Structure-dynamics relationship in ratcheted colloids: Resonance melting, dislocations, and defect clusters

We consider a two dimensional colloidal dispersion of soft-core particles driven by a one dimensional stochastic flashing ratchet that induces a time averaged directed particle current through the system. It undergoes a non-equilibrium melting transition as the directed current approaches a maximum...

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Veröffentlicht in:arXiv.org 2019-11
Hauptverfasser: Shubhendu Shekhar Khali, Chakraborty, Dipanjan, Chaudhuri, Debasish
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description We consider a two dimensional colloidal dispersion of soft-core particles driven by a one dimensional stochastic flashing ratchet that induces a time averaged directed particle current through the system. It undergoes a non-equilibrium melting transition as the directed current approaches a maximum associated with a resonance of the ratcheting frequency with the relaxation frequency of the system. We use extensive molecular dynamics simulations to present a detailed phase diagram in the ratcheting rate-mean density plane. With the help of numerically calculated structure factor, solid and hexatic order parameters, and pair correlation functions, we show that the non-equilibrium melting is a continuous transition from a quasi-long ranged ordered solid to a hexatic phase. The transition is mediated by the unbinding of dislocations, and formation of compact and string-like defect clusters.
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subjects Clusters
Computer simulation
Hexatic phases
Melting
Molecular dynamics
Order parameters
Phase diagrams
Phase transitions
Physics - Soft Condensed Matter
Ratcheting
Resonance
Serrated yielding
Structure factor
title Structure-dynamics relationship in ratcheted colloids: Resonance melting, dislocations, and defect clusters
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