Lattice dynamics coupled to charge and spin degrees of freedom in the molecular dimer-Mott insulator $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl

Inelastic neutron scattering measurements on the molecular dimer-Mott insulator $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl reveal a phonon anomaly in a wide temperature range. Starting from $T_{\rm ins}\sim50$-$60$ K where the charge gap opens, the low-lying optical phonon modes become overdamped up...

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Hauptverfasser: Matsuura, Masato, Sasaki, Takahiko, Iguchi, Satoshi, Gati, Elena, Müller, Jens, Stockert, Oliver, Piovano, Andrea, Böhm, Martin, Park, Jitae T, Biswas, Sananda, Winter, Stephen M, Valentí, Roser, Nakao, Akiko, Lang, Michael
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Sprache:eng
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