Langevin Approach to Quantum Optics with Molecules
We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles o...
Gespeichert in:
| Veröffentlicht in: | arXiv.org 2020-04 |
|---|---|
| Hauptverfasser: | , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | |
|---|---|
| container_issue | |
| container_start_page | |
| container_title | arXiv.org |
| container_volume | |
| creator | Reitz, Michael Sommer, Christian Genes, Claudiu |
| description | We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles of molecules driven by classical fields or coupled to quantized optical modes. We retrieve analytical expressions for the modification of the radiative emission branching ratio in the Purcell regime and for the asymmetric cavity transmission associated with dissipative cross-talk between upper and lower polaritons in the strong coupling regime. We also characterize the F\"{o}rster resonance energy transfer process between donor-acceptor molecules mediated by the vacuum or by a cavity mode. |
| doi_str_mv | 10.48550/arxiv.1812.08592 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_arxiv</sourceid><recordid>TN_cdi_arxiv_primary_1812_08592</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2159541890</sourcerecordid><originalsourceid>FETCH-LOGICAL-a520-6be4faf4dd119552845dafbb26ae2ae8f90e94d46c7e3cb1b12f31cf2baa24073</originalsourceid><addsrcrecordid>eNotj11LwzAYRoMgOOZ-gFcGvG5N3iRtcjmGX1AZwu7LmzRxHV1bm3bqv3cfXj03h4dzCLnjLJVaKfaIw099SLnmkDKtDFyRGQjBEy0Bbsgixh1jDLIclBIzAgW2n_5Qt3TZ90OHbkvHjn5M2I7Tnq77sXaRftfjlr53jXdT4-MtuQ7YRL_43znZPD9tVq9JsX55Wy2LBBWwJLNeBgyyqjg3SoGWqsJgLWToAb0OhnkjK5m53AtnueUQBHcBLCJIlos5ub_cnoPKfqj3OPyWp7DyHHYkHi7EUfxr8nEsd900tEenErgySnJtmPgD8K9QdA</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2159541890</pqid></control><display><type>article</type><title>Langevin Approach to Quantum Optics with Molecules</title><source>arXiv.org</source><source>Free E- Journals</source><creator>Reitz, Michael ; Sommer, Christian ; Genes, Claudiu</creator><creatorcontrib>Reitz, Michael ; Sommer, Christian ; Genes, Claudiu</creatorcontrib><description>We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles of molecules driven by classical fields or coupled to quantized optical modes. We retrieve analytical expressions for the modification of the radiative emission branching ratio in the Purcell regime and for the asymmetric cavity transmission associated with dissipative cross-talk between upper and lower polaritons in the strong coupling regime. We also characterize the F\"{o}rster resonance energy transfer process between donor-acceptor molecules mediated by the vacuum or by a cavity mode.</description><identifier>EISSN: 2331-8422</identifier><identifier>DOI: 10.48550/arxiv.1812.08592</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Coupling (molecular) ; Emitters ; Energy transfer ; Energy transmission ; Fluorescence ; Holes ; Physics - Quantum Physics ; Quantum electrodynamics ; Quantum theory</subject><ispartof>arXiv.org, 2020-04</ispartof><rights>2020. This work is published under http://arxiv.org/licenses/nonexclusive-distrib/1.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>http://arxiv.org/licenses/nonexclusive-distrib/1.0</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>228,230,776,780,881,27904</link.rule.ids><backlink>$$Uhttps://doi.org/10.1103/PhysRevLett.122.203602$$DView published paper (Access to full text may be restricted)$$Hfree_for_read</backlink><backlink>$$Uhttps://doi.org/10.48550/arXiv.1812.08592$$DView paper in arXiv$$Hfree_for_read</backlink></links><search><creatorcontrib>Reitz, Michael</creatorcontrib><creatorcontrib>Sommer, Christian</creatorcontrib><creatorcontrib>Genes, Claudiu</creatorcontrib><title>Langevin Approach to Quantum Optics with Molecules</title><title>arXiv.org</title><description>We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles of molecules driven by classical fields or coupled to quantized optical modes. We retrieve analytical expressions for the modification of the radiative emission branching ratio in the Purcell regime and for the asymmetric cavity transmission associated with dissipative cross-talk between upper and lower polaritons in the strong coupling regime. We also characterize the F\"{o}rster resonance energy transfer process between donor-acceptor molecules mediated by the vacuum or by a cavity mode.