Hyperfine magnetic field in ferromagnetic graphite

Information on atomic-scale features is required for a better understanding of the mechanisms leading to magnetism in non-metallic, carbon-based materials. This work reports a direct evaluation of the hyperfine magnetic field produced at 13C nuclei in ferromagnetic graphite by nuclear magnetic reson...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:arXiv.org 2014-06
Hauptverfasser: Freitas, Jair C C, Scopel, Wanderlã L, Paz, Wendel S, Bernardes, Leandro V, Cunha-Filho, Francisco E, Speglich, Carlos, Araújo-Moreira, Fernando M, Pelc, Damjan, Cvitanić, Tonči, Požek, Miroslav
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page
container_issue
container_start_page
container_title arXiv.org
container_volume
creator Freitas, Jair C C
Scopel, Wanderlã L
Paz, Wendel S
Bernardes, Leandro V
Cunha-Filho, Francisco E
Speglich, Carlos
Araújo-Moreira, Fernando M
Pelc, Damjan
Cvitanić, Tonči
Požek, Miroslav
description Information on atomic-scale features is required for a better understanding of the mechanisms leading to magnetism in non-metallic, carbon-based materials. This work reports a direct evaluation of the hyperfine magnetic field produced at 13C nuclei in ferromagnetic graphite by nuclear magnetic resonance (NMR). The experimental investigation was made possible by the results of first-principles calculations carried out in model systems, including graphene sheets with atomic vacancies and graphite nanoribbons with edge sites partially passivated by oxygen. A similar range of maximum hyperfine magnetic field values (18-21T) was found for all systems, setting the frequency span to be investigated in the NMR experiments; accordingly, a significant 13C NMR signal was detected close to this range without any external applied magnetic field in ferromagnetic graphite.
doi_str_mv 10.48550/arxiv.1406.1119
format Article
fullrecord <record><control><sourceid>proquest_arxiv</sourceid><recordid>TN_cdi_arxiv_primary_1406_1119</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2084509569</sourcerecordid><originalsourceid>FETCH-LOGICAL-a519-3179d334c1611b68596aee077b696e9de2e748d738bc165c42692e3e88aea00d3</originalsourceid><addsrcrecordid>eNo9j01Lw0AURQdBsNTuXUnAdeJ78z1LKWqFgpvuh0nyUqe0SZykYv-9qRVXFy6Hyz2M3SEU0ioFjyF9x68CJegCEd0Vm3EhMLeS8xu2GIYdAHBtuFJixvjq1FNqYkvZIWxbGmOVNZH2dRbbrKGUuv96m0L_EUe6ZddN2A-0-Ms527w8b5arfP3--rZ8WudBocsFGlcLISvUiKW2yulABMaU2mlyNXEy0tZG2HJCVCW5dpwEWRsoANRizu4vs78-vk_xENLJn7382WsCHi5An7rPIw2j33XH1E6XPAcrFTilnfgB9uBO3w</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2084509569</pqid></control><display><type>article</type><title>Hyperfine magnetic field in ferromagnetic graphite</title><source>Freely Accessible Journals</source><source>arXiv.org</source><creator>Freitas, Jair C C ; Scopel, Wanderlã L ; Paz, Wendel S ; Bernardes, Leandro V ; Cunha-Filho, Francisco E ; Speglich, Carlos ; Araújo-Moreira, Fernando M ; Pelc, Damjan ; Cvitanić, Tonči ; Požek, Miroslav</creator><creatorcontrib>Freitas, Jair C C ; Scopel, Wanderlã L ; Paz, Wendel S ; Bernardes, Leandro V ; Cunha-Filho, Francisco E ; Speglich, Carlos ; Araújo-Moreira, Fernando M ; Pelc, Damjan ; Cvitanić, Tonči ; Požek, Miroslav</creatorcontrib><description>Information on atomic-scale features is required for a better understanding of the mechanisms leading to magnetism in non-metallic, carbon-based materials. This work reports a direct evaluation of the hyperfine magnetic field produced at 13C nuclei in ferromagnetic graphite by nuclear magnetic resonance (NMR). The experimental investigation was made possible by the results of first-principles calculations carried out in model systems, including graphene sheets with atomic vacancies and graphite nanoribbons with edge sites partially passivated by oxygen. A similar range of maximum hyperfine magnetic field values (18-21T) was found for all systems, setting the frequency span to be investigated in the NMR experiments; accordingly, a significant 13C NMR signal was detected close to this range without any external applied magnetic field in ferromagnetic graphite.