Spatially-resolved Fluorescence-detected Two-dimensional Electronic Spectroscopy Probes Varying Electronic Couplings in Photosynthetic Bacteria

We present a variation of two-dimensional electronic spectroscopy that is capable of mapping spatially-varying differences in electronic couplings using a correlated map of excitation and detection frequencies, with sensitivity orders of magnitude better than conventional spatially-averaged electron...

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Veröffentlicht in:arXiv.org 2018-02
Hauptverfasser: Tiwari, Vivek, Acosta-Matutes, Yassel, Gardiner, Alastair T, Cogdell, Richard J, Ogilvie, Jennifer P
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Sprache:eng
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