Importance of van der Waals interactions and cation-anion coupling in an organic quantum spin liquid

The Mott insulator \(\beta'\)-EtMe\(_3\)Sb[Pd(dmit)\(_2\)]\(_2\) belongs to a class of charge transfer solids with highly-frustrated triangular lattice of \(S=1/2\) molecular dimers and a quantum-spin-liquid ground state. Our experimental and ab initio theoretical studies show the fingerprints...

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Veröffentlicht in:	arXiv.org 2017-12
Hauptverfasser:	Lazić, P, Pinterić, M, D Rivas Góngora, Pustogow, A, Treptow, K, Ivek, T, Milat, O, Gumhalter, B, Došlić, N, Dressel, M, Tomić, S
Format:	Artikel
Sprache:	eng
Schlagworte:	Bonding strength Cations Charge transfer Coupling (molecular) Dimers Dipoles Electron states Ground state Molecular structure Physics - Strongly Correlated Electrons Spin liquid
Online-Zugang:	Volltext
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