Can 3D light localization be reached in "white paint"?
When waves scatter multiple times in 3D random media, a disorder driven phase transition from diffusion to localization may occur [Anderson 1958 Phys. Rev. 109 1492-505; Abrahams et al 1979 Phys. Rev. Lett. 42 673-6]. In "The question of classical localization: A theory of white paint?" P....
Gespeichert in:
Veröffentlicht in: | arXiv.org 2016-01 |
---|---|
Hauptverfasser: | , , , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | |
---|---|
container_issue | |
container_start_page | |
container_title | arXiv.org |
container_volume | |
creator | Sperling, Tilo Schertel, Lukas Ackermann, Mirco Aubry, Geoffroy J Aegerter, Christof M Maret, Georg |
description | When waves scatter multiple times in 3D random media, a disorder driven phase transition from diffusion to localization may occur [Anderson 1958 Phys. Rev. 109 1492-505; Abrahams et al 1979 Phys. Rev. Lett. 42 673-6]. In "The question of classical localization: A theory of white paint?" P.W. Anderson suggested the possibility to observe light localization in TiO\(_2\) samples [Anderson 1985 Phil. Mag. B 52 505-9]. We recently claimed the observation of localization effects measuring photon time of flight (ToF) distributions [St\"orzer et al 2006 Phys. Rev. Lett. 96 063904] and evaluating transmission profiles (TP) [Sperling et al 2013 Nat. Photonics 7 48-52] in such TiO\(_2\) samples. Here we present a careful study of the long time tail of ToF distributions and the long time behavior of the TP width for very thin samples and different turbidities that questions the localization interpretation. We further show new data that allow an alternative consistent explanation of these previous data by a fluorescence process. An adapted diffusion model including an appropriate exponential fluorescence decay accounts for the shape of the ToF distributions and the TP width. These observations question whether the strong localization regime can be reached with visible light scattering in polydisperse TiO\(_2\) samples, since the disorder parameter can hardly be increased any further in such a "white paint" material. |
doi_str_mv | 10.48550/arxiv.1510.08092 |
format | Article |
fullrecord | <record><control><sourceid>proquest_arxiv</sourceid><recordid>TN_cdi_arxiv_primary_1510_08092</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2077942615</sourcerecordid><originalsourceid>FETCH-LOGICAL-a525-1bd19d1fb89051481e4763f4b8293c83b00f9c7c07f292d8ac2296f5a33b61ca3</originalsourceid><addsrcrecordid>eNotj0tLAzEYRYMgWGp_gCtDXU9NvrxXIuMTCm66H5JM4qSMMzUz9fXrHVtXFy6Hyz0IXVCy4loIcm3zV_pYUTEVRBMDJ2gGjNFCc4AztBiGLSEEpAIh2AzJ0naY3eE2vTYjbntv2_Rjx9R32AWcg_VNqHHq8PKzSWPAO5u6cXlzjk6jbYew-M852jzcb8qnYv3y-FzergsrQBTU1dTUNDptiKBc08CVZJE7DYZ5zRwh0XjliYpgoNbWAxgZhWXMSeotm6PL4-xBqtrl9Gbzd_UnVx3kJuLqSOxy_74Pw1ht-33upk8VEKUMB0kF-wWluE8J</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2077942615</pqid></control><display><type>article</type><title>Can 3D light localization be reached in "white paint"?</title><source>arXiv.org</source><source>Free E- Journals</source><creator>Sperling, Tilo ; Schertel, Lukas ; Ackermann, Mirco ; Aubry, Geoffroy J ; Aegerter, Christof M ; Maret, Georg</creator><creatorcontrib>Sperling, Tilo ; Schertel, Lukas ; Ackermann, Mirco ; Aubry, Geoffroy J ; Aegerter, Christof M ; Maret, Georg</creatorcontrib><description>When waves scatter multiple times in 3D random media, a disorder driven phase transition from diffusion to localization may occur [Anderson 1958 Phys. Rev. 109 1492-505; Abrahams et al 1979 Phys. Rev. Lett. 42 673-6]. In "The question of classical localization: A theory of white paint?" P.W. Anderson suggested the possibility to observe light localization in TiO\(_2\) samples [Anderson 1985 Phil. Mag. B 52 505-9]. We recently claimed the observation of localization effects measuring photon time of flight (ToF) distributions [St\"orzer et al 2006 Phys. Rev. Lett. 96 063904] and evaluating transmission profiles (TP) [Sperling et al 2013 Nat. Photonics 7 48-52] in such TiO\(_2\) samples. Here we present a careful study of the long time tail of ToF distributions and the long time behavior of the TP width for very thin samples and different turbidities that questions the localization interpretation. We further show new data that allow an alternative consistent explanation of these previous data by a fluorescence process. An adapted diffusion model including an appropriate exponential fluorescence decay accounts for the shape of the ToF distributions and the TP width. These observations question whether the strong localization regime can be reached with visible light scattering in polydisperse TiO\(_2\) samples, since the disorder parameter can hardly be increased any further in such a "white paint" material.