</description><identifier>EISSN: 2331-8422</identifier><identifier>DOI: 10.48550/arxiv.1406.1119</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Carbon 13 ; Ferromagnetic resonance ; Ferromagnetism ; First principles ; Graphene ; Graphite ; Magnetic fields ; Magnetism ; NMR ; Nuclear magnetic resonance ; Physics - Materials Science</subject><ispartof>arXiv.org, 2014-06</ispartof><rights>2014. This work is published under http://arxiv.org/licenses/nonexclusive-distrib/1.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><rights>http://arxiv.org/licenses/nonexclusive-distrib/1.0</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>228,230,776,780,881,27902</link.rule.ids><backlink>$$Uhttps://doi.org/10.1038/srep14761$$DView published paper (Access to full text may be restricted)$$Hfree_for_read</backlink><backlink>$$Uhttps://doi.org/10.48550/arXiv.1406.1119$$DView paper in arXiv$$Hfree_for_read</backlink></links><search><creatorcontrib>Freitas, Jair C C</creatorcontrib><creatorcontrib>Scopel, Wanderlã L</creatorcontrib><creatorcontrib>Paz, Wendel S</creatorcontrib><creatorcontrib>Bernardes, Leandro V</creatorcontrib><creatorcontrib>Cunha-Filho, Francisco E</creatorcontrib><creatorcontrib>Speglich, Carlos</creatorcontrib><creatorcontrib>Araújo-Moreira, Fernando M</creatorcontrib><creatorcontrib>Pelc, Damjan</creatorcontrib><creatorcontrib>Cvitanić, Tonči</creatorcontrib><creatorcontrib>Požek, Miroslav</creatorcontrib><title>Hyperfine magnetic field in ferromagnetic graphite</title><title>arXiv.org</title><description>Information on atomic-scale features is required for a better understanding of the mechanisms leading to magnetism in non-metallic, carbon-based materials. This work reports a direct evaluation of the hyperfine magnetic field produced at 13C nuclei in ferromagnetic graphite by nuclear magnetic resonance (NMR). The experimental investigation was made possible by the results of first-principles calculations carried out in model systems, including graphene sheets with atomic vacancies and graphite nanoribbons with edge sites partially passivated by oxygen. A similar range of maximum hyperfine magnetic field values (18-21T) was found for all systems, setting the frequency span to be investigated in the NMR experiments; accordingly, a significant 13C NMR signal was detected close to this range without any external applied magnetic field in ferromagnetic graphite.</description><subject>Carbon 13</subject><subject>Ferromagnetic resonance</subject><subject>Ferromagnetism</subject><subject>First principles</subject><subject>Graphene</subject><subject>Graphite</subject><subject>Magnetic fields</subject><subject>Magnetism</subject><subject>NMR</subject><subject>Nuclear magnetic resonance</subject><subject>Physics - Materials Science</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><sourceid>GOX</sourceid><recordid>eNo9j01Lw0AURQdBsNTuXUnAdeJ78z1LKWqFgpvuh0nyUqe0SZykYv-9qRVXFy6Hyz2M3SEU0ioFjyF9x68CJegCEd0Vm3EhMLeS8xu2GIYdAHBtuFJixvjq1FNqYkvZIWxbGmOVNZH2dRbbrKGUuv96m0L_EUe6ZddN2A-0-Ms527w8b5arfP3--rZ8WudBocsFGlcLISvUiKW2yulABMaU2mlyNXEy0tZG2HJCVCW5dpwEWRsoANRizu4vs78-vk_xENLJn7382WsCHi5An7rPIw2j33XH1E6XPAcrFTilnfgB9uBO3w</recordid><startdate>20140604</startdate><enddate>20140604</enddate><creator>Freitas, Jair C C</creator><creator>Scopel, Wanderlã L</creator><creator>Paz, Wendel S</creator><creator>Bernardes, Leandro V</creator><creator>Cunha-Filho, Francisco E</creator><creator>Speglich, Carlos</creator><creator>Araújo-Moreira, Fernando M</creator><creator>Pelc, Damjan</creator><creator>Cvitanić, Tonči</creator><creator>Požek, Miroslav</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><scope>GOX</scope></search><sort><creationdate>20140604</creationdate><title>Hyperfine magnetic field in