</description><subject>Coupling (molecular)</subject><subject>Emitters</subject><subject>Energy transfer</subject><subject>Energy transmission</subject><subject>Fluorescence</subject><subject>Holes</subject><subject>Physics - Quantum Physics</subject><subject>Quantum electrodynamics</subject><subject>Quantum theory</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GOX</sourceid><recordid>eNotj11LwzAYRoMgOOZ-gFcGvG5N3iRtcjmGX1AZwu7LmzRxHV1bm3bqv3cfXj03h4dzCLnjLJVaKfaIw099SLnmkDKtDFyRGQjBEy0Bbsgixh1jDLIclBIzAgW2n_5Qt3TZ90OHbkvHjn5M2I7Tnq77sXaRftfjlr53jXdT4-MtuQ7YRL_43znZPD9tVq9JsX55Wy2LBBWwJLNeBgyyqjg3SoGWqsJgLWToAb0OhnkjK5m53AtnueUQBHcBLCJIlos5ub_cnoPKfqj3OPyWp7DyHHYkHi7EUfxr8nEsd900tEenErgySnJtmPgD8K9QdA</recordid><startdate>20200424</startdate><enddate>20200424</enddate><creator>Reitz, Michael</creator><creator>Sommer, Christian</creator><creator>Genes, Claudiu</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><scope>GOX</scope></search><sort><creationdate>20200424</creationdate><title>Langevin Approach to Quantum Optics with Molecules</title><author>Reitz, Michael ; Sommer, Christian ; Genes, Claudiu</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a520-6be4faf4dd119552845dafbb26ae2ae8f90e94d46c7e3cb1b12f31cf2baa24073</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Coupling (molecular)</topic><topic>Emitters</topic><topic>Energy transfer</topic><topic>Energy transmission</topic><topic>Fluorescence</topic><topic>Holes</topic><topic>Physics - Quantum Physics</topic><topic>Quantum electrodynamics</topic><topic>Quantum theory</topic><toplevel>online_resources</toplevel><creatorcontrib>Reitz, Michael</creatorcontrib><creatorcontrib>Sommer, Christian</creatorcontrib><creatorcontrib>Genes, Claudiu</creatorcontrib><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering Collection</collection><collection>arXiv.org</collection><jtitle>arXiv.org</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Reitz, Michael</au><au>Sommer, Christian</au><au>Genes, Claudiu</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Langevin Approach to Quantum Optics with Molecules</atitle><jtitle>arXiv.org</jtitle><date>2020-04-24</date><risdate>2020</risdate><eissn>2331-8422</eissn><abstract>We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles of molecules driven by classical fields or coupled to quantized optical modes. We retrieve analytical expressions for the modification of the radiative emission branching ratio in the Purcell regime and for the asymmetric cavity transmission associated with dissipative cross-talk between upper and lower polaritons in the strong coupling regime. We also characterize the F\"{o}rster resonance energy transfer process between donor-acceptor molecules mediated by the vacuum or by a cavity mode.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><doi>10.48550/arxiv.1812.08592</doi><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | EISSN: 2331-8422 |
| ispartof | arXiv.org, 2020-04 |
| issn | 2331-8422 |
| language | eng |
| recordid | cdi_arxiv_primary_1812_08592 |
| source | arXiv.org; Free E- Journals |
| subjects | Coupling (molecular) Emitters Energy transfer Energy transmission Fluorescence Holes Physics - Quantum Physics Quantum electrodynamics Quantum theory |
| title | Langevin Approach to Quantum Optics with Molecules |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-23T21%3A29%3A14IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_arxiv&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Langevin%20Approach%20to%20Quantum%20Optics%20with%20Molecules&rft.jtitle=arXiv.org&rft.au=Reitz,%20Michael&rft.date=2020-04-24&rft.eissn=2331-8422&rft_id=info:doi/10.48550/arxiv.1812.08592&rft_dat=%3Cproquest_arxiv%3E2159541890%3C/proquest_arxiv%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2159541890&rft_id=info:pmid/&rfr_iscdi=true |