Angle-resolved photoemission spectroscopy with 9-eV photon-energy pulses generated in a gas-filled hollow-core photonic crystal fiber
A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few {\mu}J energy generate vacuum ultraviolet...
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| creator | Bromberger, H Ermolov, A Belli, F Liu, H Calegari, F Chavez-Cervantes, M Li, M T Lin, C T Abdolvand, A Russell, P St J Cavalleri, A Travers, J C Gierz, I |
| description | A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few {\mu}J energy generate vacuum ultraviolet (VUV) radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi2Se3 with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz, with photon energies that cover the first Brillouin zone of most materials. |
| doi_str_mv | 10.48550/arxiv.1504.07505 |
| format | Article |
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| subjects | Brillouin zones Crystal fibers Femtosecond pulses Gas jets Near infrared radiation Photoelectric emission Photoelectron spectroscopy Photonic crystals Physics - Optics Signal to noise ratio Spectrum analysis Ultraviolet radiation |
| title | Angle-resolved photoemission spectroscopy with 9-eV photon-energy pulses generated in a gas-filled hollow-core photonic crystal fiber |
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