Tracking ultrafast solid-state dynamics using high harmonic spectroscopy
We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy for photoinduced dynamics in strongly correlated materials through a detailed investigation of the insulator-to-metal transitions in vanadium dioxide. We benchmark our technique by comparing our measurements to e...
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| creator | Bionta, Mina R Haddad, Elissa Leblanc, Adrien Gruson, Vincent Lassonde, Philippe Ibrahim, Heide Chaillou, Jérémie Émond, Nicolas Otto, Martin R Siwick, Bradley J Chaker, Mohamed Légaré, François |
| description | We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy for photoinduced dynamics in strongly correlated materials through a detailed investigation of the insulator-to-metal transitions in vanadium dioxide. We benchmark our technique by comparing our measurements to established momentum-resolved ultrafast electron diffraction, and theoretical density functional calculations. Tr-HHG allows distinguishing of individual dynamic channels, including a transition to a thermodynamically hidden phase. In addition, the HHG yield is shown to be modulated at a frequency characteristic of a coherent phonon in the equilibrium monoclinic phase over a wide range of excitation fluences. These results demonstrate that tr-HHG is capable of tracking complex dynamics in solids through its sensitivity to the band structure. |
| doi_str_mv | 10.48550/arxiv.2003.10430 |
| format | Article |
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| subjects | Dynamic structural analysis Electron diffraction Harmonic generations Physics - Materials Science Physics - Optics Spectroscopy Spectrum analysis Theoretical density Tracking Vanadium dioxide |
| title | Tracking ultrafast solid-state dynamics using high harmonic spectroscopy |
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