</description><identifier>EISSN: 2331-8422</identifier><identifier>DOI: 10.48550/arxiv.1510.08092</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Fluorescence ; Light scattering ; Localization ; Phase transitions ; Photonics ; Physics - Disordered Systems and Neural Networks ; Physics - Mesoscale and Nanoscale Physics ; Physics - Optics</subject><ispartof>arXiv.org, 2016-01</ispartof><rights>2016. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>http://creativecommons.org/licenses/by/4.0</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>228,230,780,784,885,27925</link.rule.ids><backlink>$$Uhttps://doi.org/10.48550/arXiv.1510.08092$$DView paper in arXiv$$Hfree_for_read</backlink><backlink>$$Uhttps://doi.org/10.1088/1367-2630/18/1/013039$$DView published paper (Access to full text may be restricted)$$Hfree_for_read</backlink></links><search><creatorcontrib>Sperling, Tilo</creatorcontrib><creatorcontrib>Schertel, Lukas</creatorcontrib><creatorcontrib>Ackermann, Mirco</creatorcontrib><creatorcontrib>Aubry, Geoffroy J</creatorcontrib><creatorcontrib>Aegerter, Christof M</creatorcontrib><creatorcontrib>Maret, Georg</creatorcontrib><title>Can 3D light localization be reached in "white paint"?</title><title>arXiv.org</title><description>When waves scatter multiple times in 3D random media, a disorder driven phase transition from diffusion to localization may occur [Anderson 1958 Phys. Rev. 109 1492-505; Abrahams et al 1979 Phys. Rev. Lett. 42 673-6]. In "The question of classical localization: A theory of white paint?" P.W. Anderson suggested the possibility to observe light localization in TiO\(_2\) samples [Anderson 1985 Phil. Mag. B 52 505-9]. We recently claimed the observation of localization effects measuring photon time of flight (ToF) distributions [St\"orzer et al 2006 Phys. Rev. Lett. 96 063904] and evaluating transmission profiles (TP) [Sperling et al 2013 Nat. Photonics 7 48-52] in such TiO\(_2\) samples. Here we present a careful study of the long time tail of ToF distributions and the long time behavior of the TP width for very thin samples and different turbidities that questions the localization interpretation. We further show new data that allow an alternative consistent explanation of these previous data by a fluorescence process. An adapted diffusion model including an appropriate exponential fluorescence decay accounts for the shape of the ToF distributions and the TP width. These observations question whether the strong localization regime can be reached with visible light scattering in polydisperse TiO\(_2\) samples, since the disorder parameter can hardly be increased any further in such a "white paint" material.</description><subject>Fluorescence</subject><subject>Light scattering</subject><subject>Localization</subject><subject>Phase transitions</subject><subject>Photonics</subject><subject>Physics - Disordered Systems and Neural Networks</subject><subject>Physics - Mesoscale and Nanoscale Physics</subject><subject>Physics - Optics</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GOX</sourceid><recordid>eNotj0tLAzEYRYMgWGp_gCtDXU9NvrxXIuMTCm66H5JM4qSMMzUz9fXrHVtXFy6Hyz0IXVCy4loIcm3zV_pYUTEVRBMDJ2gGjNFCc4AztBiGLSEEpAIh2AzJ0naY3eE2vTYjbntv2_Rjx9R32AWcg_VNqHHq8PKzSWPAO5u6cXlzjk6jbYew-M852jzcb8qnYv3y-FzergsrQBTU1dTUNDptiKBc08CVZJE7DYZ5zRwh0XjliYpgoNbWAxgZhWXMSeotm6PL4-xBqtrl9Gbzd_UnVx3kJuLqSOxy_74Pw1ht-33upk8VEKUMB0kF-wWluE8J</recordid><startdate>20160119</startdate><enddate>20160119</enddate><creator>Sperling, Tilo</creator><creator>Schertel, Lukas</creator><creator>Ackermann, Mirco</creator><creator>Aubry, Geoffroy J</creator><creator>Aegerter, Christof M</creator><creator>Maret, Georg</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><scope>GOX</scope></search><sort><creationdate>20160119</creationdate><title>Can 3D light localization be reached in "white paint"?