physics - Chemical Physics Physics - Mesoscale and Nanoscale Physics |
title | Note: Vibronic coupling in light-harvesting complex II revisited |
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