ferromagnetic graphite</title><author>Freitas, Jair C C ; Scopel, Wanderlã L ; Paz, Wendel S ; Bernardes, Leandro V ; Cunha-Filho, Francisco E ; Speglich, Carlos ; Araújo-Moreira, Fernando M ; Pelc, Damjan ; Cvitanić, Tonči ; Požek, Miroslav</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a519-3179d334c1611b68596aee077b696e9de2e748d738bc165c42692e3e88aea00d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Carbon 13</topic><topic>Ferromagnetic resonance</topic><topic>Ferromagnetism</topic><topic>First principles</topic><topic>Graphene</topic><topic>Graphite</topic><topic>Magnetic fields</topic><topic>Magnetism</topic><topic>NMR</topic><topic>Nuclear magnetic resonance</topic><topic>Physics - Materials Science</topic><toplevel>online_resources</toplevel><creatorcontrib>Freitas, Jair C C</creatorcontrib><creatorcontrib>Scopel, Wanderlã L</creatorcontrib><creatorcontrib>Paz, Wendel S</creatorcontrib><creatorcontrib>Bernardes, Leandro V</creatorcontrib><creatorcontrib>Cunha-Filho, Francisco E</creatorcontrib><creatorcontrib>Speglich, Carlos</creatorcontrib><creatorcontrib>Araújo-Moreira, Fernando M</creatorcontrib><creatorcontrib>Pelc, Damjan</creatorcontrib><creatorcontrib>Cvitanić, Tonči</creatorcontrib><creatorcontrib>Požek, Miroslav</creatorcontrib><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science &amp; Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering Collection</collection><collection>arXiv.org</collection><jtitle>arXiv.org</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Freitas, Jair C C</au><au>Scopel, Wanderlã L</au><au>Paz, Wendel S</au><au>Bernardes, Leandro V</au><au>Cunha-Filho, Francisco E</au><au>Speglich, Carlos</au><au>Araújo-Moreira, Fernando M</au><au>Pelc, Damjan</au><au>Cvitanić, Tonči</au><au>Požek, Miroslav</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Hyperfine magnetic field in ferromagnetic graphite</atitle><jtitle>arXiv.org</jtitle><date>2014-06-04</date><risdate>2014</risdate><eissn>2331-8422</eissn><abstract>Information on atomic-scale features is required for a better understanding of the mechanisms leading to magnetism in non-metallic, carbon-based materials. This work reports a direct evaluation of the hyperfine magnetic field produced at 13C nuclei in ferromagnetic graphite by nuclear magnetic resonance (NMR). The experimental investigation was made possible by the results of first-principles calculations carried out in model systems, including graphene sheets with atomic vacancies and graphite nanoribbons with edge sites partially passivated by oxygen. A similar range of maximum hyperfine magnetic field values (18-21T) was found for all systems, setting the frequency span to be investigated in the NMR experiments; accordingly, a significant 13C NMR signal was detected close to this range without any external applied magnetic field in ferromagnetic graphite.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><doi>10.48550/arxiv.1406.1119</doi><oa>free_for_read</oa></addata></record>
fulltext fulltext
identifier EISSN: 2331-8422
ispartof arXiv.org, 2014-06
issn 2331-8422
language eng
recordid cdi_arxiv_primary_1406_1119
source Freely Accessible Journals; arXiv.org
subjects Carbon 13
Ferromagnetic resonance
Ferromagnetism
First principles
Graphene
Graphite
Magnetic fields
Magnetism
NMR
Nuclear magnetic resonance
Physics - Materials Science
title Hyperfine magnetic field in ferromagnetic graphite
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-08T07%3A14%3A10IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_arxiv&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Hyperfine%20magnetic%20field%20in%20ferromagnetic%20graphite&rft.jtitle=arXiv.org&rft.au=Freitas,%20Jair%20C%20C&rft.date=2014-06-04&rft.eissn=2331-8422&rft_id=info:doi/10.48550/arxiv.1406.1119&rft_dat=%3Cproquest_arxiv%3E2084509569%3C/proquest_arxiv%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2084509569&rft_id=info:pmid/&rfr_iscdi=true