</title><author>Sperling, Tilo ; Schertel, Lukas ; Ackermann, Mirco ; Aubry, Geoffroy J ; Aegerter, Christof M ; Maret, Georg</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a525-1bd19d1fb89051481e4763f4b8293c83b00f9c7c07f292d8ac2296f5a33b61ca3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Fluorescence</topic><topic>Light scattering</topic><topic>Localization</topic><topic>Phase transitions</topic><topic>Photonics</topic><topic>Physics - Disordered Systems and Neural Networks</topic><topic>Physics - Mesoscale and Nanoscale Physics</topic><topic>Physics - Optics</topic><toplevel>online_resources</toplevel><creatorcontrib>Sperling, Tilo</creatorcontrib><creatorcontrib>Schertel, Lukas</creatorcontrib><creatorcontrib>Ackermann, Mirco</creatorcontrib><creatorcontrib>Aubry, Geoffroy J</creatorcontrib><creatorcontrib>Aegerter, Christof M</creatorcontrib><creatorcontrib>Maret, Georg</creatorcontrib><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Access via ProQuest (Open Access)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering Collection</collection><collection>arXiv.org</collection><jtitle>arXiv.org</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Sperling, Tilo</au><au>Schertel, Lukas</au><au>Ackermann, Mirco</au><au>Aubry, Geoffroy J</au><au>Aegerter, Christof M</au><au>Maret, Georg</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Can 3D light localization be reached in "white paint"?</atitle><jtitle>arXiv.org</jtitle><date>2016-01-19</date><risdate>2016</risdate><eissn>2331-8422</eissn><abstract>When waves scatter multiple times in 3D random media, a disorder driven phase transition from diffusion to localization may occur [Anderson 1958 Phys. Rev. 109 1492-505; Abrahams et al 1979 Phys. Rev. Lett. 42 673-6]. In "The question of classical localization: A theory of white paint?" P.W. Anderson suggested the possibility to observe light localization in TiO\(_2\) samples [Anderson 1985 Phil. Mag. B 52 505-9]. We recently claimed the observation of localization effects measuring photon time of flight (ToF) distributions [St\"orzer et al 2006 Phys. Rev. Lett. 96 063904] and evaluating transmission profiles (TP) [Sperling et al 2013 Nat. Photonics 7 48-52] in such TiO\(_2\) samples. Here we present a careful study of the long time tail of ToF distributions and the long time behavior of the TP width for very thin samples and different turbidities that questions the localization interpretation. We further show new data that allow an alternative consistent explanation of these previous data by a fluorescence process. An adapted diffusion model including an appropriate exponential fluorescence decay accounts for the shape of the ToF distributions and the TP width. These observations question whether the strong localization regime can be reached with visible light scattering in polydisperse TiO\(_2\) samples, since the disorder parameter can hardly be increased any further in such a "white paint" material.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><doi>10.48550/arxiv.1510.08092</doi><oa>free_for_read</oa></addata></record> |
fulltext | fulltext |
identifier | EISSN: 2331-8422 |
ispartof | arXiv.org, 2016-01 |
issn | 2331-8422 |
language | eng |
recordid | cdi_arxiv_primary_1510_08092 |
source | arXiv.org; Free E- Journals |
subjects | Fluorescence Light scattering Localization Phase transitions Photonics Physics - Disordered Systems and Neural Networks Physics - Mesoscale and Nanoscale Physics Physics - Optics |
title | Can 3D light localization be reached in "white paint"? |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-20T11%3A50%3A54IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_arxiv&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Can%203D%20light%20localization%20be%20reached%20in%20%22white%20paint%22?&rft.jtitle=arXiv.org&rft.au=Sperling,%20Tilo&rft.date=2016-01-19&rft.eissn=2331-8422&rft_id=info:doi/10.48550/arxiv.1510.08092&rft_dat=%3Cproquest_arxiv%3E2077942615%3C/proquest_arxiv%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2077942615&rft_id=info:pmid/&rfr_iscdi=true |