Tuning Perpendicular Magnetic Anisotropy by Oxygen Octahedral Rotations in (La$_{1-x}$Sr$_{x}$MnO$_{3}$)/(SrIrO$_{3}$) Superlattices

Perpendicular magnetic anisotropy (PMA) plays a critical role in the development of spintronics, thereby demanding new strategies to control PMA. Here we demonstrate a conceptually new type of interface induced PMA that is controlled by oxygen octahedral rotation. In superlattices comprised of La$_{...

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Hauptverfasser: Yi, Di, Flint, Charles L, Balakrishnan, Purnima P, Mahalingam, Krishnamurthy, Urwin, Brittany, Vailionis, Arturas, NDiaye, Alpha T, Shafer, Padraic, Arenholz, Elke, Choi, Yongseong, Stone, Kevin H, Chu, JiunHaw, Howe, Brandon M, Liu, Jian, Fisher, Ian R, Suzuki, Yuri
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creator Yi, Di
Flint, Charles L
Balakrishnan, Purnima P
Mahalingam, Krishnamurthy
Urwin, Brittany
Vailionis, Arturas
NDiaye, Alpha T
Shafer, Padraic
Arenholz, Elke
Choi, Yongseong
Stone, Kevin H
Chu, JiunHaw
Howe, Brandon M
Liu, Jian
Fisher, Ian R
Suzuki, Yuri
description Perpendicular magnetic anisotropy (PMA) plays a critical role in the development of spintronics, thereby demanding new strategies to control PMA. Here we demonstrate a conceptually new type of interface induced PMA that is controlled by oxygen octahedral rotation. In superlattices comprised of La$_{1-x}$Sr$_{x}$MnO$_{3}$ and SrIrO$_{3}$, we find that all superlattices (0$\leq$x$\leq$1) exhibit ferromagnetism despite the fact that La$_{1-x}$Sr$_{x}$MnO$_{3}$ is antiferromagnetic for x$>$0.5. PMA as high as 4$\times$10$^6$ erg/cm$^3$ is observed by increasing x and attributed to a decrease of oxygen octahedral rotation at interfaces. We also demonstrate that oxygen octahedral deformation cannot explain the trend in PMA. These results reveal a new degree of freedom to control PMA, enabling discovery of emergent magnetic textures and topological phenomena.
doi_str_mv 10.48550/arxiv.1707.03460
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title Tuning Perpendicular Magnetic Anisotropy by Oxygen Octahedral Rotations in (La$_{1-x}$Sr$_{x}$MnO$_{3}$)/(SrIrO$_{3}$) Superlattices
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